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Two-dimensional Ruddlesden-Popper hybrid lead halide perovskites have become a major topic in perovskite optoelectronics. Here, we aim to unravel the ultrafast dynamics governing the evolution of charge carriers and excitons in these…

Applied Physics · Physics 2020-09-02 Andrés Burgos-Caminal , Etienne Socie , Marine E. F. Bouduban , Jacques-E. Moser

Two-dimensional perovskites, in which inorganic layers are stabilized by organic spacer molecules, are attracting increasing attention as a more robust analogue to the conventional three-dimensional metal-halide perovskites. However,…

Excitons in two dimensional Ruddlesden Popper perovskites (RPPs) exhibit large and tunable binding energies, making them promising candidates for optoelectronic applications. In particular, long-range exciton energy transfer in these…

Two-dimensional (2D) organic-inorganic hybrid perovskites emerged as a versatile platform for light-emitting and photovol-taic applications due to their unique structural design and chemical flexibility. Their properties depend heavily on…

Two-dimensional halide perovskites are among intensely studied materials platforms profiting from solution based growth and chemical flexibility. They feature exceptionally strong interactions among electronic, optical as well as…

Two-dimensional hybrid perovskites are currently in the spotlight of condensed matter and nanotechnology research due to their intriguing optoelectronic and vibrational properties with emerging potential for light-harvesting and -emitting…

Lead halide perovskites have emerged as platforms for exciton-polaritonic studies at room temperature thanks to their excellent photoluminescence efficiency and synthetic versatility. In this work we find proof of strong exciton-photon…

Materials Science · Physics 2024-05-07 Maximilian Black , Mehdi Asadi , Parsa Darman , Finja Schillmöller , Sara Darbari , Nahid Talebi

Realizing semiconductors with high symmetry of their crystallographic structures has been a virtue of inorganic materials and has resulted in novel physical behaviors. In contrast, hybrid (organic and inorganic) crystals such as…

Photogenerated carrier transport and recombination in metal halide perovskites are critical to device performance. Despite considerable efforts, sample quality issues and measurement techniques have limited the access to their intrinsic…

Halide perovskites are known for their rich phase diagram and superior performance in diverse optoelectronics applications. The latter property is often attributed to the long electron-hole recombination time, whose underlying physical…

Two-dimensional halide perovskite nanoplatelets (NPLs) have exceptional light-emitting properties, including wide spectral tunability, ultrafast radiative decays, high quantum yields (QY), and oriented emission. To realize efficient…

Quasi two-dimensional (2D) colloidal synthesis made quantum confinement readily accessible in perovskites, generating additional momentum in perovskite LED research and lasing. Ultrathin perovskite layers exhibit high exciton binding…

Materials Science · Physics 2024-09-04 André Niebur , Eugen Klein , Rostyslav Lesyuk , Christian Klinke , Jannika Lauth

Halide perovskites offer a great platform for room-temperature exciton-polaritons (EPs) due to their strong oscillator strength and large exciton binding energy, promising applications in next-generation photonic and polaritonic devices.…

Layered hybrid perovskites containing larger organic cations have demonstrated superior environmental stability, but the presence of these insulating spacers also strengthens the exciton binding energy, which contributes to reduced carrier…

Semiconductor nanocrystals could replace conventional bulk materials completely in displays and light-emitting diodes. Exciton transport dominates over charge carrier transport for materials with high exciton binding energies and long…

Layered halide perovskites exhibit remarkable optoelectronic properties and technological promise, driven by strongly bound excitons. The interplay of spin-orbit and exchange coupling creates a rich excitonic landscape, determining their…

Two-dimensional (2D) perovskite materials have recently re-attracted intense research interest for applications in photovoltaics and optoelectronics. As a consequence of the dielectric and quantum confinement effect, they show strongly…

Understanding energy transport in semiconductors is critical for design of electronic and optoelectronic devices. Semiconductor material properties such as charge carrier mobility or diffusion length are commonly measured in bulk crystals…

Understanding the nature and energy distribution of optical resonances is of central importance in low-dimensional materials$^{1-4}$ and its knowledge is critical for designing efficient optoelectronic devices. Ruddlesden-Popper halide…

We study theoretically the excitonic nonlinearity in hybrid organic-inorganic Ruddlesden-Popper perovskite thin films. The composite layered structure of these materials allows for flexible modulation of their excitonic response between the…

Mesoscale and Nanoscale Physics · Physics 2022-11-14 D. A. Baghdasaryan , E. S. Hakobyan , D. B. Hayrapetyan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan
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