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Heat transport in bulk materials is well described using the Debye theory of 3D vibrational modes (phonons) and the acoustic match model. However, in cryogenic nanodevices, phonon wavelengths exceed device dimensions, leading to confinement…

Mesoscale and Nanoscale Physics · Physics 2024-10-14 M. Sidorova , A. D. Semenov , A. Zaccone , I. Charaev , M. Gonzalez , A. Schilling , S. Gyger , S. Steinhauer

Zero-mode waveguides (ZMWs) are confining light into attoliter volumes, enabling single molecule fluorescence experiments at physiological micromolar concentrations. Among the fluorescence spectroscopy techniques that can be enhanced by…

Organic-inorganic halide perovskite solar cells have attracted much attention due to their low-cost fabrication, flexibility, and high-power conversion efficiency. More recent efforts show that the reduction from three- to two-dimensions…

Materials Science · Physics 2021-09-03 Rahul Singh , Prashant Singh , Ganesh Balasubramania

Resonance energy transfer (RET) is an inherently anisotropic process. Even the simplest, well-known F\"orster theory, based on the transition dipole-dipole coupling, implicitly incorporates the anisotropic character of RET. In this…

Chemical Physics · Physics 2017-03-23 Gabriel Gil , Stefano Corni , Alain Delgado , Andrea Bertoni , Guido Goldoni

Strongly bound excitons confined in two-dimensional (2D) semiconductors are dipoles with a perfect in-plane orientation. In a vertical stack of semiconducting 2D crystals, such in-plane excitonic dipoles are expected to efficiently couple…

Metal halide perovskites are attracting tremendous interest for a variety of optoelectronic applications. The ability to tune the perovskite bandgap by tweaking the chemical compositions opens up new applications as coloured emitters and as…

Halide perovskite nanocrystals (NCs) have emerged as a promising material for applications ranging from light-emitting diodes (LEDs) to solar cells and photodetectors. Still, several issues impede the realization of the nanocrystals' full…

Energy transfer from photoexcited zero-dimensional systems to metallic systems plays a prominent role in modern day materials science. A situation of particular interest concerns the interaction between a photoexcited dipole and an…

Chemical Physics · Physics 2013-04-30 Zheyuan Chen , Stéphane Berciaud , Colin Nuckolls , Tony F. Heinz , Louis E. Brus

Understanding how dielectric anisotropy governs excitonic behavior in two-dimensional (2D) halide perovskites is critical for predicting and engineering their optoelectronic properties. In this work, we investigate Cs(n+1)PbnBr3n+1…

Hybrid halide perovskite semiconductors exhibit complex, dynamical disorder while also harboring properties ideal for optoelectronic applications that include photovoltaics. However, these materials are structurally and compositionally…

Materials Science · Physics 2020-12-10 Eve M. Mozur , James R. Neilson

Mixed-halide lead perovskites, with photoexcited charge-carrier properties suitable for high-efficiency photovoltaics, hold significant promise for high-efficiency tandem solar cells. However, phase segregation under illumination, where an…

We describe a strategy for conversion of optical power into DC electrical power using resonant absorption in plasmonic nanostructures. A thermodynamic analysis of the underlying mechanism motivates our description of the phenomenon, which…

Mesoscale and Nanoscale Physics · Physics 2012-02-03 Matthew T. Sheldon , Harry A. Atwater

The new class of hybrid organic-inorganic semiconductor (HOIS) materials, based on halide perovskites, is constantly being pursued for applications such as Light Emitting Diodes (LEDs) and solar cells, due to their momentous optoelectronic…

Metal halide perovskites possess desirable optical, material, and electrical properties which have had substantial impact on next-generation optoelectronics. However, given the toxicity of lead, alternative lead-free perovskite…

Halide perovskites are a versatile class of semiconductors employed for high performance emerging optoelectronic devices, including flexoelectric systems, yet the influence of their ionic nature on their mechanical behaviour is still to be…

Whilst electron correlations were previously recognized to trigger beyond conventional direct current (DC) electronic transportations (e.g. metal-to-insulator transitions, bad metal, thermistors), their respective influences to the…

Materials Science · Physics 2020-03-17 Jikun Chen , Haifan Li , Jiaou Wang , Xinyou Ke , Binghui Ge , Jinhao Chen , Hongliang Dong , Yong Jiang , Nuofu Chen

Physical reservoir computing is a promising framework for efficient neuromorphic in and near-sensor computing applications. Here, we demonstrate a multimodal optoelectronic reservoir network based on halide perovskite semiconductor devices,…

Materials Science · Physics 2025-08-28 Jeroen J. de Boer , Agustin O. Alvarez , Moritz C. Schmidt , Bruno Ehrler

Chalcogenide perovskites have emerged as non-toxic and stable photovoltaic materials, acting as an alternative to lead halide hybrid perovskites having similar optoelectronic properties. In the present work, we report the electronic and…

Materials Science · Physics 2021-06-03 Manish Kumar , Arunima Singh , Deepika Gill , Saswata Bhattacharya

Halide perovskites have emerged as promising materials for next-generation photovoltaics, laser sources and X-ray detectors. There is intense debate as to whether some photoactive halide perovskites exhibit ferroelectric behaviour and…

Materials Science · Physics 2026-01-21 Weilun Li , Qimu Yuan , Michael B. Johnston , Joanne Etheridge

The family of hybrid organic-inorganic lead-halide perovskites are the subject of intense interest for optoelectronic applications, from light-emitting diodes to photovoltaics to X-ray detectors. Due to the inert nature of most organic…

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