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The influence of oscillating quadrupole fields on atomic energy levels is examined theoretically and general expressions for the quadrupole matrix elements are given. The results are relevant to any ion-based clock in which one of the clock…

Quantum Physics · Physics 2019-03-06 Kyle J. Arnold , R. Kaewuan , T. R. Tan , M. D. Barrett

By employing singles, doubles, and triples excitations within the relativistic coupled-cluster framework, we perform comprehensive calculations of a wide range of atomic properties for the Th$^{3+}$ ion. These properties are essential for…

Atomic Physics · Physics 2026-05-06 A. Chakraborty , B. K. Sahoo

Accurate values of electric dipole (E1) amplitudes along with their uncertainties for a number of transitions among low-lying states of Mg$^+$, Ca$^+$, Sr$^+$, and Ba$^+$ are listed by carrying out calculations using a relativistic…

Atomic Physics · Physics 2020-12-30 Mandeep Kaur , Danish Furekh Dar , B. K. Sahoo , Bindiya Arora

Our calculations have shown that the 5f_5/2-7s_1/2 23131 cm^{-1} transition from the ground state in the ion Th^{3+} is very sensitive to the temporal variation of the fine structure constant alpha (q=-75300 cm^{-1}). The line is very…

Atomic Physics · Physics 2010-04-29 V. V. Flambaum , S. G. Porsev

Electric polarizabilities of four low-J even-parity states and three low-J odd-parity states of atomic barium in the range $35,600 $ to $36,000\ $cm$^{-1}$ are investigated. The states of interest are excited (in an atomic beam) via an…

Atomic Physics · Physics 2007-05-23 Chih-Hao Li , S. M. Rochester , M. G. Kozlov , D. Budker

An ultrastable optical clock based on neutral atoms trapped in an optical lattice is proposed. Complete control over the light shift is achieved by employing the $5s^2 {}^1S_0 \to 5s5p {}^3P_0$ transition of ${}^{87}{\rm Sr}$ atoms as a…

Atomic Physics · Physics 2009-11-10 Hidetoshi Katori , Masao Takamoto , V. G. Pal'chikov , V. D. Ovsiannikov

The nucleus of 229Thorium presents a unique isomer state of very low energy and long lifetime, current estimates are around 7.8 eV and seconds to hours respectively. This nuclear transitions therefore is a promising candidate for a novel…

Atomic Physics · Physics 2013-04-18 G. A. Kazakov , M. Schreitl , G. Winkler , J. H. Sterba , G. Steinhauser , T. Schumm

The highest performance atomic clocks are based on interrogation of ultra-narrow optical transitions. There is now significant interest in developing these systems as a source of GNSS-independent time in deployed, dynamic environments. We…

The differential polarizability, due to near-infrared light at 1126 nm, of the 27Al+ 1S0 -> 3P0 clock transition is measured to be 4\pi\epsilon_0 x (1.6 +/- 0.5) x 10^{-31} m^3. This measurement is combined with experimental oscillator…

Demands from several areas of science and technology have lead to a worldwide search for accurate optical clocks with an uncertainty of 1 part in $10^{18}$, which is $10^{3}$ times more accurate than the present day cesium atomic clocks…

Atomic Physics · Physics 2017-08-23 Chiranjib Sur , K. V. P. Latha , Rajat K. Chaudhuri , B. P. Das , D. Mukherjee

We experimentally investigate an optical frequency standard based on the $^2S_{1/2} (F=0)\to {}^2F_{7/2} (F=3)$ electric octupole (\textit{E}3) transition of a single trapped $^{171}$Yb$^+$ ion. For the spectroscopy of this strongly…

Atomic and Molecular Clusters · Physics 2016-02-15 N. Huntemann , C. Sanner , B. Lipphardt , Chr. Tamm , E. Peik

A sharp resonance line that appears in three-photon transitions between the $^{1}S_{0}$ and $^{3}P_{0}$ states of alkaline earth and Yb atoms is proposed as an optical frequency standard. This proposal permits the use of the even isotopes,…

Optics · Physics 2007-05-23 Tao Hong , Claire Cramer , Warren Nagourney , E. N. Fortson

We present precise values of the dipole polarizabilities ($\alpha$) of the ground $\rm [4f^{14}6s] ~ ^2S_{1/2}$ and metastable $\rm [4f^{14} 5d] ~ ^2D_{3/2}$ states of Yb$^+$, that are %vital {\bf important} in reducing systematics in the…

Atomic Physics · Physics 2017-10-25 A. Roy , S. De , Bindiya Arora , B. K. Sahoo

We present a novel method for engineering an optical clock transition that is robust against external field fluctuations and is able to overcome limits resulting from field inhomogeneities. The technique is based on the application of…

Atomic Physics · Physics 2019-12-03 Nati Aharon , Nicolas Spethmann , Ian D. Leroux , Piet O. Schmidt , Alex Retzker

We report on an evaluation of an optical clock that uses the $\phantom{}^2S_{1/2} \rightarrow \phantom{}^2D_{5/2}$ transition of a single $^{88}$Sr$^+$ ion as the reference. In contrast to previous work, we estimate the effective…

We observe a weakly allowed optical transition of atomic ytterbium from the ground state to the metastable state $4f^{13}5d6s^2 \: (J=2)$ for all five bosonic and two fermionic isotopes with resolved Zeeman and hyperfine structures. This…

Atomic Physics · Physics 2023-04-18 Taiki Ishiyama , Koki Ono , Tetsushi Takano , Ayaki Sunaga , Yoshiro Takahashi

We study the prospects of using the electric quadrupole transitions from the ground states of Cu, Ag and Au to the metastable state $^2{\rm D}_{5/2}$ as clock transitions in optical lattice clocks. We calculate lifetimes, transition rates,…

Atomic Physics · Physics 2021-02-24 V. A. Dzuba , Saleh O. Allehabi , V. V. Flambaum , Jiguang Li , S. Schiller

The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary…

We report on a $^{88}$Sr$^{+}$ single-ion optical clock with an estimated fractional systematic uncertainty of $7.9\times 10^{-19}$. The low uncertainty is enabled by small rf losses, a thorough evaluation of the blackbody-radiation…

Atomic Physics · Physics 2025-10-02 T. Lindvall , T. Fordell , K. J. Hanhijärvi , M. Doležal , J. Rahm , S. Weyers , A. E. Wallin

We analyze an optical atomic clock using two-photon $5S_{1/2} \rightarrow 4D_J$ transitions in rubidium. Four one- and two-color excitation schemes to probe the fine-structure states $4D_{3/2}$ and $4D_{5/2}$ are considered in detail. We…

Atomic Physics · Physics 2024-10-04 Alisher Duspayev , Carlos Owens , Bineet Dash , Georg Raithel
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