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A simple theory for glassy polymeric mechanical response which accounts for large scale chain relaxation is presented. It captures the crossover from perfect-plastic response to strong strain hardening as the degree of polymerization $N$…

Soft Condensed Matter · Physics 2015-05-18 Robert S. Hoy , Corey S. O'Hern

We analyze the equlibrium statistics of a long linear homo-polymer chain confined in between two flat geometrical constraints under good solvent condition. The chain is ocupying two dimensional space and geometrical constraints are two…

Statistical Mechanics · Physics 2015-12-29 Pramod Kumar Mishra

We study the dynamics of a knot in a semiflexible polymer confined to a narrow channel of width comparable to the polymers' persistence length. Using a combination of Brownian dynamics simulations and a coarse-grained stochastic model, we…

Soft Condensed Matter · Physics 2008-08-14 Wolfram Mobius , Erwin Frey , Ulrich Gerland

This work presents a general and unified theory describing block copolymer self-assembly in the presence of free surfaces and nanoparticles in the context of Self-Consistent Filed Theory. Specifically, the derived theory applies to free and…

Soft Condensed Matter · Physics 2021-12-17 Daniil Bochkov , Ivana Bagaric , Gaddiel Ouaknin , Frederic Gibou

We study equilibrium shapes and shape transformations of a confined semiflexible chain inside a soft lipid tubule using simulations and continuum theories. The deformed tubular shapes and chain conformations depend on the relative magnitude…

Soft Condensed Matter · Physics 2020-06-11 Subhadip Biswas , Buddhapriya Chakrabarti

Polymer fibers consist of macromolecules oriented along the fiber axis. Better alignment of chains leads to an increased strength of the fiber. It is believed that the key factor preventing formation of a perfectly oriented fiber is…

Soft Condensed Matter · Physics 2022-10-03 Artem Petrov , Vladimir Yu. Rudyak , Alexander Chertovich

Understanding how highly symmetric, robust, monodisperse protein cages self-assemble can have major applications in various areas of bio-nanotechnology, such as drug delivery, biomedical imaging and gene therapy. We develop a model to…

Soft Condensed Matter · Physics 2018-09-11 Sanaz Panahandeh , Siyu Li , Roya Zandi

We consider ideal chains in a hypercubic lattice \mathbb{Z}^{d}, d\geq3, with a fixed ratio m of self-intersection per monomer. Despite the simplicity of the geometrical constraint, this model shows some interesting properties, such as a…

Statistical Mechanics · Physics 2011-11-09 Simone Franchini

Constitutive equations are derived for the time-dependent behavior of particle-reinforced elastomers at isothermal loading with finite strains. A rubbery polymer is modelled as a network of macromolecules bridged by junctions which can slip…

Materials Science · Physics 2007-05-23 Aleksey D. Drozdov , Al Dorfmann

In this chapter we review the rich behavior of polymer chains embedded in a quenched random environment. We first consider the problem of a Gaussian chain free to move in a random potential with short-ranged correlations. We derive the…

Disordered Systems and Neural Networks · Physics 2007-05-23 Yadin Y. Goldschmidt , Yohannes Shiferaw

A {\it new} formula for the force vs extension relation is derived from the discrete version of the so called {\it worm like chain} model. This formula correctly fits some recent experimental data on polymer stretching and some numerical…

Statistical Mechanics · Physics 2009-11-10 A. Rosa , T. X. Hoang , D. Marenduzzo , A. Maritan

We analyze the nonequilibrium dynamics of single inextensible semiflexible biopolymers as stretching forces are applied at the ends. Based on different (contradicting) heuristic arguments, various scaling laws have been proposed for the…

Soft Condensed Matter · Physics 2007-09-17 B. Obermayer , O. Hallatschek , E. Frey , K. Kroy

Single-chain elasticity of polyethylene at $\theta$ point up to 90% of stretching with respect to its contour length is computed by Monte-Carlo simulation of an atomistic model in continuous space. The elasticity law together with the…

Soft Condensed Matter · Physics 2009-11-07 John T. Titantah , Carlo Pierleoni , Jean-Paul Ryckaert

Lattice-field calculations are performed on a Gaussian polymer chain confined to move within the region defined by two fused spheres. The results of the calculations are in accord with recent experimental measurements and computer…

Condensed Matter · Physics 2009-10-31 S. Tsonchev , R. D. Coalson

Analytical relations for the mechanical response of single polymer chains are valuable for modeling purposes, on both the molecular and the continuum scale. These relations can be obtained using statistical thermodynamics and an idealized…

Statistical Mechanics · Physics 2023-10-02 Michael R. Buche , Meredith N. Silberstein , Scott J. Grutzik

We introduce an efficient, scalable Monte Carlo algorithm to simulate cross-linked architectures of freely-jointed and discrete worm-like chains. Bond movement is based on the discrete tractrix construction, which effects conformational…

Soft Condensed Matter · Physics 2010-12-27 Henry E. Amuasi , Cornelis Storm

We study the conformations of a semiflexible chain, confined in nano-scaled spherical cavities, under two distinct processes of confinement. Radial contraction and packaging are employed as two confining procedures. The former method is…

Soft Condensed Matter · Physics 2014-09-29 Arman Fathizadeh , Maziar Heidari , Behrouz Eslami-Mossallam , Mohammad Reza Ejtehadi

We consider the folding of a self-avoiding homopolymer on a lattice, with saturating hydrogen bond interactions. Our goal is to numerically evaluate the statistical distribution of the topological genus of pseudoknotted configurations. The…

Biomolecules · Quantitative Biology 2009-11-11 G. Vernizzi , P. Ribeca , H. Orland , A. Zee

We explore the transport features of a single flexible polymer chain that walks on a periodic ratchet potential coupled with spatially varying temperature. At steady state the polymer exhibits a fast unidirectional motion where the…

Soft Condensed Matter · Physics 2015-07-20 Mesfin Asfaw Taye

The freely rotating chain is one of the classic discrete models of a polymer in dilute solution. It consists of a broken line of N straight segments of fixed length such that the angle between adjacent segments is constant and the N-1…

Probability · Mathematics 2017-11-15 Philip Kilanowski , Peter March , Marko Samara