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Second-order nonlinear optical materials enable frequency doubling of light (second-harmonic generation, SHG), which is essential for optoelectronic applications ranging from materials characterization to quantum technologies. However,…

Materials Science · Physics 2026-03-25 Aubrey G. J. Nyiri , Michael J. Waters , James M. Rondinelli

Intense laser-driven nonlinear optical phenomena in two-dimensional (2D) nodal-line semimetals (NLS) exhibit complex mechanisms, particularly in the NbSi$_{x}$Te$_{2}$ material systems characterized by nonsymmorphic symmetry-protected band…

Optics · Physics 2025-08-25 Navdeep Rana , M. S. Mrudul , Amar Bharti , Sucharita Giri , Gopal Dixit

Nonlinear optics has long been a cornerstone of modern photonic technology, enabling a wide array of applications, from frequency conversion to the generation of ultrafast light pulses. Recent breakthroughs in two-dimensional (2D) materials…

Optics · Physics 2025-04-11 Liuxin Gu , You Zhou

All-optical signal processing based on nonlinear optical devices is promising for ultrafast information processing in optical communication systems. Recent advances in two-dimensional (2D) layered materials with unique structures and…

Optics · Physics 2024-03-07 David J. Moss

Recently, a lot of effort has been dedicated to developing next-generation optoelectronic devices based on two-dimensional materials, thanks to their unique optical properties that are significantly different from those of their bulk…

Despite being only a few atoms thick, single-layer two-dimensional (2D) materials display strong electron-photon interactions that could be utilized in efficient light modulators on extreme subwavelength scales. In various applications…

Mesoscale and Nanoscale Physics · Physics 2018-09-21 Sunny Gupta , Sharmila N. Shirodkar , Alex Kutana , Boris I. Yakobson

Nonlinear optics is of crucial importance in several fields of science and technology with applications in frequency conversion, entangled-photon generation, self-referencing of frequency combs, crystal characterization, sensing, and…

Optics · Physics 2022-09-19 O. Dogadov , C. Trovatello , B. Yao , G. Soavi , G. Cerullo

Two-dimensional (2D) materials with large band gaps and strong and tunable second-harmonic generation (SHG) coefficients play an important role in the miniaturization of deep-ultraviolet (DUV) nonlinear optical (NLO) devices. Despite the…

Mesoscale and Nanoscale Physics · Physics 2025-03-04 Linlin Liu , Congwei Xie , Abudukadi Tudi , Keith Butler , Zhihua Yang

Optical nonlinearities, one of the most fascinating properties of two-dimensional (2D) materials, are essential for exploring novel physics in 2D systems and developing next-generation nonlinear optical applications. While tremendous…

This article reviews the material properties that enable maximum optical response. We highlight theoretical results that enable shape-independent quantification of material "figures of merit," ranging from classical sum rules to more recent…

Optics · Physics 2020-04-30 Hyungki Shim , Zeyu Kuang , Owen D. Miller

Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…

Materials Science · Physics 2024-12-05 Simone Grillo , Elena Cannuccia , Maurizia Palummo , Olivia Pulci , Claudio Attaccalite

Nonlinear processes are at the core of many optical technologies including lasers, information processing, sensing, and security, and require optimised materials suitable for nanoscale integration. Here we demonstrate the emergence of a…

Optics · Physics 2018-01-03 B. Wells , A. Yu. Bykov , G. Marino , M. E. Nasir , A. V. Zayats , V. A. Podolskiy

The interplay of polarization and magnetism in materials with light can create rich nonlinear magneto-optical (NLMO) effects, and the recent discovery of two-dimensional (2D) van der Waals magnets provides remarkable control over NLMO…

Materials Science · Physics 2024-04-30 Dezhao Wu , Meng Ye , Haowei Chen , Yong Xu , Wenhui Duan

In this work, the polar tetrahedron [PN$_2$O$_2$] was revealed as a new deep-ultraviolet (deep-UV) nonlinear optically active unit. Accordingly, a thermodynamically stable compound (PNO) consisting of the polar [PN$_2$O$_2$] units was…

Optics · Physics 2022-08-29 Congwei Xie , Abudukadi Tudi , Artem R. Oganov

Nonlinear optical responses provide a powerful way to understand the microscopic interactions between laser fields and matter. They are critical for plenty of applications, such as in lasers, integrated photonic circuits, biosensing and…

As a novel layered noble metal dichalcogenide material, palladium diselenide (PdSe2) has attracted wide interest due to its excellent optical and electronic properties. In this work, a strong third-order nonlinear optical response of 2D…

Optics · Physics 2021-07-01 David Moss

Two-dimensional (2D) layered semiconductors with both ultrawide bandgap and strong second harmonic generation (SHG) are essential for expanding the nonlinear optical (NLO) applications to deep-ultraviolet (DUV) region in nanoscale.…

Mesoscale and Nanoscale Physics · Physics 2020-11-24 Lei Kang , Xiaomeng Liu , Zheshuai Lin , Bing Huang

The emerging two-dimensional (2D) materials exhibit a wide range of electronic properties, ranging from insulating hexagonal boron nitride, semiconducting transition metal dichalcogenides such as molybdenum disulfide, to semi-metallic…

Mesoscale and Nanoscale Physics · Physics 2014-12-01 Fengnian Xia , Han Wang , Di Xiao , Madan Dubey , Ashwin Ramasubramaniam

The optical properties of two-dimensional materials are exceptional in several respects. They are highly anisotropic and frequently dominated by excitonic effects. Dipole-allowed second order non-linear optical properties require broken…

Mesoscale and Nanoscale Physics · Physics 2023-07-05 M. F. C. Martins Quintela , T. Garm Pedersen

In its 60 years of existence, the field of nonlinear optics has gained momentum especially over the past two decades thanks to major breakthroughs in material science and technology. In this article, we present a new set of data tables…

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