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Related papers: Rydberg Excitons in Synthetic Cuprous Oxide (Cu$_2…

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A novel, copper-based plasmonic system is presented to provide optical to microwave photon conversion. The process uses highly excited levels in Cu2O Rydberg excitons and takes advantage of spoof plasmons, which allow for significant…

Optics · Physics 2025-02-19 David Ziemkiewicz , Sylwia Zielińska-Raczyńska

We investigate the neutralization of charged defects in a Cu$_2$O crystal experimentally with a cw two-color pump-probe setup. We demonstrate that the excitation of high-lying Rydberg excitons at low densities generates an enhancement of…

Mesoscale and Nanoscale Physics · Physics 2023-11-07 Julian Heckötter , Binodbihari Panda , Katharina Brägelmann , Marc Aßmann

In this study we analyze the transmission spectrum of a thin plate of Cuprous Oxide in the range of the absorption of the yellow exciton states with the coherent transfer matrix method. We demonstrate that, in contrast to the usual analysis…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Heinrich Stolz , Rico Schwartz , Julian Heckötter , Marc Aßmann , Dirk Semkat , Sjard O. Krüger , Manfred Bayer

Photonic materials are an emerging platform to explore quantum matter and quantum dynamics. The development of Rydberg electromagnetically induced transparency provided a clear route to strong interactions between individual optical…

Quantum Gases · Physics 2018-05-21 Alexandros Georgakopoulos , Ariel Sommer , Jonathan Simon

Rydberg atoms are currently a very fast advancing quantum platform. For many interesting and demanding applications, including quantum computation, fast detection of a Rydberg excitation or a Rydberg qubit for information readout would be…

Quantum Physics · Physics 2025-09-30 Jinjin Du , Thibault Vogt , Ningxuan Zheng , Wenhui Li

We use two-color pump-probe spectroscopy to study Rydberg excitons in Cu$_2$O in the presence of free carriers injected by above-band-gap excitation. Already at plasma densities $\rho_\text{eh}$ below one hundredth electron-hole pair per…

Materials Science · Physics 2018-09-12 J. Heckötter , M. Freitag , D. Fröhlich , M. Aßmann , M. Bayer , P. Grünwald , F. Schöne , D. Semkat , H. Stolz , S. Scheel

Owing to ring-strain, cyclic ketones exhibit complex excited-state dynamics with multiple competing photochemical channels active on the ultrafast timescale. While the excited-state dynamics of cyclobutanone after $\pi^{\ast}\leftarrow n$…

Chemical Physics · Physics 2024-02-15 Julien Eng , Conor Rankine , Thomas Penfold

We investigate the influence of a static, uncorrelated distribution of charged impurities on the spectrum of bound excitons in the copper oxide Cu$_{\text{2}}$O. We show that the statistical distribution of Stark shifts and ionisation rates…

Mesoscale and Nanoscale Physics · Physics 2020-06-19 Sjard Ole Krüger , Heinrich Stolz , Stefan Scheel

We have performed two-photon excitation via the 6P3/2 state to n=50-80 S or D Rydberg state in Bose-Einstein condensates of rubidium atoms. The Rydberg excitation was performed in a quartz cell, where electric fields generated by plates…

Atomic Physics · Physics 2015-06-04 M. Viteau , M. Bason , J. Radogostowicz , N. Malossi , O. Morsch , D. Ciampini , E. Arimondo

Two of the most striking experimental findings when investigating exciton spectra in cuprous oxide using high-resolution spectroscopy are the observability and the fine structure splitting of $F$ excitons reported by J. Thewes et al. [Phys.…

Engineering of the dielectric environment represents a powerful strategy to control the electronic and optical properties of two-dimensional (2D) materials without compromising their structural integrity. Here we show that the recent…

Materials Science · Physics 2020-11-18 Anders C. Riis-Jensen , Morten N. Gjerding , Saverio Russo , Kristian S. Thygesen

A mechanism for amplification of weak quadrupole transitions of Rydberg excitons in Cu$_2$O by a plasmonic nanostructure is investigated. The theoretical description of exciton-plasmon interaction is presented and a field averaging…

Optics · Physics 2025-07-17 David Ziemkiewicz , Sylwia Zielińska-Raczyńska

Rydberg excitons in transition metal dichalcogenides (TMDs) have emerged as a promising platform for investigating the properties of open quantum systems, thanks to their large binding energies(hundreds of meV). However, the study of…

Optics · Physics 2024-10-10 Xiaofeng Li , Jiaxing Tu , Zhanyunxin Du , Mingjie Zha , Xiao Li , Zhibo Liu

Cold Rydberg atoms are a promising platform for quantum technologies and combining them with optical waveguides has the potential to create robust quantum information devices. Here, we experimentally observe the excitation of cold rubidium…

The various decay mechanisms of excitons in cuprous oxide (Cu2O) are highly sensitive to defects which can relax selection rules. Here we report cryogenic hyperspectral imaging of exciton luminescence from cuprous oxide crystals grown via…

We study the ultrastrong driving of Rydberg excitons in Cu$_2$O by a microwave field. The effect of the field is studied using optical absorption spectroscopy, and through the observation of sidebands on the transmitted laser light. A model…

The coupling of weak light fields to Rydberg states of atoms under conditions of electromagnetically induced transparency (EIT) leads to the formation of Rydberg polaritons which are quasi-particles with tunable effective mass and…

Quantum Physics · Physics 2013-09-17 Johannes Otterbach , Matthias Moos , Dominik Muth , Michael Fleischhauer

We demonstrate the single-photon Rydberg excitation of cesium atoms in a magneto-optical trap (MOT). We excite atoms directly from ${{6S}_{1/2}}$ ground state to ${{nP}_{3/2}}(n=70-100)$ Rydberg state with a narrow-linewidth 319 nm…

Atomic Physics · Physics 2019-11-22 Jiandong Bai , Shuo Liu , Jieying Wang , Jun He , Junmin Wang

We show that transient supersolid quantum states of Rydberg-excitations can be created dynamically from a Mott insulator of ground state atoms in a 2D optical-lattices by irradiating it with short laser pulses. The structure of these…

Quantum Physics · Physics 2011-08-05 P. -L. Giscard , D. Jaksch

Monolayer transition metal dichalcogenide (TMDC) semiconductors exhibit strong excitonic optical resonances which serve as a microscopic, non-invasive probe into their fundamental properties. Like the hydrogen atom, such excitons can…

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