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A comprehensive study of second harmonic generation on thermally oxidized MoS2 flakes with thickness ranging from monolayer up to seven layers is presented. Observing the fundamental nonlinear behavior for non-treated and oxidized MoS2…

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at…

We report the first fully self-consistent calculations of the nonlinear optical properties of superlattices. The materials investigated are mono-layer superlattices with GaP grown on the the top of InP, AlP and GaAs (110) substrates. We use…

Materials Science · Physics 2009-11-07 S. Sharma , J. K. Dewhurst , C. Ambrosch-Draxl

The phasing problem of heterodyne-detected nonlinear spectroscopy states that the relative time delay between the exciting pulses and a local oscillator must be known with subcycle precision to separate absorptive and dispersive…

Using the Jones matrix formalism, crystal optical properties of inhomogeneous material consisting of a pile of weakly birefringent plates are analysed in relation to the cell model adopted in polarization tomography of 3D dielectric tensor…

Optics · Physics 2007-09-04 O. Kushnir , P. Nek , R. Vlokh , N. Kukhtarev

We experimentally show an all-optical multipolar decomposition of the lowest-order Eigenmodes of a single gold nanoprism using azimuthally and radially polarized cylindrical vector beams. By scanning the particle through these tailored…

Optics · Physics 2015-03-10 Thomas Bauer , Sergej Orlov , Gerd Leuchs , Peter Banzer

We study the linear polarization properties of the photoluminescence of the neutral and negatively charged nitrogen vacancies and neutral vacancies in diamond crystals as function of their symmetry and their response to strong external…

Mesoscale and Nanoscale Physics · Physics 2018-03-28 D. Braukmann , V. P. Popov , E. R. Glaser , T. A. Kennedy , M. Bayer , J. Debus

Black phosphorus (P), a layered material that can be isolated down to individual 2D crystalline sheets, exhibits highly anisotropic mechanical properties due to its corrugated crystal structure in each atomic layer, which are intriguing for…

Mesoscale and Nanoscale Physics · Physics 2015-04-07 Zenghui Wang , Philip X. -L. Feng

Polarization-resolved second-harmonic spectra are obtained from the resonant modes of a two-dimensional planar photonic crystal microcavity patterned in a free-standing InP slab. The photonic crystal microcavity is comprised of a single…

We carried out a joint theoretical and experimental study of the polarization of high-order harmonics generated from ZnO by intense infrared laser pulses. Experimentally we found that the dependence of parallel and perpendicular…

The notion of spontaneous symmetry breaking has been used to describe phase transitions in a variety of physical systems. In crystalline solids, the breaking of certain symmetries, such as mirror symmetry, is difficult to detect…

Materials Science · Physics 2020-07-01 Bryan T. Fichera , Anshul Kogar , Linda Ye , Bilal Gökce , Alfred Zong , Joseph G. Checkelsky , Nuh Gedik

We analyze the occurrence of in-plane anisotropy in the electronic, magnetic, elastic and transport properties of more than one thousand 2D materials from the C2DB database. We identify hundreds of anisotropic materials and classify them…

Materials Science · Physics 2020-09-09 Luca Vannucci , Urko Petralanda , Asbjørn Rasmussen , Thomas Olsen , Kristian S. Thygesen

Crystallization from an amorphous atomic structure is usually seen as a spontaneous process in pursuit of a lower energy state, but for alloy systems it is often hard to elucidate because of the intrinsic structural and compositional…

Materials Science · Physics 2020-04-10 Y. Huang , L. Xie , D. S. He , J. Q. He

Black phosphorus has been the subject of growing interest due to its unique band structure that is both layer dependent and anisotropic. While many have studied the linear optical response of black phosphorus, the nonlinear response has…

Materials Science · Physics 2016-11-16 Nathan Youngblood , Ruoming Peng , Andrei Nemilentsau , Tony Low , Mo Li

The optical response of materials based on gold nanoparticle assemblies depends on many parameters regarding both material morphology and light excitation characteristics. In this paper, the interplay between the optical and thermal…

We analyze third-harmonic generation from high-index dielectric nanoparticles and discuss the basic features and multipolar nature of the parametrically generated electromagnetic fields near the Mie-type optical resonances. By combining…

Nonlinear phononics relies on the resonant optical excitation of infrared-active lattice vibrations to coherently induce targeted structural deformations in solids. This form of dynamical crystal-structure design has been applied to control…

Applied Physics · Physics 2021-05-19 Meredith Henstridge , Michael Först , Edward Rowe , Michael Fechner , Andrea Cavalleri

The optical response of metallic nanoparticle arrays is dominated by localized surface plasmon excitations and is the sum of individual particle contributions modified by inter-particle coupling depending on specific array geometry. Here we…

We report second- and third-harmonic generation in monolayer MoS$_\mathrm{2}$ as a tool for imaging and accurately characterizing the material's nonlinear optical properties under 1560 nm excitation. Using a surface nonlinear optics…

The paper suggests to treat the infrared reflectivity spectra of single crystal perovskite relaxors as fine-grained ferroelectric ceramics: locally frozen polarization makes the dielectric function strongly anisotropic in the phonon…

Materials Science · Physics 2009-11-11 J. Hlinka , T. Ostapchuk , D. Noujni , S. Kamba , J. Petzelt
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