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A coarse grained model for flexible polymers end-grafted to repulsive spherical nanoparticles is studied for various chain lengths and grafting densities under good solvent conditions, by Molecular Dynamics methods and density functional…

Soft Condensed Matter · Physics 2015-05-18 Federica Lo Verso , Sergei A. Egorov , Andrey Milchev , Kurt Binder

We report numerical investigations of a three-dimensional model of diffusive growth of fine particles, the internal structure of which corresponds to different crystal lattices. A growing cluster (particle) is immersed in, and exchanges…

Statistical Mechanics · Physics 2010-10-12 Vyacheslav Gorshkov , Alexandr Zavalov , Vladimir Privman

The fluid phase diagram of trimer particles composed of one central attractive bead and two repulsive beads was determined as a function of simple geometric parameters using flat-histogram Monte Carlo methods. A variety of self-assembled…

Soft Condensed Matter · Physics 2015-05-20 Harold W. Hatch , Jeetain Mittal , Vincent K. Shen

We investigate the chain conformation of ring polymers confined to a cylindrical nanochannel using both theoretical analysis and three dimensional Langevin dynamics simulations. We predict that the longitudinal size of a ring polymer scales…

Soft Condensed Matter · Physics 2012-12-06 Junfang Sheng , Kaifu Luo

We use computational modeling to investigate the assembly thermodynamics of a particle-based model for geometrically frustrated assembly, in which the local packing geometry of subunits is incompatible with uniform, strain-free large-scale…

Soft Condensed Matter · Physics 2021-09-06 Botond Tyukodi , Farzaneh Mohajerani , Douglas M. Hall , Gregory M. Grason , Michael F. Hagan

The bioactivity of nanoparticles crucially depends on their ability to cross biomembranes. Recent simulations indicate the cooperative wrapping and internalization of spherical nanoparticles in tubular membrane structures. In this article,…

Soft Condensed Matter · Physics 2014-01-09 Michael Raatz , Reinhard Lipowsky , Thomas R. Weikl

Co-assembly of inorganic nanoparticles (NPs) and nanostructured polymer matrix represents an intricate interplay of enthalpic or entropic forces. Particle size largely affects the phase behavior of the nanocomposite. Theoretical studies…

Soft Condensed Matter · Physics 2022-04-25 Le Ma , Hejin Huang , Peter Ercius , Alfredo Alexander-Katz , Ting Xu

We study equilibrium shapes and shape transformations of a confined semiflexible chain inside a soft lipid tubule using simulations and continuum theories. The deformed tubular shapes and chain conformations depend on the relative magnitude…

Soft Condensed Matter · Physics 2020-06-11 Subhadip Biswas , Buddhapriya Chakrabarti

Molecular self-assembly on surfaces constitutes a powerful method for creating tailor-made surface structures with dedicated functionalities. Varying the intermolecular interactions allows for tuning the resulting molecular structures in a…

Mesoscale and Nanoscale Physics · Physics 2020-07-24 Christoph Schiel , Maximilian Vogtland , Ralf Bechstein , Angelika Kühnle , Philipp Maass

Magnetic composite materials i.e. elastomers, polymer gels, or polymer solutions with embedded magnetic nanoparticles are useful for many technical and bio-medical applications. However, the microscopic details of the coupling mechanisms…

Soft Condensed Matter · Physics 2020-10-30 Patrick Kreissl , Christian Holm , Rudolf Weeber

We model the stabilization of clusters and lattices of cuboidal particles with long-ranged magnetic dipolar and short-ranged surface interactions. Two realistic systems were considered: one with magnetization orientated in the [001]…

Soft Condensed Matter · Physics 2020-09-09 Igor Stankovic , Luis Lizardi , Carlos Garcia

In living cells, proteins self-assemble into large functional structures based on specific interactions between molecularly complex patches. Due to this complexity, protein self-assembly results from a competition between a large number of…

Soft Condensed Matter · Physics 2024-12-10 Lara Koehler , Pierre Ronceray , Martin Lenz

Molecular Dynamics simulations of a coarse-grained bead-spring model of flexible macromolecules tethered with one end to the surface of a cylindrical pore are presented. Chain length $N$ and grafting density $\sigma$ are varied over a wide…

Soft Condensed Matter · Physics 2007-05-23 Dimitar I. Dimitrov , Andrey Milchev , Kurt Binder , Dieter W. Heermann

Nanothermodynamics extends standard thermodynamics to facilitate finite-size effects on the scale of nanometers. A key ingredient is Hill's subdivision potential that accommodates the non-extensive energy of independent small systems,…

Statistical Mechanics · Physics 2015-04-21 Ralph V. Chamberlin

Trapping macromolecules in nanopits finds multifarious applications in polymer separation, filtering biomolecules etc. However, tuning the locomotion of polymers in channels of nanoscopic dimensions is greatly restricted by the comparative…

Fluid Dynamics · Physics 2016-05-10 Sree Hari P D , Chirodeep Bakli , Suman Chakraborty

The change of the structure of concentrated colloidal suspensions upon addition of non-adsorbing polymer is studied within a two-component, Ornstein-Zernicke based liquid state approach. The polymers' conformational degrees of freedom are…

Soft Condensed Matter · Physics 2009-10-31 M. Fuchs , K. S. Schweizer

Self-assembly kinetics is usually described by approaches which assume that the shape of the aggregates has a definite form (e.g., spherical, cylindrical, cubic, etc), however that is unlikely to be the case in many finite-sized…

Soft Condensed Matter · Physics 2022-07-13 L. F. Trugilho , L. G. Rizzi

Granular and nanoscale materials containing a relatively small number of constituents have been studied to discover how their properties differ from their macroscopic counterparts. These studies are designed to test how far the known…

Statistical Mechanics · Physics 2007-05-23 A. K. Rajagopal , C. S. Pande , Sumiyoshi Abe

Nanochains of atoms, molecules and polymers have gained recent interest in the experimental sciences. This article contributes to an advanced mathematical modeling of the mechanical properties of nanochains that allow for heterogenities,…

Analysis of PDEs · Mathematics 2019-09-17 Laura Lauerbach , Stefan Neukamm , Mathias Schäffner , Anja Schlömerkemper

The nucleation of carbon nanotubes on small nickel clusters is studied using a tight binding model coupled to grand canonical Monte Carlo simulations. This technique closely follows the conditions of the synthesis of carbon nanotubes by…

Materials Science · Physics 2007-05-23 Hakim Amara , Christophe Bichara , François Ducastelle