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Gold-decorated TiO$_2$ nanotubes were used for the photocatalytic abatement of Hg(II) in aqueous solutions. The presence of dewetted Au nanoparticles induces a strong enhancement of photocatalytic reduction and scavenging performances, with…

In the present work we use TiO2 nanotube arrays, carrying a Pt coating that is optimally dewetted, as a photocatalyst to generate H2. In order to achieve a maximum H2-generation efficiency, on the one hand an ideal thermal dewetting of the…

Au nanoparticles at the TiO$_2$ surface can enhance the photocatalytic H$_2$ generation performances owing to their electron transfer co-catalytic ability. Key to maximize the co-catalytic effect is a fine control over Au nanoparticle size…

Applied Physics · Physics 2020-06-05 Seyedsina Hejazi , Marco Altomare , Shiva Mohajernia , Patrik Schmuki

Converting CO$_2$ to useful compounds through the solar photocatalytic reduction has been one of the most promising strategies for artificial carbon recycling. The highly relevant photocatalytic substrate for CO$_2$ conversion has been the…

Chemical Physics · Physics 2015-05-28 Shijing Tan , Yan Zhao , Jin Zhao , Zhuo Wang , Chuanxu Ma , Aidi Zhao , Bing Wang , Yi Luo , Jinlong Yang , Jianguo Hou

Substitutional doping with transition metals is carried out in the Lepidocrocite phase - the stable monolayer geometry of TiO$_2$, using density functional theory (DFT) methods. The doping is carried out at the differently coordinated O…

Materials Science · Physics 2024-10-14 Kati Asikainen , Matti Alatalo , Marko Huttula , S. Assa Aravindh

We apply high-energy proton ion-implantation to modify TiO2 nanotubes selectively at their tops. In the proton-implanted region we observe the creation of intrinsic co-catalytic centers for photocatalytic H2-evolution. We find proton…

Samples of nitrogen-doped titanium dioxide (anatase, $0.2 \leq N \leq 1.0~wt\%$) prepared by the sol-gel method were investigated using X-band EPR spectroscopy, photoconductivity and photocatalysis measurements. $N\bullet$ and $NO\bullet$…

Materials Science · Physics 2017-04-18 A. A. Minnekhanov , N. T. Le , E. A. Konstantinova , P. K. Kashkarov

Achieving both broad solar-spectrum absorption and strong redox capability is critical for semiconductor photocatalysts in environmental remediation and energy conversion. Herein, an S-scheme heterojunction photocatalyst is constructed by…

Materials Science · Physics 2026-03-31 Xiaoyi Zhou , Min Zhang , Qiushi Wang , Shiwen Du , Xuedong Jing , Zhenyi Zhang

Light chargeable metal-ion batteries using semiconductor heterostructures are gaining enormous interest. A few such heterostructures such as MoS2/MoOy and TiS2/TiO2 have been shown to function as photocathodes in photochargeable Li-ion…

Materials Science · Physics 2023-07-07 Raheel Hammad , Amar Kumar , Tharangattu N. Narayanan , Soumya Ghosh

Atomic and electronic structures of TiO_2(110) surface with possible adsorptional, substitutional and interstitial Au or Pt elemental impurities at full and one-sixth monolayer concentrations were investigated by density functional theory…

Strongly Correlated Electrons · Physics 2012-11-19 Ersen Mete , Oğuz Gülseren , Şinasi Ellialtıoğlu

Recently, van der Waals heterostructure has attracted interest both theoretically and experimentally for their potential applications in photoelectronic devices, photovoltaic devices, plasmonic devices and photocatalysis. Inspired by this,…

Materials Science · Physics 2021-02-09 Yilin Zhao , Hong Zhang , Xinlu Cheng

Overlaid self-ordering processes: we form anodic self-organized TiO2 nanostumps and exploit them for self-ordering dewetting of Au-Ag sputtered films. This forms ordered particle configurations at tube top (crown position) or bottom (ground…

Materials Science · Physics 2016-10-17 Nhat Truong Nguyen , Marco Altomare , JeongEun Yoo , Patrik Schmuki

We propose an alternative structure of TiO2 anatase that has a higher energy oxygen p-like valence band maximum than the pristine TiO2 anatase and thus has a much better alignment with the water splitting levels. This alternative structure…

Materials Science · Physics 2017-02-22 Sinisa Coh , Peter Y. Yu , Yuta Aoki , Susumu Saito , Steven G. Louie , Marvin L. Cohen

Titanium dioxide (TiO$_2$) thin films are commonly used as photocatalytic materials. Here, we enhance the photocatalytic activity of devices based on TiO$_2$ by combining nanostructured glass substrates with metallic plasmonic…

We investigate the photocatalytic performance of nanocomposites prepared in a one-step process by liquid-phase exfoliation of graphite in the presence of TiO$_2$ nanoparticles (NPs) at atmospheric pressure and in water, without heating or…

In this paper, I demonstrate a density functional theory plus dynamical mean field theory study on the electronic properties of doped $TiO_2$ rutile as well as another tetragonal phase anatase with oxygen vacancy. The density of states and…

Strongly Correlated Electrons · Physics 2021-12-24 S. Koley

The optical properties of thermally annealed TiO2 samples depend on their preparation process, and the TiO2 thin films usually exist in the form of anatase or rutile or the mixture of the two phases. The electronic structures and optical…

Materials Science · Physics 2016-11-29 Li Jinping , Meng Songhe , Qin Liyuan , Hantao Lu

Earth-abundant materials exhibiting Mie resonances across the visible and near-infrared offer opportunities for efficient and sustainable sensing, thermal regulation, and sunlight harvesting. For anatase TiO$_2$, a broadband optical and…

Materials Science · Physics 2025-11-14 Pedro Tartaj , Yurena Luengo , Pedro Moronta , Luisina Forzani , Alvaro Blanco , Cefe López

We show that mixed-phase titanium dioxide (TiO2) can be effectively employed as an unconventional, inorganic, dual-emitting and ratiometric optical sensor of O2. Simultaneous availability of rutile and anatase TiO2 PL and their peculiar…

Materials Science · Physics 2016-08-03 S. Lettieri , D. K. Pallotti , F. Gesuele , P. Maddalena

Configuring TiO2 into bicontinuous mesostructures greatly improves its photocatalytic efficiency. This is often ascribed to the expanded surface area. Yet, whether mesostructuring modulates TiO2's electronic structure and how that…

Materials Science · Physics 2023-10-23 Ying-Hao Lu , Bor Kae Chang , Yi-Fan Chen