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Amplitude and phase of wavepackets encode the dynamics of quantum systems. However, the rapidity of electron dynamics on the attosecond timescale has precluded their complete measurement in the time domain. Here, we demonstrate that…

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

Formulas to describe the photoabsorption and the photon scattering by a plasma or a liquid metal are derived in a unified manner with each other. It is shown how the nuclear motion, the free-electron motion and the core-electron behaviour…

Materials Science · Physics 2009-10-31 Junzo Chihara

The Epoch of Reionization marks the last major phase transition in the early Universe, during which the majority of neutral hydrogen once filling the intergalactic medium was ionized by the first galaxies. The James Webb Space Telescope is…

Astrophysics of Galaxies · Physics 2025-07-01 Cody Carr , Renyue Cen , Sophia Flury , Sally Oey , Stephan McCandliss , Allison Strom

I propose to consider photon tunneling as a space-time correlation phenomenon between the emission and absorption of a photon on the two sides of a barrier. Standard technics based on an appropriate counting rate formula may then be applied…

Quantum Physics · Physics 2007-05-23 Peter Hrasko

We present the first numerical simulation of the time delay in the photoionization of the simplest diatomic molecule H$_2^+$ as observed by attosecond streaking. We show that the strong variation of the Eisenbud-Wigner-Smith time delay as a…

We apply time-dependent R-matrix theory to study inner-shell ionization of C atoms in ultra-short high-frequency light fields with a photon energy between 170 and 245 eV. At an intensity of 10$^{17}$ W/cm$^2$, ionization is dominated by…

Atomic Physics · Physics 2015-08-12 H. F. Rey , H. W. van der Hart

We investigate laser induced nonsequential multiple ionization using a simple statistical model in which an electron recollides inelastically with its parent ion. In this collision, it thermalizes with the remaining $N-1$ bound electrons…

Atomic Physics · Physics 2007-05-23 C. Figueira de Morisson Faria , X. Liu

We study photon production in the early stage of heavy-ion collisions using a multistage model combining IP-Glasma, K\o{}MP\o{}ST and relativistic hydrodynamics. We discuss the small momentum anisotropy of these photons, highlighting the…

Nuclear Theory · Physics 2020-09-17 Charles Gale , Jean-François Paquet , Björn Schenke , Chun Shen

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

We calculate the photoionization cross-section of a molecular endohedral. We limit ourselves to two-atomic molecules. The consideration is much more complex than for atomic endohedrals because the system even for almost spherical fullerenes…

Atomic and Molecular Clusters · Physics 2019-09-04 M. Ya. Amusia , L. V. Chernysheva , S. K. Semenov

Photoionization cross sections and rate coefficients have been calculated for all bound vibrational levels of the 1s$\sigma_{\mathrm{g}}$ state of H$_{2}^{+}$, HD$^{+}$, and D$_{2}^{+}$. The Born-Oppenheimer approximation is employed in our…

Atomic Physics · Physics 2023-11-03 Adam Singor , Liam H. Scarlett , Mark C. Zammit , Igor Bray , Dmitry V. Fursa

Attosecond interferometry (AI) is an experimental technique based on ionizing a system with an attosecond pulse train in the presence of an assisting laser. This assisting laser provides multiple pathways for the photoelectron wave packet…

Chemical Physics · Physics 2020-10-07 Denis Jelovina , Armin Scrinzi , Hans Jakob Wörner , Axel Schild

How quanta of energy and charge are transported on both atomic spatial and ultrafast time scales is at the heart of modern technology. Recent progress in ultrafast spectroscopy has allowed us to directly study the dynamical response of an…

Other Condensed Matter · Physics 2015-04-28 R. Locher , L. Castiglioni , M. Lucchini , M. Greif , L. Gallmann , J. Osterwalder , M. Hengsberger , U. Keller

Photo-ionization induced ultrafast electron dynamics is considered as a precursor to the slower nuclear dynamics associated with molecular dissociation. Here, using ab initio multielectron wave-packet propagation method, we study the…

Chemical Physics · Physics 2022-11-30 K. Chordiya , V. Despré , B. Nagyillés , F. Zeller , Z. Diveki , A. I. Kuleff , M. U. Kahaly

The mediated photon-photon interaction due to the resonant Kerr nonlinearity in an inhomogeneously broadened atomic vapor is considered. The time-scale for photon-photon scattering is computed and found to be determined by the inhomogeneous…

Optics · Physics 2009-11-06 M. W. Mitchell , R. Y. Chiao

Extracting single photoionization time delays associated with atomic (or molecular) species from attosecond time scale two-photon experiments usually relies on the theoretical description of continuum-continuum transitions. The available…

Atomic Physics · Physics 2022-08-29 D. I. R. Boll , L. Martini , O. A. Fojón

We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…

We study time-delays in atomic multiphoton ionization (MPI) using the phase-sensitive detection of photoelectron vortices. Photoelectron vortices are created by MPI with counter-rotating circularly polarized (CRCP) ultrashort double pulse…

Atomic Physics · Physics 2025-01-13 D. Köhnke , T. Bayer , M. Wollenhaupt