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The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10-120 Hz) and the…

Various schemes are presented for the generation of circularly polarized molecular high-order harmonic generation (MHOHG) from molecules. In particular it is shown that combinations of counter-rotating circularly polarized pulses produce…

Optics · Physics 2015-12-15 Andre D. Bandrauk , Kai-Jun Yuan

The interaction between an ultrastrong laser and a cone-like target is an efficient approach to generate high power radiations like attosecond pulses and terahertz waves. The object is to study the $\gamma$-ray generation under this…

Plasma Physics · Physics 2022-06-28 Cui-Wen Zhang , Yi-Xuan Zhu , Jian-Feng Lv , Bai-Song Xie

The interaction of intense femtosecond laser pulses with atomic Argon clusters has been investigated by using nano-plasma model. Based on the dynamic simulations, ionization process, heating and expansion of a cluster after irradiation by…

Atomic and Molecular Clusters · Physics 2016-08-15 H. Ghaforyan , R. Sadighi , E. Irani

The field of attosecond physics has expanded significantly in recent years, yet experimental facilities supporting attosecond pump attosecond probe spectroscopy remain rare. Here, we present a newly constructed beamline for the generation…

Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high…

Atomic Physics · Physics 2020-01-08 D. Hammerland , P. Zhang , S. Kuehn , P. Jojart , I. Seres , V. Zuba , Z. Varallyay , K. Osvay , T. T. Luu , H. J. Woerner

We consider several aspects of high-order harmonic generation in solids: the effects of elastic and inelastic scattering; varying pulse characteristics; and inclusion of material-specific parameters through a realistic band structure. We…

Other Condensed Matter · Physics 2013-02-07 A. F. Kemper , B. Moritz , J. K. Freericks , T. P. Devereaux

The interaction of relativistically strong tailored laser pulses with an atomic system is considered. Due to a special tailoring of the laser pulse, the suppression of the relativistic drift of the ionized electron and a dramatic…

Atomic Physics · Physics 2007-05-23 M. Klaiber , K. Z. Hatsagortsyan , C. H. Keitel

Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…

Atomic and Molecular Clusters · Physics 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

High harmonic spectra generated in condensed matter carry the fingerprints of sub-cycle electronic motion and the energy structure of the studied system. Here we show that tailoring the waveform of mid-infrared driving light by using a…

A method is proposed for arbitrarily engineering the high-order harmonic generation phase achieved by shaping a laser pulse and employing xuv light or x rays for ionization. This renders the production of bandwidth-limited attosecond pulses…

Atomic Physics · Physics 2011-02-25 Markus C. Kohler , Christoph H. Keitel , Karen Z. Hatsagortsyan

We present calculation of photoexcitation and high-harmonic generation in bulk diamond induced by intense near-infrared laser pulse of photon energy 1.55 eV, time duration of 15 fs and peak field strength $F=$ 0.4 V/{\AA}. Depending on the…

Atomic Physics · Physics 2018-10-31 T. Apostolova , B. Obreshkov

High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…

We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…

Coherent time is a characteristic time in the extreme nonlinear optics regime and thus generally introduced as the dephasing time in the simulations of the solid-state high-harmonic generation. This characteristic time linked with the…

Optics · Physics 2019-11-13 Tao-Yuan Du

Anomalously high generation efficiency of coherent higher field-harmonics in collisions between {\em oppositely charged particles} in the field of femtosecond lasers is predicted. This is based on rigorous numerical solutions of a quantum…

Condensed Matter · Physics 2009-10-31 H. Haberland , M. Bonitz , D. Kremp

We propose a real-time time-dependent ab__initio approach within a configuration-interaction-singles ansatz to decompose the high-harmonic generation (HHG) signal of molecules in terms of individual molecular-orbital (MO) contributions.…

Chemical Physics · Physics 2025-12-11 Marco Marchetta , Chiara Morassut , Julien Toulouse , Emanuele Coccia , Eleonora Luppi

Present ultra-fast laser optics is at the frontier between atto- and zeptosecond photon pulses, giving rise to unprecedented applications. We show that high-energetic photon pulses down to the yoctosecond timescale can be produced in heavy…

High Energy Physics - Phenomenology · Physics 2010-05-28 Andreas Ipp , Christoph H. Keitel , Jörg Evers

High-order harmonic generation (HHG) is investigated for H$_2^+$ and its isotopomers under seven- and ten-cycle trapezoidal laser pulses at 800 nm wavelength and $I$=4$\times 10^{14}$ W$/$cm$^2$ intensity. We solved numerically…

Atomic Physics · Physics 2016-03-03 H. Ahmadi , M. Vafaee , A. Maghari