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Soft particles display highly versatile properties with respect to hard colloids, even more so at fluid-fluid interfaces. In particular, microgels, consisting of a cross-linked polymer network, are able to deform and flatten upon adsorption…

The ability to assemble mesoscopic colloidal lattices above a surface is important for fundamental studies related with nucleation and crystallization, but also for a variety of technological applications in photonics and micro-engineering.…

Soft Condensed Matter · Physics 2019-08-27 Pietro Tierno

Additive manufacturing at the micro- and nanoscale has seen a recent upsurge to suit the increasing demand for more elaborate structures. However, the integration and precise placement of multiple distinct materials at small scales remain a…

Soft Condensed Matter · Physics 2022-08-05 Steven van Kesteren , Xueting Shen , Michele Aldeghi , Lucio Isa

Colloidal particles at complex fluid interfaces and within films assemble to form ordered structures with high degrees of symmetry via interactions that include capillarity, elasticity, and other fields like electrostatic charge. Here we…

We consider a lattice model for amphiphiles in a solvent with molecules chemically similar to one part of the amphiphilic molecule. The dependence of the interaction potential on orientation of the amphiphilic molecules is taken into…

Soft Condensed Matter · Physics 2014-11-14 Jakub Pękalski , Paweł Rogowski , Alina Ciach

The fabrication of novel soft materials is an important scientific and technological challenge. We investigate the response of magnetic ellipsoidal particles adsorbed at fluid-fluid interfaces to external magnetic fields. By exploiting…

Soft Condensed Matter · Physics 2014-10-29 Gary B. Davies , Timm Krueger , Peter V. Coveney , Jens Harting , Fernando Bresme

We study the self-assembly of colloidal microgel particles at a quasi-two-dimensional air-water interface of a drying droplet. Using bright-field microscopy, we demonstrate that increasing particle elasticity drives interfacial organization…

Soft Condensed Matter · Physics 2026-03-10 Vaibhav Raj Singh Parmar , Sayantan Chanda , Rituparno Mandal , Ranjini Bandyopadhyay

We perform numerical simulations to study self-assembly of nanoparticles mediated by an elastic planar surface. We show how the nontrivial elastic response to deformations of these surfaces leads to anisotropic interactions between the…

Soft Condensed Matter · Physics 2012-01-04 Andela Šarić , Angelo Cacciuto

Thin elastic films can spontaneously attach to liquid interfaces, offering a platform for tailoring their physical, chemical, and optical properties. Current understanding of the elastocapillarity of thin films is based primarily on studies…

Although common in nature, the self-assembly of small molecules at sold-liquid interfaces is difficult to control in artificial systems. The high mobility of dissolved small molecules limits their residence at the interface, typically…

This paper presents an overview and discussion of magnetocapillary self-assemblies. New results are presented, in particular concerning the possible development of future applications. These self-organizing structures possess the notable…

Fluid Dynamics · Physics 2017-07-21 Galien Grosjean , Maxime Hubert , Nicolas Vandewalle

Self-assembled monolayers of microparticles encoding Archimedean and non-regular tessellations promise unprecedented structure-property relationships for a wide spectrum of applications in fields ranging from optoelectronics to surface…

Microgels are soft colloidal particles constituted by cross-linked polymer networks with a high potential for applications. In particular, after adsorption at a fluid interface, interfacial tension provides two-dimensional (2D) confinement…

Soft Condensed Matter · Physics 2021-09-03 Jacopo Vialetto , Natalie Nussbaum , Jotam Bergfreund , Peter Fischer , Lucio Isa

Monolayers of soft colloidal particles confined at fluid interfaces have been attracting increasing interest for fundamental studies and applications alike. However, establishing the relation between their internal architecture, which is…

Soft Condensed Matter · Physics 2021-03-30 Jacopo Vialetto , Fabrizio Camerin , Fabio Grillo , Lorenzo Rovigatti , Emanuela Zaccarelli , Lucio Isa

Soft colloids are increasingly used as model systems to address fundamental issues such as crystallisation and the glass and jamming transitions. Among the available classes of soft colloids, microgels are emerging as the gold standard.…

The assembly of colloidal particles at liquid/liquid or air/liquid interfaces is a versatile procedure to create microstructured monolayers and study their behavior under compression. When combined with soft and deformable particles such as…

Colloidal assembly at fluid interfaces has a great potential for the bottom-up fabrication of novel structured materials. However, challenges remain in realizing controllable and tunable assembly of particles into diverse structures.…

Soft Condensed Matter · Physics 2020-12-29 Qingguang Xie , Jens Harting

Self-assembly of nanoparticles at fluid-fluid interfaces is a promising route to fabricate functional materials from the bottom-up. However, directing and controlling particles into highly tunable and predictable structures -- while…

Soft Condensed Matter · Physics 2019-09-25 Qingguang Xie , Gary B. Davies , Jens Harting

Self-assembly of colloidal particles is poised to become a powerful composite material fabrication technique, but remains challenged by a limited control over the ensuing structures. We develop a new breed of nematic colloids that are…

Soft Condensed Matter · Physics 2017-02-01 Sungoh Park , Qingkun Liu , Ivan I. Smalyukh

Colloidal particles or nanoparticles, with equal affinity for two fluids, are known to adsorb irreversibly to the fluid-fluid interface. We present large-scale computer simulations of the demixing of a binary solvent containing such…

Soft Condensed Matter · Physics 2007-05-23 K. Stratford , R. Adhikari , I. Pagonabarraga , J. -C. Desplat , M. E. Cates
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