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The electronic and nuclear dynamics in methanol, following 156~nm photoexcitation, are investigated by combining a detailed analysis of time-resolved photoelectron spectroscopy experiments with electronic structure calculations. The…

We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

We determine and analyze the quantum phases and time delays in photoionization and photorecombination of valence 3p and 3s electrons of argon using the Kohn-Sham local density functional approach. The time-dependent local density…

Electron scattering and dielectronic recombination with an ion in the presence of a neighboring atom is studied. The incident electron is assumed to be captured by the ion, leading to resonant excitation of the atom which afterwards may…

Atomic Physics · Physics 2018-08-01 A. Eckey , A. Jacob , A. B. Voitkiv , C. Müller

Consensus has been reached that recollision, as the most important post-tunneling process, is responsible for nonsequential double ionization process in intense infrared laser field, however, its effect has been restricted to interaction…

Atomic Physics · Physics 2021-06-14 Xiaolei Hao , Yuxing Bai , Chan Li , Jingyu Zhang , Weidong Li , Weifeng Yang , MingQing Liu , Jing Chen

The ability to modulate free electrons with light has emerged as a powerful tool to produce attosecond electron wavepackets. However, research has so far aimed at the manipulation of the longitudinal wave function component, while the…

Optics · Physics 2023-06-14 F. Javier García de Abajo , Claus Ropers

The exact delay-zero calibration in an attosecond pump-probe experiment is important for the correct interpretation of experimental data. In attosecond transient absorption spectroscopy the determination of the delay-zero exclusively from…

We studied the recollision dynamics between the electrons and D$_2^+$ ions following the tunneling ionization of D$_2$ molecules in an intense short pulse laser field. The returning electron collisionally excites the D$_2^+$ ion to excited…

Atomic Physics · Physics 2009-11-10 X. M. Tong , Z. X. Zhao , C. D. Lin

Photoionization from energetically distinct electronic states may have a relative time delay of tens of attoseconds. Here we demonstrate that pulses of optical vortices allow measuring such attoseconds delays from magnetic sublevels, even…

Atomic Physics · Physics 2016-10-03 Jonas Wätzel , Jamal Berakdar

Coherent, broadband pulses of extreme ultraviolet (XUV) light provide a new and exciting tool for exploring attosecond electron dynamics. Using photoelectron streaking, interferometric spectrograms can be generated that contain a wealth of…

Atomic Physics · Physics 2020-08-26 Luca Pedrelli , Phillip D. Keathley , Laura Cattaneo , Franz X. Kärtner , Ursula Keller

The full three-dimensional photoelectron momentum distributions of argon are measured in intense near-circularly polarized laser fields. We observed that the transverse momentum distribution of ejected electrons by 410-nm near-circularly…

Atomic Physics · Physics 2020-02-19 Xiang Huang , Qingbin Zhang , Shengliang Xu , Xianglong Fu , Xu Han , Wei Cao , Peixiang Lu

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

Ultrashort electron pulses with a high average current provide a powerful means of enhancing time-resolved imaging and photon generation. In this study, we report the attosecond shaping of sub-relativistic electron beams using membranes in…

The collective response of matter is ubiquitous and widely exploited, e.g. in plasmonic, optical and electronic devices. Here we trace on an attosecond time scale the birth of collective excitations in a finite system and find distinct new…

Atomic and Molecular Clusters · Physics 2017-02-15 A. S. Moskalenko , Y. Pavlyukh , J. Berakdar

Strong field ionization provides a unique mean to address complex dynamics of an electron in competing Coulomb and laser fields. Recent streak camera experiment (K\"ubel, et al., Phys. Rev. Lett. 119, 183201) analyzed asymmetries in the…

For two-electron diatomic molecules, we investigate magnetic field effects in non-sequential double ionization where recollisions prevail. We do so by formulating a three-dimensional semi-classical model that fully accounts for the Coulomb…

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

We analyze the effects of electron-electron and electron-phonon interactions in the dynamics of a system of two or three electrons that can be trapped to a localized state and detrapped to ab extended band states of a quantum dot using a…

Mesoscale and Nanoscale Physics · Physics 2025-12-11 R. Carmina Monreal

Soft recollisions are laser-driven distant collisions of an electron with its parent ion. Such collisions may cause an energy bunching, since electrons with different initial drift momenta can acquire impacts, which exactly counterbalance…

Atomic Physics · Physics 2012-04-25 Alexander Kästner , Ulf Saalmann , Jan M. Rost

Determining the pulse duration of femtosecond electron bunches is challenging and often experimentally invasive. An effective method for measuring the duration based on the time-dependent variations in electron beam divergence induced by a…

Accelerator Physics · Physics 2025-07-01 Andreas Seidel , Carola Zepter , Alexander Sävert , Stephan Kuschel , Matt Zepf