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Light-induced molecular dynamics often involve the excitation of several electronic, vibrational, and rotational states. Since the ensuing electronic and nuclear motion determines the pathways and outcomes of photoinduced reactions, our…

A novel technique was demonstrated that overcome important drawbacks to crosslink cells by irradiation with ultrashort UV laser pulses (L-crosslinking). To use this technique coupled to Chromatin ImmunoPrecipitation (ChIP) in a high…

We provide an analytical description of the dynamics of an atom in an optical lattice using the method of perturbative adiabatic expansion. A precise understanding of the lattice-atom interaction is essential to taking full advantage of the…

Atomic Physics · Physics 2015-05-14 Tim Kovachy , Jason M. Hogan , David M. S. Johnson , Mark A. Kasevich

Light, weakly coupled bosonic particles such as axions can mediate long range monopole-dipole interactions between matter and spins. We propose a new experimental method using atom interferometry to detect such a force on a freely falling…

High Energy Physics - Phenomenology · Physics 2024-09-24 Mahiro Abe , Jason M. Hogan , David E. Kaplan , Chris Overstreet , Surjeet Rajendran

The motion of chemical bonds within molecules can be observed in real time, in the form of vibrational wavepackets prepared and interrogated through ultrafast nonlinear spectroscopy. Such nonlinear optical measurements are commonly…

We propose a two-dimensional interferometry based on electron wave packet interference with a cycle-shaped orthogonally polarized two-color laser field. With such method, sub-cycle and inter-cycle interferences can be disentangled into…

Atomic Physics · Physics 2015-06-04 Xinhua Xie

While the emerging field of vibrational polariton chemistry has the potential to overcome traditional limitations of synthetic chemistry, the underlying mechanism is not yet well understood. Here, we explore how the dynamics of unimolecular…

Chemical Physics · Physics 2021-11-16 Derek S Wang , Tomáš Neuman , Susanne F Yelin , Johannes Flick

Light-pulse atom interferometers rely on the wave nature of matter and its manipulation with coherent laser pulses. They are used for precise gravimetry and inertial sensing as well as for accurate measurements of fundamental constants.…

Quantum Physics · Physics 2015-12-02 Stephan Kleinert , Endre Kajari , Albert Roura , Wolfgang P. Schleich

How atoms and electrons in a molecule move during a chemical reaction and how rapidly energy is transferred to or from the surroundings can be studied with flashes of laser light. However, despite prolonged efforts to develop various…

Chemical Physics · Physics 2022-01-05 JunWoo Kim , Jonggu Jeon , Tai Hyun Yoon , Minhaeng Cho

Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene, 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and…

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost

We show that if the laser is intense enough, it may always ionize an atom or induce transitions between discrete energy levels of the atom, no matter what is its frequency. It means in the quantum transition of an atom interacting with an…

Quantum Physics · Physics 2007-05-23 Qi-Ren Zhang

Molecular matter-wave interferometry enables novel strategies for manipulating the internal mechanical motion of complex molecules. Here, we show how chiral molecules can be prepared in a quantum superposition of two enantiomers by…

Quantum Physics · Physics 2021-09-22 Benjamin A. Stickler , Mira Diekmann , Robert Berger , Daqing Wang

Vibrational dynamics in conventional molecules usually takes place on a timescale of picoseconds or shorter. A striking exception are ultralong-range Rydberg molecules, for which dynamics is dramatically slowed down as a consequence of the…

Molecular vibrations and their dynamics are of outstanding importance for electronic and thermal transport in nanoscale devices as well as for molecular catalysis. The vibrational dynamics of <100 molecules are studied through three-colour…

Exploration of a new ultrafast-ultrasmall frontier in atomic and molecular physics has begun. Not only is is possible to control outer-shell electron dynamics with intense ultrafast optical lasers, but now control of inner-shell processes…

We outline new laser interferometer measurements to search for variation of the electromagnetic fine-structure constant $\alpha$ and particle masses (including a non-zero photon mass). We propose a strontium optical lattice clock -- silicon…

Atomic Physics · Physics 2016-06-29 Y. V. Stadnik , V. V. Flambaum

We show that combining vibrational spectroscopy with signal processing can result in a scheme for ultrasensitive detection of molecules. We consider the vibrational spectrum as a signal on the energy axis and apply a matched filter on that…

Computational Physics · Physics 2018-12-10 Tay Yong Boon , Ian Tay Rongde , Loy Liang Yi , Aw Ke Fun , Ong Zhi Li , Sergei Manzhos

Biologically inspired photonic structures are the key for technological advances and for miniaturized lasers. Here random lasers in dye-doped titania with the disordered structure of paper are proposed. Sharp electromagnetic resonances with…

Recently it has been recognized that electronic conical intersections in molecular systems can be induced by laser light even in diatomics. As is known a direct consequence of these accidental degeneracies is the appearence of nonadiabatic…

Atomic and Molecular Clusters · Physics 2013-10-30 Gábor J. Halász , Ágnes Vibók , Nimrod Moiseyev , Lorenz S. Cederbaum