Related papers: Coupling electrons and vibrations in molecular qua…
For ultrashort VUV pulses with a pulse length comparable to the orbital time of the bound electrons they couple to we propose a simplified envelope Hamiltonian. It is based on the Kramers-Henneberger representation in connection with a…
We introduce a hybrid classical-quantum algorithm to compute dynamical correlation functions and excitation spectra in many-body quantum systems, with a focus on molecular systems. The method combines classical preparation of a perturbed…
The expectation value of the Hamiltonian using a model wave function is widely used to estimate the eigenvalues of electronic Hamiltonians. We explore here a modified formula for models based on long-range interaction. It scales differently…
Since quantum feedback is based on classically accessible measurement results, it can provide fundamental insights into the dynamics of quantum systems by making available classical information on the evolution of system properties and on…
We characterize excited state quantum phase transitions in the two dimensional limit of the vibron model with the quantum fidelity susceptibility, comparing the obtained results with the information provided by the participation ratio. As…
Exactly solvable models of topologically ordered phases with non-abelian anyons typically require complicated many-body interactions which do not naturally appear in nature. This motivates the "inverse problem" of quantum many-body physics:…
We present a model of electron transport through a random distribution of interacting quantum dots embedded in a dielectric matrix to simulate realistic devices. The method underlying the model depends only on fundamental parameters of the…
We introduce a framework for the calculation of ground and excited state energies of bosonic systems suitable for near-term quantum devices and apply it to molecular vibrational anharmonic Hamiltonians. Our method supports generic reference…
We present an approach for carrying out non-adiabatic molecular dynamics simulations of systems in which non-adiabatic transitions arise from the coupling between the classical atomic motions and a quasi-continuum of electronic quantum…
Classical simulation of quantum systems plays an important role in the study of many-body phenomena and in the benchmarking and verification of quantum technologies. Exact simulation is often limited to small systems because the dimension…
The triaxial quadrupole collective Hamiltonian, based on relativistic energy density functionals, is extended to include a pairing collective coordinate. In addition to triaxial shape vibrations and rotations, the model describes pairing…
We construct a classical action for a system of $N$ point-like sources which carry SU(2) non-Abelian charges coupled to non-Abelian Chern-Simons gauge fields, and develop a quantum mechanics for them. Adopting the coherent state…
An approximate relativistic two-component Hamiltonian for use in molecular electronic structure calculations is derived in the form of a sum of fixed atom-centered kinetic and spin-orbit operators added to the non-relativistic Hamiltonian.…
We derive an explicit Hamiltonian for copying the basis up and down states of a quantum two-state system - a qubit - onto n "copy" qubits initially all prepared in the down state. In terms of spin components, for spin-1/2 particle spin…
This paper derives master equations for an atomic two-level system for a large set of unitarily equivalent Hamiltonians without employing the rotating wave and certain Markovian approximations. Each Hamiltonian refers to physically…
In this work we show how to engineer bilinear and quadratic Hamiltonians in cavity quantum electrodynamics (QED) through the interaction of a single driven two-level atom with cavity modes. The validity of the engineered Hamiltonians is…
The static and dynamical properties of a one-dimensional quantum system described by a non-Hermitian Hamiltonian of the so-called Hatano-Nelson type; a tight-binding model with asymmetric (or non-reciprocal) hopping, are studied. The static…
In this work we set up a model Hamiltonian to study the excited state quantum dynamics of 1,1-difluoroethylene, a molecule that has equivalent atoms exchanged by a torsional symmetry operation leading to equivalent minima on the potential…
A framework for statistical-mechanical analysis of quantum Hamiltonians is introduced. The approach is based upon a gradient flow equation in the space of Hamiltonians such that the eigenvectors of the initial Hamiltonian evolve toward…
We establish a connection between ground states of local quantum Hamiltonians and thermal states of classical spin systems. For any discrete classical statistical mechanical model in any spatial dimension, we find an associated quantum…