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Experiments show that light-matter strong coupling affects chemical properties, though the underlying mechanism remains unclear. We present an ab initio quantum electrodynamics coupled cluster method for the collective strong coupling…

Chemical Physics · Physics 2024-11-18 Matteo Castagnola , Marcus T. Lexander , Henrik Koch

The interaction between an atomic ensemble and a light mode in a high-finesse optical cavity can easily reach the strong-coupling regime, where quantum effects dominate. In this regime, the interaction can be used to generate both…

In an optical cavity, strong light--matter coupling between excitons and photons has been widely reported as a way to enhance energy delocalization through spatially extended polaritonic states. In contrast, leveraging cavity-mediated…

Quantum Physics · Physics 2026-04-08 Vincent Pouthier , Saad Yalouz

An important goal of modern condensed matter physics involves the search for states of matter with new emergent properties and desirable functionalities. Although the tools for material design remain relatively limited, notable advances…

Strongly Correlated Electrons · Physics 2023-06-21 Jacqueline Bloch , Andrea Cavalleri , Victor Galitski , Mohammad Hafezi , Angel Rubio

Since its inception, research of cavity quantum electrodynamics (CQED) has extended our understanding of light-matter interactions and our ability to utilize them. Thus far, all the work in this field has been focused on light interacting…

Strong coupling of quantum emitters with confined electromagnetic modes of nanophotonic structures may be used to change optical, chemical and transport properties of materials, with significant theoretical effort invested towards a better…

Quantum Physics · Physics 2020-01-22 M. Sánchez-Barquilla , R. E. F. Silva , J. Feist

We provide a general quantum theory to describe the coupling of light with the motion of a dielectric object inside a high finesse optical cavity. In particular, we derive the total Hamiltonian of the system as well as a master equation…

The availability of efficient photon sources with specific properties is important for quantum-technological applications. However, the realization of such photon sources is often challenging and hence alternative perspectives that suggest…

Experiments at the interface of quantum-optics and chemistry have revealed that strong coupling between light and matter can substantially modify chemical and physical properties of molecules and solids. While the theoretical description of…

Quantum Physics · Physics 2020-02-06 Christian Schäfer , Michael Ruggenthaler , Vasil Rokaj , Angel Rubio

The idea of making photons effectively interact has attracted a lot of interest in recent years, for several reasons. Firstly, since photons do not naturally interact with each other, it is of fundamental physical interest to see what kind…

Quantum Physics · Physics 2023-11-08 Simon Panyella Pedersen

Cavity photon resonators with ultrastrong light-matter interactions are attracting interest both in semiconductor and superconducting systems displaying the capability to manipulate the cavity quantum electrodynamic ground state with…

We investigate structural resonances in multi-element optical resonators and provide a roadmap for the description of the interaction of single extended cavity modes with quantum emitters or mechanical resonators. Using a first principle…

Quantum Physics · Physics 2017-05-01 Claudiu Genes , Aurélien Dantan

The hybridization between light and matter is fundamental for achieving cavity-induced control over quantum materials, necessitating accurate ab initio methods for their analysis. Among these, the quantum electrodynamics Hartree-Fock…

Quantum Physics · Physics 2024-11-25 Ilia Mazin , Yu Zhang

Strong light-matter coupling gives rise to polaritons - hybrid excitations whose mixed photonic and matter character enables control over optical, electronic and chemical properties. This Feature Article surveys the main architectures…

I introduce and analyse chiral light--matter interaction in the ultrastrong coupling limit where the rotating-wave approximation cannot be made. Within this limit, a two-level system (TLS) with a circularly polarized transition dipole…

Quantum Physics · Physics 2019-10-02 Sahand Mahmoodian

We perform extensive simulations of the two-dimensional cavity-coupled electron gas in a modulating potential as a minimal model for cavity quantum materials. These simulations are enabled by a newly developed quantum-electrodynamical (QED)…

Strongly Correlated Electrons · Physics 2025-10-08 Lukas Weber , Miguel A. Morales , Johannes Flick , Shiwei Zhang , Angel Rubio

Despite the potential paradigm breaking capability of microcavities to control chemical processes, the extent to which photonic devices change properties of molecular materials is still unclear, in part due to challenges in modeling hybrid…

Chemical Physics · Physics 2021-12-30 Raphael F. Ribeiro

Cavity and circuit QED study light-matter interaction at its most fundamental level. Yet, this interaction is most often neglected when considering the coupling of this system with an environment. In this paper, we show how this…

Quantum Physics · Physics 2011-10-24 Félix Beaudoin , J. M. Gambetta , A. Blais

Engineering the interaction between light and matter is an important goal in the emerging field of quantum opto-electronics. Thanks to the use of cavity quantum electrodynamics architectures, one can envision a fully hybrid multiplexing of…

Mesoscale and Nanoscale Physics · Physics 2013-03-12 M. R. Delbecq , L. E. Bruhat , J. J. Viennot , S. Datta , A. Cottet , T. Kontos

This work sets a road-map towards an experimental realization of strong coupling between free-electrons and photons, and analytically explores entanglement phenomena that emerge in this regime. The proposed model unifies the strong-coupling…

Quantum Physics · Physics 2019-09-11 Ofer Kfir