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The development of multifunctional solid-state materials is key to advancing lithium-ion batteries with enhanced safety and simplified architectures. Here, we report a scalable, highly efficient (near $100\%$), solvent-free mechanochemical…

${\beta}$- Eucryptite (LiAlSiO4) is a potential electrolyte for Li- ion battery due to its high Li- ion conductivity and very small volume thermal expansion coefficient. We have performed ab-initio molecular dynamics simulations of $\beta$-…

Materials Science · Physics 2018-03-26 Baltej Singh , Mayanak K. Gupta , Ranjan Mittal , Samrath L. Chaplot

We develop a continuum phase-field model for the simulation of diffusion limited solid-solid phase transformations during lithium insertion in LiFePO4-nano-particles. The solid-solid phase boundary between the LiFePO4 (LFP)-phase and the…

Materials Science · Physics 2018-07-20 Michael Fleck , Holger Federmann , Evgeny Pogorelov

We investigate the structure and magnetic properties of thin films of the LaCoO$_{3}$ compound. Thin films are deposited by pulsed laser deposition on various substrates in order to tune the strain from compressive to tensile. Single-phase…

Strongly Correlated Electrons · Physics 2015-05-18 A. D. Rata , A. Herklotz , L. Schultz , K. Doerr

Alternating layers of granular Iron (Fe) and Titanium dioxide (TiO$_{2-\delta}$) were deposited on (100) Lanthanum aluminate (LaAlO$_3$) substrates in low oxygen chamber pressure using a controlled pulsed laser ablation deposition…

Materials Science · Physics 2007-05-23 Soack Dae Yoon , Carmine Vittoria , Vincent G. Harris , Allan Widom

We fabricated NiFe2O thin films on MgAl2O4 (001) substrates by reactive dc magnetron co-sputtering in a pure oxygen atmosphere at different substrate temperatures. The film properties were investigated by various techniques with a focus on…

In this study, we address the challenge of electrolyte degradation in all-solid-state humidified Li-$O_2$ batteries, which offer high theoretical energy density and potential cost advantages over conventional lithium-ion batteries.…

All-solid-state batteries are currently developed at high pace and show a strong potential for market introduction within the next years. Though their performance has improved considerably over the last years, investigation of their…

In this article, an overview of the fabrication and properties of high quality La0.67Sr0.33MnO3 (LSMO) thin films is given. A high quality LSMO film combines a smooth surface morphology with a large magnetization and a small residual…

The superconducting nominal "non-doped" $La_{1.85}Y_{0.15}CuO_4$ (LYCO) thin films are successfully prepared by dc magnetron-sputtering and in situ post-annealing in vacuum. The best $T_{C0}$ more than 13K is achieved in the optimal LYCO…

Superconductivity · Physics 2015-06-25 L. Zhao , G. Wu , R. H. Liu , X. H. Chen

We introduce an adhesion parameter that enables rapid screening for materials interfaces with high adhesion. This parameter is obtained by density functional theory calculations of individual single-material slabs rather than slabs…

This work reports a pulsed laser-assisted synthesis, detailed structural characterization, and study of plasmonic properties of three sets of TiN/TiNO thin films with high electron density. The first two sets of TiN films were grown at 600C…

We investigate the structure and magneto-transport properties of thin films of the Co_2Cr_xFe_(1-x)Al full-Heusler compound, which is predicted to be a half-metal by first-principles theoretical calculations. Thin films are deposited by…

Materials Science · Physics 2009-11-11 A. D. Rata , H. Braak , D. E. Buergler , S. Cramm , C. M. Schneider

SrVO3 thin films with a high figure of merit for applications as transparent conductors were crystallized from amorphous layers using solid phase epitaxy (SPE). Epitaxial SrVO3 films crystallized on SrTiO3 using SPE exhibit a room…

We compile data and machine learned models of solid Li-ion electrolyte performance to assess the state of materials discovery efforts and build new insights for future efforts. Candidate electrolyte materials must satisfy several…

Materials Science · Physics 2019-04-22 Austin D. Sendek , Gowoon Cheon , Mauro Pasta , Evan J. Reed

La-doped SrSnO3 (LSSO) is known as one of deep-ultraviolet (DUV)-transparent conducting oxides with an energy bandgap of ~4.6 eV. Since LSSO can be grown heteroepitaxially on more wide bandgap substrates such as MgO (Eg ~7.8 eV), LSSO is…

Materials Science · Physics 2020-01-29 Mian Wei , Anup V. Sanchela , Bin Feng , Yuichi Ikuhara , Hai Jun Cho , Hiromichi Ohta

Al-doped ZnO thin films were deposited using reactive high power impulse magnetron sputtering at substrate temperatures between room temperature and 600 $\bullet$ C. Two sample series with different oxygen partial pressures were studied.…

Materials Science · Physics 2025-03-03 Martin Mickan , Ulf Helmersson , David Horwat

Solid-ion conductors (SICs) comprising non-ionic plastic crystals and lithium salts often require compositing with polymers to render them processable for use in solid-state lithium-metal batteries. Here, we show that polymer-doped plastic…

Boron-doped polycrystalline silicon-germanium (SiGe) thin films are grown by low-pressure chemical vapor deposition (LPCVD) and their thermoelectric properties are characterized from 120 K to 300 K for the potential applications in…

Materials Science · Physics 2015-06-23 Jianbiao Lu , Ruiqiang Guo , Weijing Dai , Baoling Huang

Optical reflectivity measurements were performed on a single crystal of the d-electron heavy-fermion (HF) metal LiV2O4. The results evidence the highly incoherent character of the charge dynamics for all temperatures above T^* \approx 20 K.…

Strongly Correlated Electrons · Physics 2007-10-24 P. E. Jönsson , K. Takenaka , S. Niitaka , T. Sasagawa , S. Sugai , H. Takagi