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Tip-enhanced Raman spectroscopy (TERS) combines inelastic light scattering well below the diffraction limit down to the nanometer range and scanning probe microscopy and, possibly, spectroscopy. In this way, topographic and spectroscopic as…

Superconductivity · Physics 2023-06-06 Leander Peis , Ge He , Daniel Jost , Gabriele Rager , Rudi Hackl

We examine anharmonic contributions to the optical phonon modes in bulk $T_d$-MoTe$_2$ through temperature-dependent Raman spectroscopy. At temperatures ranging from 100 K to 200 K, we find that all modes redshift linearly with temperature…

Materials Science · Physics 2016-07-20 Jaydeep Joshi , Iris Stone , Ryan Beams , Sergiy Krylyuk , Irina Kalish , Albert Davydov , Patrick Vora

One of the most widely used chiroptical spectroscopic methods for studying chiral molecules is Raman optical activity; however, the chiral Raman optical activity signal is extremely weak. Here, we theoretically examine enhanced chiral…

Quantum Physics · Physics 2019-05-03 Tuguldur Kh. Begzjav , Zhedong Zhang , Marlan O. Scully , Girish S. Agarwal

We extend the analysis of photon coincidence spectroscopy beyond bichromatic excitation and two-photon coincidence detection to include multichromatic excitation and multiphoton coincidence detection. Trichromatic excitation and…

Quantum Physics · Physics 2009-09-25 L. Horvath , B. C. Sanders , B. F. Wielinga

In this letter, we highlight the enhanced functionalization of the electronic and optical properties in the hybrid heterojunction of 1D Tellurene with 2D monolayer of Graphene and MoS2 in both lateral and vertical geometries, having…

Materials Science · Physics 2022-04-01 Tuhin Kumar Maji , Kumar Vaibhav , Anna Delin , Olle Eriksson , Debjani Karmakar

Surface plasmons or phonons propagating on a two-dimensional (2D) material can exhibit coupling with resonant excitations in its substrate, and the resulting coupled modes were extensively studied. Similar coupling of edge modes propagating…

Optics · Physics 2025-07-23 Azat F. Aminov , Alexey A. Sokolik

Raman scattering excitation (RSE) is an experimental technique in which the spectrum is made up by sweeping the excitation energy when the detection energy is fixed. We study the low-temperature ($T$=5~K) RSE spectra measured on four high…

We identify carrier scattering at densities below which it has previously been observed in semiconductor quantum wells. These effects are evident in the peakshapes of 2D double-quantum spectra, which change as a function of excitation…

Optics · Physics 2016-05-25 Jonathan O. Tollerud , Jeffrey A. Davis

Highly nonlinear optical phenomena can provide access to properties of electronic systems which are otherwise difficult to access through conventional linear optical spectroscopies. In particular, high harmonic generation (HHG) in…

Optics · Physics 2021-04-28 K. Uchida , V. Pareek , K. Nagai , K. M. Dani , K. Tanaka

We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage…

The asymmetric peak at 212 - 218 cm-1 occurring in InAs micro-nano wires is investigated using spatially resolved Raman spectroscopy (SRRS) of uniform, bent and long tapered MNWs grown on a Si (001) substrate. It is attributed to…

Materials Science · Physics 2016-05-25 Vandna Kumari Gupta , Alka A. Ingale , Suparna Pal , R. Aggarwal , V. Sathe

We present a microfluidic method leading to accurate measurements of the mutual diffusion coefficient of a liquid binary mixture over the whole solute concentration range in a single experiment. This method fully exploits solvent…

Soft Condensed Matter · Physics 2017-09-21 Anne Bouchaudy , Charles Loussert , Jean-Baptiste Salmon

We present a new method for high precision measurements of polarization rotation in the frequency range from 0.2 to 2.2 THz using a fiber coupled time-domain THz spectrometer. A free standing wire-grid polarizer splits THz light into…

Optics · Physics 2023-12-21 Zhenisbek Tagay , Ralph Romero , N. P. Armitage

We report a comprehensive micro-Raman scattering study of electrochemically-gated graphene field-effect transistors. The geometrical capacitance of the electrochemical top-gates is accurately determined from dual-gated Raman measurements,…

Mesoscale and Nanoscale Physics · Physics 2016-08-08 Guillaume Froehlicher , Stéphane Berciaud

Through comprehensive data analysis, we demonstrate that a ${\chi}^{(2)}$-induced artifact, arising from imperfect balancing in the conventional electro-optic sampling (EOS) detection scheme, contributes significantly to the measured signal…

Plasmon-enhanced chemical transformations at the solid-liquid interface can be imaged with high sensitivity, chemical selectivity, and nanoscale precision through tip-enhanced Raman scattering (TERS). We demonstrate the latter for the first…

Chemical Physics · Physics 2019-03-29 Ashish Bhattarai , Patrick Z. El-Khoury

One of the main goals for hadron colliders is the study of the properties of the third generation quarks. We study the signatures for new TeV resonances that couple to top or bottom quarks both at the Tevatron Run II and at the LHC. We find…

High Energy Physics - Phenomenology · Physics 2009-11-10 T. Han , G. Valencia , Yili Wang

The marriage between a two-dimensional layered material (2DLM) and a complex transition metal oxide (TMO) results in a variety of physical and chemical phenomena that would not have been achieved in either material alone. Interesting recent…

Materials Science · Physics 2019-05-09 Kyeong Tae Kang , Jeongmin Park , Dongseok Suh , Woo Seok Choi

Coherent Raman microscopy provide label-free imaging by interrogating the intrinsic vibration of biomolecules. Nevertheless, trade-off between high chemical-specificity and high imaging-speed currently exists in transition from spectroscopy…

Optics · Physics 2017-10-11 Kun Chen , Tao Wu , Tao Chen , Tian Zhou , Haoyun Wei , Yan Li

Raman spectroscopy is a powerful tool to detect, analyze and identify molecules. It has been a long-history pursuit to push the detection limit of Raman spectroscopy down to the fundamental single-molecule (SM) level. Due to the tiny cross…

Optics · Physics 2023-11-10 Haiyao Yang , Haoran Mo , Lihong Hong , Zhi-Yuan Li