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The striking anomalies in physical properties of supercooled water that were discovered in the 1960-70s, remain incompletely understood and so provide both a source of controversy amongst theoreticians, and a stimulus to experimentalists…

Chemical Physics · Physics 2016-05-31 Sander Woutersen , Michiel Hilbers , Zuofeng Zhao , C. Austen Angell

We have mapped the molecular-atomic transition in liquid hydrogen using first principles molecular dynamics. We predict that a molecular phase with short-range orientational order exists at pressures above 100 GPa. The presence of this…

Materials Science · Physics 2010-02-11 Isaac Tamblyn , Stanimir A. Bonev

Nucleation phenomena commonly observed in our every day life are of fundamental, technological and societal importance in many areas, but some of their most intimate mechanisms remain however to be unravelled. Crystal nucleation, the early…

Disordered Systems and Neural Networks · Physics 2021-09-17 Sébastien Becker , Emilie Devijver , Rémi Molinier , Noël Jakse

We propose experimentally feasible ways to probe universal features of absorbing phase transitions from two different approaches, both based on numerical validations. On one hand, we numerically study a probability distribution of…

Statistical Mechanics · Physics 2018-12-20 Keiichi Tamai , Masaki Sano

A canonical ensemble model is used to describe a caloric curve of nuclear liquid-gas phase transition. Allowing a discontinuity in the freeze out density from one spinodal density to another for a given initial temperature, the nuclear…

Nuclear Theory · Physics 2008-11-26 S. J. Lee , A. Z. Mekjian

The primary distinction between solid and liquid phases is mechanical rigidity, with liquids having a disordered atomic structure that allows flow. While melting is a common phase transition, its microscopic mechanisms still remain unclear.…

Clarifying the factors that control the contact angle of a liquid on a solid substrate is a long-standing scientific problem pertinent across physics, chemistry and materials science. Progress has been hampered by the lack of a…

Statistical Mechanics · Physics 2019-11-11 Robert Evans , Maria C. Stewart , Nigel B. Wilding

Friction is the basic, ubiquitous mechanical interaction between two surfaces that results in resistance to motion and energy dissipation. In spite of its technological and economic significance, our ability to control friction remains…

Atomic Physics · Physics 2018-08-10 Dorian Gangloff , Alexei Bylinskii , Ian Counts , Wonho Jhe , Vladan Vuletić

The properties of hydrogen at high pressure have wide implications in astrophysics and high-pressure physics. Its phase change in the liquid is variously described as a metallization, H2-dissociation, density discontinuity or plasma phase…

Materials Science · Physics 2020-03-17 Hua Y. Geng , Q. Wu , Miriam Marqués , Graeme J. Ackland

We perform molecular dynamics simulations driven by accurate Quantum Monte Carlo forces on dense liquid hydrogen. Recently it has been reported a complete atomization transition between a mixed-atomic liquid and a completely dissociated…

Strongly Correlated Electrons · Physics 2015-06-23 Guglielmo Mazzola , Sandro Sorella

A rigorous theory of liquid-crystal transitions is developed starting from the Liouville equation. The starting point is an all-atom description and a set of order parameter field variables that are shown to evolve slowly via Newton's…

Soft Condensed Matter · Physics 2010-01-05 Zeina Shreif , Stephen Pankavich , Peter Ortoleva

Temperature-driven polyamorphism has been reported in various supercooled liquids and glasses. The dynamical and structural routes followed by the system during such crossovers are however not universal and appear to be related to intrinsic…

Disordered Systems and Neural Networks · Physics 2018-08-29 S. Hechler , B. Ruta , M. Stolpe , E. Pineda , Z. Evenson , O. Gross , W. Hembree , A. Bernasconi , R. Busch , I. Gallino

The properties of the interface between solid and melt are key to solidification and melting, as the interfacial free energy introduces a kinetic barrier to phase transitions. This makes solidification happen below the melting temperature,…

Statistical Mechanics · Physics 2015-12-02 Bingqing Cheng , Gareth A. Tribello , Michele Ceriotti

V-T theory is constructed in the many-body Hamiltonian formulation, and differs at the foundation from current liquid dynamics theories. In V-T theory the liquid atomic motion consists of two contributions, normal mode vibrations in a…

Statistical Mechanics · Physics 2016-05-04 Duane C. Wallace , Giulia De Lorenzi-Venneri , Eric D. Chisolm

An equilibrated model glass-forming liquid is studied by mapping successive configurations produced by molecular dynamics simulation onto a time series of inherent structures (local minima in the potential energy). Using this ``inherent…

Soft Condensed Matter · Physics 2012-03-27 Thomas B. Schroeder , Srikanth Sastry , Jeppe C. Dyre , Sharon C. Glotzer

We study the liquid-solid transition in a collection of interacting particles moving through a dissipative medium under the action of a constant, spatially uniform external force, e.g. a charge-stabilized suspension in a fluidized bed or a…

Soft Condensed Matter · Physics 2007-05-23 Rangan Lahiri , Sriram Ramaswamy

The ordering transitions of a 2D lattice liquid characterized by a single favoured local structure (FLS) are studied using Monte Carlo simulations. All eight distinct geometries for the FLS are considered and we find a variety of ordering…

Statistical Mechanics · Physics 2015-06-12 Pierre Ronceray , Peter Harrowell

The melting point of a material constitutes a pivotal property with profound implications across various disciplines of science, engineering, and technology. Recent advancements in machine learning potentials have revolutionized the field,…

Materials Science · Physics 2024-09-02 Fu-Zhi Dai , Si-Hao Yuan , Yan-Bo Hao , Xin-Fu Gu , Shipeng Zhu , Jidong Hu , Yifen Xu

The physics of critical phenomena in a many-body system far from thermal equilibrium is an interesting and important issue to be addressed both experimentally and theoretically. The trapped cold atoms have been actively used as a clean and…

Atomic Physics · Physics 2017-09-13 Geol Moon , Myoung-Sun Heo , Yonghee Kim , Heung-Ryoul Noh , Wonho Jhe

It is well known that the similar universal behavior of infinite-size (bulk) systems of different nature requires the same basic conditions: space dimensionality; number components of order parameter; the type (short- or long-range) of the…