Related papers: Orientational quantum revivals induced by a single…
Significant molecular orientation can be achieved by time-symmetric single-cycle pulses of zero area, in the THz region. We show that in spite of the existence of a combined time-space symmetry operation, not only large peak instantaneous…
Intense single-cycle THz pulses resonantly interacting with molecular rotations are shown to induce significant field-free orientation under ambient conditions. We calculate and measure the angular distribution associated with THz-driven…
The numerical prediction, theoretical analysis, and experimental verification of the phenomenon of wave packet revivals in quantum systems has flourished over the last decade and a half. Quantum revivals are characterized by initially…
The ability of quantum walks to evolve in a superposition of distinct quantum states has been used as a resource in quantum communication protocols. Under certain settings, the $k$-cycle discrete-time quantum walks\,(DTQW) are known to…
Control of molecular rotations by laser fields is an active area of research focusing on the alignment/orientation of otherwise isotropic molecular samples. Oriented molecules are useful in many applications, such as molecular orbital…
We propose a novel scheme to generate single-cycle terahertz (THz) pulses via reflection of an optical femtosecond pulse train from a thin layer of nonlinear resonant medium. Our method is based on a coherent control of low-frequency…
The ability to manipulate the space-time structure of light waves diversifies light-matter interaction and light-driven applications. Conventionally, metasurfaces are employed to locally control the amplitude and phase of light fields by…
The Quantitative Rescattering Theory (QRS) for high-order harmonic generation (HHG) by intense laser pulses is presented. According to the QRS, HHG spectra can be expressed as a product of a returning electron wave packet and the…
We experimentally study the optical- and terahertz- induced rotational dynamics of asymmetric molecules in the gas phase. Terahertz and optical fields are identified as two distinct control handles over asymmetric molecules, as they couple…
The possibility to manipulate the wavepackets of single photons or biphotons has enriched quantum optics and quantum information science, with examples ranging from faithful quantum-state mapping and high-efficiency quantum memory to the…
We present a combined analytical and numerical investigation to show how an optimal control field can be designed to generate maximum field-free orientation of molecules for three populated rotational states. Based on a model involving pure…
We use an optical centrifuge to excite coherent rotational wave packets in N$_2$O, CS$_2$ and OCS molecules with rotational quantum numbers reaching up to J=465, 690 and 1186, respectively. Time-resolved rotational spectroscopy at such…
Polar molecules represent a promising platform for quantum simulation and computation protocols. Highly controllable arrays of optical tweezers are now accessible in experiments, allowing for unprecedented control of individual molecules.…
The at-will control of quantum states is a primary goal of quantum science and technology. The celebrated Hahn echo exemplifies such quantum-state control based on a time-reversal process in a few-level system. Here, we propose a different…
A molecule can be optically accelerated to rotate unidirectionally at a frequency of a few terahertzes which is many orders higher than the classical mechanical rotor. Such a photon-induced ultrafast molecular unidirectional rotation has…
A model for THz generation by optical rectification using tilted-pulse-fronts is developed. It simultaneously accounts for (i) the spatio-temporal distortions of the optical pump pulse, (ii) the nonlinear coupled interaction of THz and…
We explore the quantum dynamics of heteronuclear atomic collisions in waveguides and demonstrate the existence of a novel mechanism for the resonant formation of polar molecules. The molecular formation probabilities can be tuned by…
Quantum Cascade Lasers (QCL) constitute an intriguing opportunity for the production of on-chip optical Dissipative Kerr Solitons (DKS): self-organized optical waves which can travel while preserving their shape thanks to the interplay…
Control over the quantum states of individual molecules is crucial in the quest to harness their rich internal structure and dipolar interactions for applications in quantum science. In this paper, we develop a toolbox of techniques for the…
We present a combined analytical and numerical study for coherent terahertz control of a single molecular polariton, formed by strongly coupling two rotational states of a molecule with a single-mode cavity. Compared to the bare molecules…