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The antiferromagnetism in $\alpha$-Cu$_3$Mg(OH)$_6$Br$_2$ was studied by magnetic-susceptibility, specific-heat and neutron-diffraction measurements. The crystal structure consists of Cu$^{2+}$ kagome layers with Mg$^{2+}$ ions occupying…

Strongly Correlated Electrons · Physics 2019-10-23 Yuan Wei , Zili Feng , Clarina dela Cruz , Wei Yi , Zi Yang Meng , Jia-Wei Mei , Youguo Shi , Shiliang Li

We study the $S=1/2$ pyrochlore Heisenberg antiferromagnet in a magnetic field. Using large scale density-matrix renormalization group (DMRG) calculations for clusters up to $128$ spins, we find indications for a finite triplet gap, causing…

Strongly Correlated Electrons · Physics 2022-09-14 Imre Hagymási , Robin Schäfer , Roderich Moessner , David J. Luitz

We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices---barlowite Cu$_{4}$(OH)$_{6}$FBr. Magnetic susceptibility gives $\theta_{CW}$ = $-$136 K, while long-range order does not happen…

Strongly Correlated Electrons · Physics 2014-12-05 Tian-Heng Han , John Singleton , John A. Schlueter

The two-dimensional (2D) spin-1/2 kagome Heisenberg antiferromagnet is believed to host quantum spin liquid (QSL) states with no magnetic order, but its ground state remains largely elusive. An important outstanding question concerns the…

Strongly Correlated Electrons · Physics 2024-05-30 S. Suetsugu , T. Asaba , Y. Kasahara , Y. Kohsaka , K. Totsuka , B. Li , Y. Zhao , Y. Li , M. Tokunaga , Y. Matsuda

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Strongly Correlated Electrons · Physics 2021-06-15 H. Murayama , T. Tominaga , T. Asaba , A. de Oliveira Silva , Y. Sato , H. Suzuki , Y. Ukai , S. Suetsugu , Y. Kasahara , R. Okuma , I. Kimchi , Y. Matsuda

The spin-1/2 kagome lattice antiferromagnet herbertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, is a candidate material for a quantum spin liquid ground state. We show that the magnetic response of this material displays an unusual scaling…

Strongly Correlated Electrons · Physics 2010-04-07 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Qiu , D. G. Nocera , Y. S. Lee

Magnetism of Cu$_2$(OH)$_3$Br single crystals based on a triangular lattice is studied by means of magnetic susceptibility, pulsed-field magnetization, and specific heat measurements. There are two inequivalent Cu$^{2+}$ sites in an…

Strongly Correlated Electrons · Physics 2019-09-04 Z Y Zhao , H L Che , R Chen , J F Wang , X F Sun , Z Z He

Neutron spectroscopy and diffuse neutron scattering on herbertsmithite [ZnCu3 (OH)6Cl2], a near-ideal realisation of the s = 1/2 kagome antiferromagnet, reveal the hallmark property of a quantum spin liquid; instantaneous short-ranged…

Strongly Correlated Electrons · Physics 2009-12-21 M. A. de Vries , J. R. Stewart , P. P. Deen , J. O. Piatek , G. J. Nilsen , H. M. Ronnow , A. Harrison

Frustrated magnetism on the kagome lattice has been a fertile ground for rich and fascinating physics, ranging from experimental evidence of a spin liquid to theoretical predictions of exotic superconductivity. Among experimentally realized…

Strongly Correlated Electrons · Physics 2015-12-16 Yasir Iqbal , Harald O. Jeschke , Johannes Reuther , Roser Valentí , I. I. Mazin , Martin Greiter , Ronny Thomale

We performed high-precision magnetization measurements up to 120~T on three compositions of the newly discovered kagome antiferromagnet YCu$_3$(OD)$_{7-x}$Br$_{2+x}$ (YCOB), revealing a previously unobserved 5/9 fractional magnetization…

Fractional magnetisation plateaus, in which the magnetisation is pinned at a fraction of its saturated value within a range of external magnetic field, are spectacular macroscopic manifestations of the collective quantum behaviours. One…

The spin-1/2 antiferromagnetic Heisenberg model on a Kagome lattice is geometrically frustrated, which is expected to promote the formation of many-body quantum entangled states. The most sought-after among these is the quantum spin liquid…

We investigate the low temperature magnetic properties of a $S=\frac{5}{2}$ Heisenberg kagom\'e antiferromagnet, the layered monodiphosphate Li$_9$Fe$_3$(P$_2$O$_7$)$_3$(PO$_4$)$_2$, using magnetization measurements and $^{31}$P nuclear…

Strongly Correlated Electrons · Physics 2021-10-08 E. Kermarrec , R. Kumar , G. Bernard , R. Hénaff , P. Mendels , F. Bert , P. L. Paulose , B. K. Hazra , B. Koteswararao

We have synthesized high-quality single crystals of volborthite, a seemingly distorted kagome antiferromagnet, and carried out high-field magnetization measurements up to 74 T and 51V NMR measurements up to 30 T. An extremely wide 1/3…

Strongly Correlated Electrons · Physics 2015-06-03 H. Ishikawa , M. Yoshida , K. Nawa , M. Jeong , S. Krämer , M. Horvatić , C. Berthier , M. Takigawa , M. Akaki , A. Miyake , M. Tokunaga , K. Kindo , J. Yamaura , Y. Okamoto , Z. Hiroi

Strongly correlated Fermi systems are among the most intriguing and fundamental systems in physics, whose realization in some compounds is still to be discovered. We show that herbertsmithite ZnCu_3(OH)_6Cl_2 can be viewed as a strongly…

Strongly Correlated Electrons · Physics 2015-05-27 V. R. Shaginyan , A. Z. Msezane , K. G. Popov

We report results of 51V NMR experiments on a high-quality powder sample of volborthite Cu3V2O7(OH)2/2H2O, a spin-1/2 Heisenberg antiferromagnet on a distorted kagome lattice. Following the previous experiments in magnetic fields $B$ below…

We prepared a powder sample of edwardsite Cd2Cu3(SO4)2(OH)6 4H2O, which is a new candidate compound for the spin-1/2 kagome antiferromagnet, and studied its magnetic properties by magnetic susceptibility and heat capacity measurements.…

Materials Science · Physics 2015-06-15 Hajime Ishikawa , Yoshihiko Okamoto , Zenji Hiroi

We study an anisotropic Heisenberg antiferromagnet with ferromagnetic transverse spin exchange using exact quantum Monte Carlo methods. Such a model is relevant to a class of rare earth tetraboride materials that display a range of…

Strongly Correlated Electrons · Physics 2013-10-02 Keola Wierschem , Pinaki Sengupta

Herbertsmithite (ZnCu3(OH)6Cl2) is often discussed as the best realization of the highly frustrated antiferromagnetic kagome lattice known so far. We employ density functional theory calculations to determine eight exchange coupling…

Strongly Correlated Electrons · Physics 2014-01-31 Harald O. Jeschke , Francesc Salvat-Pujol , Roser Valenti

We investigate the properties in finite magnetic field of an extended anisotropic XXZ spin-1/2 model on the Kagome lattice, originally introduced by Balents, Fisher, and Girvin [Phys. Rev. B, 65, 224412 (2002)]. The magnetization curve…

Strongly Correlated Electrons · Physics 2015-11-10 X. Plat , F. Alet , S. Capponi , K. Totsuka