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Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

Quantum spectroscopy was performed using the frequency-entangled broadband photon pairs generated by spontaneous parametric down-conversion. An absorptive sample was placed in front of the idler photon detector, and the frequency of signal…

Quantum Physics · Physics 2009-11-10 Atsushi Yabushita , Takayoshi Kobayashi

The most important problem of spectroscopic chiral analysis is the inherently weak chiral signals are easily overwhelmed by the environment noises. Enormous efforts had been spent to overcome this problem by enhancing the symmetry break in…

Quantum Physics · Physics 2023-10-05 Chong Ye , Yifan Sun , Xiangdong Zhang

The final goal of quantum hypothesis testing is to achieve quantum advantage over all possible classical strategies. In the protocol of quantum reading this advantage is achieved for information retrieval from an optical memory, whose…

Quantum Physics · Physics 2021-01-22 Giuseppe Ortolano , Elena Losero , Ivano Ruo Berchera , Stefano Pirandola , Marco Genovese

We numerically analyze the use of intense entangled twin beams for ultra-sensitive spectroscopic measurements in chemical and biological systems. The examined scheme makes use of intense frequency-modulated (chirped) entangled beams to…

Quantum Physics · Physics 2018-05-16 Jiří Svozilík , Jan Peřina , Roberto de J. León-Montiel

Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that…

Quantum Physics · Physics 2021-08-25 Stefan Lerch , André Stefanov

Quantum entanglement is recognized as a fundamental resource in quantum information processing and is essential for understanding quantum many-body physics. However, experimentally detecting entanglement, particularly in many-particle…

Quantum Physics · Physics 2025-08-13 Hao-Yue Qi , Wei Zheng

It is controversial what is the true role of entanglement in two-photon virtual-state spectroscopy [Saleh et al, Phys. Rev. Lett. 80, 3483, 1998], a two-photon absorption spectroscopic technique that can retrieve information about the…

Quantum Physics · Physics 2015-06-11 R. de J. León-Montiel , J. Svozilík , L. J. Salazar-Serrano , J. P. Torres

Entangled photons have the remarkable ability to be more sensitive to signal and less sensitive to noise than classical light. Joint photons can sample an object collectively, resulting in faster phase accumulation and higher spatial…

Optics · Physics 2015-09-04 Chien-Hung Lu , Matthew Reichert , Xiaohang Sun , Jason W. Fleischer

The laws of quantum physics endow superior performance and security for information processing: quantum sensing harnesses nonclassical resources to enable measurement precision unmatched by classical sensing, whereas quantum cryptography…

Scattering in complex media scrambles light, thus obscuring images and limiting applications from astronomy to microscopy. Existing computational and wavefront-shaping methods treat scattering as a linear optical-wave inversion problem that…

Quantum Physics · Physics 2026-03-18 Chloé Vernière , Raphaël Guitter , Baptiste Courme , Hugo Defienne

We investigate how entanglement can enhance two-photon absorption in a three-level system. First, we employ the Schmidt decomposition to determine the entanglement properties of the optimal two-photon state to drive such a transition, and…

Quantum Physics · Physics 2021-10-29 Edoardo G Carnio , Andreas Buchleitner , Frank Schlawin

Nonlinear spectroscopy with quantum entangled photons is an emerging field of research that holds the promise to achieve a superior signal-to-noise ratio and effectively isolate many-body interactions. Photon sources used for this purpose…

Entangled photon pairs are predicted to linearize and increase the efficiency of two-photon absorption, allowing continuous wave laser diodes to drive ultrafast time-resolved spectroscopy and nonlinear processes. Despite a range of…

Quantum Physics · Physics 2022-05-31 Bryce P. Hickam , Manni He , Nathan Harper , Szilard Szoke , Scott Cushing

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

Quantum Physics · Physics 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

Absorption spectroscopy is a widely used technique that permits the detection and characterization of gas species at low concentrations. We propose a sensing strategy combining the advantages of frequency modulation spectroscopy with the…

Quantum Physics · Physics 2023-03-30 Alexandre Belsley

Nonclassical states are essential for optics-based quantum information processing, but their fragility limits their utility for practical scenarios in which loss and noise inevitably degrade, if not destroy, nonclassicality. Exploiting…

Quantum Physics · Physics 2015-03-25 Zheshen Zhang , Sara Mouradian , Franco N. C. Wong , Jeffrey H. Shapiro

Quantum-enhanced sensing promises to improve the performance of sensing tasks using non-classical probes and measurements that require far fewer scene-modulated photons than the best classical schemes, thereby granting…

Quantum Physics · Physics 2021-08-11 Michael R. Grace , Christos N. Gagatsos , Saikat Guha

Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the…

Quantum Physics · Physics 2023-09-20 Haowei Shi , Zaijun Chen , Scott E. Fraser , Mengjie Yu , Zheshen Zhang , Quntao Zhuang

Spectroscopy is an indispensable tool in understanding the structures and dynamics of molecular systems. However computational modelling of spectroscopy is challenging due to the exponential scaling of computational complexity with system…

Quantum Physics · Physics 2021-06-22 Chee-Kong Lee , Chang-Yu Hsieh , Shengyu Zhang , Liang Shi
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