Related papers: Probing light-driven quantum materials with ultraf…
Free electrons provide a powerful tool to probe material properties at atomic-scale spatial resolution. Recent advances in ultrafast electron microscopy enable the manipulation of free electron wavefunctions using laser pulses. It would be…
Resonant soft x-ray scattering (RSXS) is a leading probe of valence band order in materials best known for detecting charge density wave order in the copper-oxide superconductors. One of the biggest limitations on the RSXS technique is the…
We propose a novel way to image dynamical properties of nonstationary electron systems using ultrafast resonant x-ray scattering. Employing a rigorous theoretical analysis within the framework of quantum electrodynamics, we demonstrate that…
We develop a formalism to study the Resonant Inelastic X-ray Scattering (RIXS) response in metals based on the diagrammatic expansion for its cross section. The standard approach to the solution of the RIXS problem relies on two key…
The interaction of chirped femtosecond laser pulses with hybrid materials - materials comprised of plasmon sustaining structures and resonant molecules - is scrutinized using a self-consistent model of coupled Maxwell-Bloch equations. The…
Quantum computing exploits the quantum-mechanical nature of matter to exist in multiple possible states simultaneously. This new approach promises to revolutionize the present form of computing. As an approach to quantum computing, we…
We provide a perspective on the burgeoning field of controlling quantum materials at will and its potential for quantum simulations in and out equilibrium. After briefly outlining a selection of key recent advances in controlling materials…
Terahertz two-dimensional coherent spectroscopy (THz-2DCS) is transforming our ability to probe, visualize, and control quantum materials far from equilibrium. This emerging technique brings multi-dimensional resolution to the ultrafast…
Extending super-resolution imaging techniques to objects hidden in strongly scattering media potentially revolutionize the technical analysis for much broader categories of samples, such as biological tissues. The main challenge is the…
Entanglement and quantum correlations are central to the physics of quantum materials, yet they have remained notoriously difficult to probe experimentally. Probing these phenomena in solids requires quantum optical probes that operate at…
Light as a carrier of information and energy plays a fundamental role in both general relativity and quantum physics, linking these areas that are still not fully compliant with each other. Its quantum nature and spatio-temporal structure…
Qudits have proven to be a powerful resource for quantum information processing, offering enhanced channel capacities, improved robustness to noise, and highly efficient implementations of quantum algorithms. The encoding of photonic qudits…
I present a tractable theory for the Resonant Inelastic X-ray Scattering (RIXS) spectral function of magnons. The low-energy transition operator is written as a product of local spin operators times fundamental x-ray absorption spectra.…
We report a method to characterize the propagation of an ultrashort pulse of light through a multiple scattering medium by measuring its time-resolved transmission matrix. This method is based on the use of a spatial light modulator…
The consistent quantum theory of self-phase modulation (SPM) and cross-phase modulation (XPM) for ultrashort light pulses (USP) in medium with electronic Kerr-nonlinearity are developed. The approach makes use of momentum operator of…
The chaotic nature of x-ray free-electron-laser pulses is a major bottleneck that has limited the joint temporal and spectral resolution of spectroscopic measurements. We show how to use the stochastic x-ray field statistics to overcome…
We demonstrate a novel technique for producing high-order harmonics with designer spectral combs in the extreme ultraviolet-soft X-ray range for resonance applications using spectrally controlled visible lasers. Our approach enables…
Scattering-assisted synthesis of broadband optical pulses is recognized to have a cross-disciplinary funda-mental and application importance. Achieving full-waveform synthesis generally requires means for assessing the instantaneous…
Time-resolved x-ray diffraction (TR-XRD) and ultrafast electron diffraction (TR-UED) are emerging tools for probing ultrafast quantum dynamics. From a theoretical perspective, they are commonly described within different frameworks and…
Owing to their extremely narrow line-widths and exceptional coherence properties, M\"ossbauer nuclei form a promising platform for quantum optics, spectroscopy and dynamics at energies of hard x-rays. A key requirement for further progress…