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We present the One-orbital Ensemble Self-Consistent Field (OE-SCF) method, an {alternative} orbital-free DFT solver that extends the applicability of DFT to system sizes beyond the nanoscale while retaining the accuracy required to be…

Materials Science · Physics 2021-05-05 Xuecheng Shao , Wenhui Mi , Michele Pavanello

A new approach to solving the Time-Dependent Self-Consistent-Field equations is developed based on the double quotient formulation of Tsiper [J. Phys. B, 34 L401 (2001)]. Dual channel, quasi-independent non-linear optimization of these…

Quantum Physics · Physics 2010-01-19 Matt Challacombe

This paper considers estimation of sparse covariance matrices and establishes the optimal rate of convergence under a range of matrix operator norm and Bregman divergence losses. A major focus is on the derivation of a rate sharp minimax…

Statistics Theory · Mathematics 2013-02-14 T. Tony Cai , Harrison H. Zhou

The self-consistent field (SCF) generation of the three-dimensional (3D) electron density distribution ($\rho$) represents a fundamental aspect of density functional theory (DFT) and related first-principles calculations, and how one can…

Computational Physics · Physics 2024-11-19 Ryong-Gyu Lee , Yong-Hoon Kim

The convergence of stochastic interacting particle systems in the mean-field limit to solutions of conservative stochastic partial differential equations is established, with optimal rate of convergence. As a second main result, a…

Probability · Mathematics 2022-12-15 Benjamin Gess , Rishabh S. Gvalani , Vitalii Konarovskyi

We establish optimal convergence rates for the continuous piecewise affine finite element approximation of the Sobolev constant in arbitrary dimensions N\geq 2 and for Lebesgue exponents 1<p<N. Our analysis relies on a refined study of the…

Numerical Analysis · Mathematics 2026-05-28 Liviu I. Ignat , Enrique Zuazua

We study a one-dimensional one-phase Stefan problem with a Neumann boundary condition on the fixed part of the boundary. We construct the unique self-similar solution, and show that starting from arbitrary initial data, solution orbits…

Analysis of PDEs · Mathematics 2024-02-05 Danielle Hilhorst , Sabrina Roscani , Piotr Rybka

Over the past decade, various matrix completion algorithms have been developed. Thresholded singular value decomposition (SVD) is a popular technique in implementing many of them. A sizable number of studies have shown its theoretical and…

Methodology · Statistics 2016-05-10 Juhee Cho , Donggyu Kim , Karl Rohe

We have shown that the vector of the point spread function (PSF) lexicographical presentation belongs to the left side conjugated null space (NS) of the autoregression (AR) matrix operator on condition the AR parameters are common for…

Computer Vision and Pattern Recognition · Computer Science 2015-03-02 Yuriy A. Bunyak , Roman N. Kvetnyy , Olga Yu. Sofina

Machine learning problems such as neural network training, tensor decomposition, and matrix factorization, require local minimization of a nonconvex function. This local minimization is challenged by the presence of saddle points, of which…

Optimization and Control · Mathematics 2018-07-23 Santiago Paternain , Aryan Mokhtari , Alejandro Ribeiro

Achieving self-consistent convergence with the conventional effective-mass approach at ultra-low temperatures (below $4.2~K$) is a challenging task, which mostly lies in the discontinuities in material properties (e.g., effective-mass,…

Mesoscale and Nanoscale Physics · Physics 2025-04-14 Vahid Mosallanejad , Haiou Li , Gang Cao , Kuei-Lin Chiu , Wenjie Dou , Guo-ping Guo

We present a unified framework for analyzing local SGD methods in the convex and strongly convex regimes for distributed/federated training of supervised machine learning models. We recover several known methods as a special case of our…

Machine Learning · Computer Science 2020-11-06 Eduard Gorbunov , Filip Hanzely , Peter Richtárik

Proofs of convergence of adaptive finite element methods for the approximation of eigenvalues and eigenfunctions of linear elliptic problems have been given in a several recent papers. A key step in establishing such results for multiple…

Numerical Analysis · Mathematics 2016-05-27 Andrea Bonito , Alan Demlow

Federated Averaging (FedAvg), also known as Local SGD, is one of the most popular algorithms in Federated Learning (FL). Despite its simplicity and popularity, the convergence rate of FedAvg has thus far been undetermined. Even under the…

Machine Learning · Computer Science 2022-02-15 Margalit Glasgow , Honglin Yuan , Tengyu Ma

We present a modification of the $\Delta$SCF method of calculating energies of excited states, in order to make it applicable to resonance calculations of molecules adsorbed on metal surfaces, where the molecular orbitals are highly…

Materials Science · Physics 2009-03-06 Jeppe Gavnholt , Thomas Olsen , Mads Engelund , Jakob Schiøtz

Sparse Inverse Covariance Estimation (SICE) is useful in many practical data analyses. Recovering the connectivity, non-connectivity graph of covariates is classified amongst the most important data mining and learning problems. In this…

Machine Learning · Computer Science 2019-04-05 Ashkan Esmaeili , Farokh Marvasti

A computationally efficient method to solve non-convex programming problems with linear equality constraints is presented. The proposed method is based on a recursively feasible and descending sequential convex programming procedure proven…

Optimization and Control · Mathematics 2018-10-25 Josep Virgili-Llop , Marcello Romano

For solving large-scale non-convex problems, we propose inexact variants of trust region and adaptive cubic regularization methods, which, to increase efficiency, incorporate various approximations. In particular, in addition to approximate…

Optimization and Control · Mathematics 2018-02-21 Zhewei Yao , Peng Xu , Farbod Roosta-Khorasani , Michael W. Mahoney

It is shown that the superconformal filling (SCF) efficiency ($\epsilon_{SCF}$) of nano-scale cavities can be rationalized in terms of relevant physical and geometric parameters. Based on extensive numerical simulations and using the…

Materials Science · Physics 2009-11-07 A. De Virgiliis , O. Azzaroni , R. C. Salvarezza , E. V. Albano

The selective frequency damping (SFD) method is an alternative to classical Newton's method to obtain unstable steady-state solutions of dynamical systems. However this method has two main limitations: it does not converge for arbitrary…

Fluid Dynamics · Physics 2015-10-28 Bastien E. Jordi , Colin J. Cotter , Spencer J. Sherwin
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