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We perform a combined experimental and theoretical investigation of the orientational dynamics of rod-like colloidal particles in dilute suspension as they are subjected to a time-dependent homogeneous planar elongational flow. Our…

Complex fluids containing low concentrations of slender colloidal rods can display a high viscosity, while little flow is needed to thin the fluid. This feature makes slender rods essential constituents in industrial applications and…

Polymers and rod-like colloids (PaRC) adopt a favorable orientation under sufficiently strong flows. However, how the flow kinematics affect the alignment of such nanostructures according to their extensibility remains unclear. By analysing…

Cellulose nanocrystals (CNC) are naturally-derived nanostructures of growing importance for the production of composites having attractive mechanical properties, and offer improved sustainability over purely petroleum-based alternatives.…

Soft Condensed Matter · Physics 2019-01-15 Abhinav Rao , Thibaut Divoux , Gareth H. McKinley , A. John Hart

Orientation and relaxation dynamics of rod-like colloids under flow govern the optical and mechanical properties of many emerging soft materials. In polydisperse suspensions, particles of different lengths exhibit distinct rotational…

Soft Condensed Matter · Physics 2026-04-23 Yuto Yokoyama , Vincenzo Calabrese , Fabian Hillebrand , Henry J. London , Simon J. Haward , Amy Q. Shen

Cellulose nanocrystals (CNCs) are polycrystalline, rod-shaped nanoparticles isolated from cellulose, which have attracted increasing attention for a wide variety of applications. While there has been significant research into CNCs in…

Hypothesis Understanding the scission of rod-like micelles under mechanical forces is crucial for optimizing their stability and behavior in industrial applications. This study investigates how micelle length, flexibility, and external…

Soft Condensed Matter · Physics 2025-01-24 Guan-Rong Huang , Ryan P. Murphy , Lionel Porcar , Chi-Huan Tung , Changwoo Do , Wei-Ren Chen

Cellulose nanocrystals (CNCs) are elongated nanoparticles derived from natural cellulose, with potential applications ranging from rheological modifiers and emulsion stabilizers to photonic pigments and sensors. For most applications,…

The increased availability and brilliance of new X-ray facilities have in the recent years opened up the possibility to characterize the motion of dispersed nanoparticles in various microfluidic applications. One of these applications is…

Soft Condensed Matter · Physics 2018-04-24 Tomas Rosén , Christophe Brouzet , Stephan V. Roth , Fredrik Lundell , L. Daniel Söderberg

We study the flow stability and spatio-temporal spectral dynamics of cellulose nanocrystal (CNC) suspensions in a custom Taylor-Couette flow cell using the intrinsic shear induced birefringence and liquid crystalline properties of CNC…

New materials made through controlled assembly of dispersed cellulose nanofibrils (CNF) has the potential to develop into biobased competitors to some of the highest performing materials today. The performance of these new cellulose…

Soft Condensed Matter · Physics 2020-06-02 Tomas Rosén , Nitesh Mittal , Stephan V. Roth , Peng Zhang , L. Daniel Söderberg , Fredrik Lundell

There is now convincing evidence that inter-particle frictional contacts are essential for observing shear-thickening in concentrated suspensions of compact particles. While this has inspired many strategies to tailor the rheology in these…

Soft Condensed Matter · Physics 2020-04-15 Vikram Rathee , Srishti Arora , Daniel L. Blair , Jeffrey S. Urbach , A. K. Sood , Rajesh Ganapathy

Main characteristics of colloidal systems that develop fluid phases with different mechanical properties, namely shear-banding fluids, are briefly reviewed both from experimental and theoretical (modelling) point of view. A non-monotonic…

Soft Condensed Matter · Physics 2009-03-05 Daniel Quemada , Claudio Berli

The rheology of dense granular shear flows is influenced by friction and particle shape. We investigate numerically the impact of non-spherical particle geometries under shear on packing fraction, stress ratios, velocity fluctuations, force…

Soft Condensed Matter · Physics 2025-11-04 Jacopo Bilotto , Martin Trulsson , Jean-François Molinari

We use a nonequilibrium variational principle to optimize the steady-state, shear-induced interconversion of self-assembled nanoclusters of DNA-coated colloids. Employing this principle within a stochastic optimization algorithm allows us…

Soft Condensed Matter · Physics 2023-08-23 Avishek Das , David T. Limmer

We assess the possibility of shear banding of semidilute rod-like colloidal suspensions under steady shear ow very close to the isotropic-nematic spinodal, using a combination of rheology, small angle neutron scattering, and laser Doppler…

Soft Condensed Matter · Physics 2018-12-03 Christian Lang , Lionel Porcar , Hartmut Kriegs , M. Paul Lettinga

The evolution of wide shear zones (or shear bands) was investigated experimentally and numerically for quasistatic dry granular flows in split bottom shear cells. We compare the behavior of materials consisting of beads, irregular grains…

We present a single, unified, multi-scale model to study the attachment\detachment dynamics of two deforming, near spherical cells, coated with binding ligands and subject to a slow, homogeneous shear flow in a viscous fluid medium. The…

Cell Behavior · Quantitative Biology 2015-04-23 Sarthok Sircar , Anthony J. Roberts

This study systematically investigates the flow birefringence of cellulose nanocrystal (CNC) suspensions. The aim is to clarify the importance of the stress component along the camera's optical axis in the stress-optic law (SOL), which…

Understanding the hydrodynamic alignment of colloidal rods in polymer solutions is pivotal for manufacturing structurally ordered materials. How polymer crowding influences the flow-induced alignment of suspended colloidal rods remains…

Soft Condensed Matter · Physics 2022-10-12 Vincenzo Calabrese , Stylianos Varchanis , Simon J. Haward , Amy Q. Shen
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