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Core-shell electrode particle designs offer a route to improved lithium-ion battery performance. However, they are susceptible to mechanical damage such as fracture and debonding, which can significantly reduce their lifetime. Using a…

Chemical Physics · Physics 2024-03-21 Y. Tu , B. Wu , W. Ai , E. Martínez-Pañeda

We present an atomistic model of a single nanoparticle with core/shell structure that takes into account its lattice strucutre and spherical geometry, and in which the values of microscopic parameters such as anisotropy and exchange…

Materials Science · Physics 2009-09-29 Oscar Iglesias , Amilcar Labarta , Xavier Batlle

Understanding the oxidation and reduction mechanisms of catalytically active transition metal nanoparticles is important to improve their application in a variety of chemical processes. In nanocatalysis the nanoparticles can undergo…

Chemical Physics · Physics 2017-05-18 Alec Lagrow , Michael Ward , David Lloyd , Pratibha Gai , Edward Boyes

FePt nanoparticles are known to exhibit reduced L1$_0$ order with decreasing particle size. The reduction in order reduces the magnetic anisotropy and the thermal stability of the direction of magnetization of the particle. The phenomenon…

Mesoscale and Nanoscale Physics · Physics 2009-11-18 Roman V. Chepulskii , W. H. Butler , A. van de Walle , Stefano Curtarolo

We present temperature-, magnetic-field-, and pressure-dependent Raman scattering studies of single crystal Mn3O4, combined with temperature- and field-dependent x-ray diffraction studies, revealing the novel magnetostructural phases in…

Strongly Correlated Electrons · Physics 2015-05-28 M. Kim , X. M. Chen , X. Wang , C. S. Nelson , R. Budakian , P. Abbamonte , S. L. Cooper

The surface stabilized MnO(100)-like monolayer, characterised by a regular c(4x2) distribution of Mn vacancies, is studied by hybrid functionals and discussed in the light of available scanning tunneling microscopy and high-resolution…

Materials Science · Physics 2009-11-13 C. Franchini , J. Zabloudil , R. Podloucky , F. Allegretti , F. Li , S. Surnev , F. P. Netzer

Some of the main experimental observations related to the occurrence of exchange bias in magnetic systems are reviewed, focusing the attention on the peculiar phenomenology associated to nanoparticles with core/shell structure as compared…

Materials Science · Physics 2008-06-20 Oscar Iglesias , Amilcar Labarta , Xavier Batlle

Ferromagnetic-ferroelectric nanocomposites are of interest for realizing strong strain mediated coupling between electric and magnetic subsystems due to high surface area-to-volume ratio. This report is on the synthesis of nickel ferrite…

Materials Science · Physics 2017-12-27 G. Sreenivasulu , Jitao Zhang , Ru Zhang , M. Popov , V. M. Petrov , G. Srinivasan

Mott transitions in real materials are first order and almost always associated with lattice distortions, both features promoting the emergence of nanotextured phases. This nanoscale self-organization creates spatially inhomogeneous…

We present a study of the control of electric field induced strain on the magnetic and electrical transport properties in a magneto-elastically coupled artificial multiferroic Fe3O4/BaTiO3 heterostructure. In this Fe3O4/BaTiO3…

We present a microscopic model for nanoparticles, of the maghemite ($\gamma $% -Fe$_{2}$O$_{3}$) type, and perform classical Monte Carlo simulations of their magnetic properties. On account of M\"{o}ssbauer spectroscopy and high-field…

Materials Science · Physics 2009-10-31 H. Kachkachi , A. Ezzir , M. Nogues , E. Tronc

Engineering strain critically affects the properties of materials and has extensive applications in semiconductors and quantum systems. However, the deployment of strain-engineered nanocatalysts faces challenges, particularly in maintaining…

Materials Science · Physics 2024-07-29 Chuqiao Shi , Zhihua Cheng , Alberto Leonardi , Yao Yang , Michael Engel , Matthew R. Jones , Yimo Han

The nanostructural evolution of the strain-induced structural phase transition in BiFeO3 is examined. Using high-resolution X-ray diffraction and scanning-probe microscopy-based studies we have uniquely identified and examined the numerous…

Materials Science · Physics 2011-05-23 A. R. Damodaran , C. -W. Liang , Q. He , C. -Y. Peng , L. Chang , Y. -H. Chu , L. W. Martin

The nanoscale distribution of magnetic anisotropies was measured in core@shell MnFe$_2$O$_4$@CoFe$_2$O$_4$ 7.0 nm particles using a combination of element selective magnetic spectroscopies with different probing depths. As this picture is…

Cathode materials undergo various phase transitions during the charge/discharge process, and the structural transitions significantly affect the battery performance. Although phonon properties can provide a direct clue for structural…

Materials Science · Physics 2022-08-08 Haeyoon Jung , Jiyeon Kim , Sooran Kim

The structure and magnetic properties of Mn1+xV2-xO4 (0<x<=1), a complex frustrated system, were investigated by heat capacity, magnetization, x-ray diffraction, and neutron diffraction measurements. For x<=0.3, a cubic-to-tetragonal (c >…

Strongly Correlated Electrons · Physics 2020-10-07 J. L. Jiao , H. P. Zhang , Q. Huang , W. Wang , G. Wang , Q. Ren , R. Sinclair , G. T. Lin , A. Huq , H. Cao , H. D. Zhou , M. Z. Li , J. Ma

Transition metal spinel oxides comprised of Earth-abundant Mn and Co have long been explored for their use in catalytic reactions and energy storage. However, understanding of functional properties can be challenging due to differences in…

The reduction of ferromanganese ores into metallic feedstock is an energy-intensive process with substantial carbon emissions, necessitating sustainable alternatives. Hydrogen-based pre-reduction of manganese-rich ores offers a low-emission…

Materials Science · Physics 2025-07-15 Anurag Bajpai , Barak Ratzker , Shiv Shankar , Dierk Raabe , Yan Ma

We study dilute suspensions of magnetic nanoparticles in a nematic host, on two-dimensional (2D) polygons. These systems are described by a nematic order parameter and a spontaneous magnetization, in the absence of any external fields. We…

Soft Condensed Matter · Physics 2021-05-19 Yucen Han , Joseph Harris , Joshua Walton , Apala Majumdar

Heteroepitaxy offers a new type of control mechanism for the crystal structure, the electronic correlations, and thus the functional properties of transition-metal oxides. Here, we combine electrical transport measurements, high-resolution…