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The magnetic insulator $\alpha$-RuCl$_{3}$ is a promising candidate to realize Kitaev interactions on a quasi-2D honeycomb lattice. We perform extensive susceptibility measurements on single crystals of $\alpha$-RuCl$_{3}$, including…

We investigate the structural and magnetic properties of a Kitaev spin liquid candidate material Ag$_3$LiIr$_2$O$_6$ based on $^7$Li nuclear magnetic resonance line shape, Knight shift and spin-lattice relaxation rate $1/T_1$. The first…

Strongly Correlated Electrons · Physics 2021-06-18 Jiaming Wang , Weishi Yuan , Takashi Imai , Philip M. Singer , Faranak Bahrami , Fazel Tafti

Motivated by the rich interplay among electronic correlation, spin-orbit coupling (SOC), crystal-field splitting, and geometric frustrations in the honeycomb-like lattice, we systematically investigated the electronic and magnetic…

Strongly Correlated Electrons · Physics 2013-05-01 Yongkang Luo , Chao Cao , Bingqi Si , Yuke Li , Jinke Bao , Hanjie Guo , Xiaojun Yang , Chenyi Shen , Chunmu Feng , Jianhui Dai , Guanghan Cao , Zhu-an Xu

Motivated by the absence of both spin freezing and a cooperative Jahn-Teller effect at the lowest measured temperatures, we study the ground state of Ba3CuSb2O9. We solve a general spin-orbital model on both the honeycomb and the decorated…

Strongly Correlated Electrons · Physics 2014-10-02 Andrew Smerald , Frederic Mila

The honeycomb compound $\alpha$-RuCl$_3$ is widely discussed as a proximate Kitaev spin-liquid material. This scenario builds on spin-orbit entangled $j = 1/2$ moments arising for a $t_{2g}^5$ electron configuration with strong spin-orbit…

Strongly Correlated Electrons · Physics 2020-10-21 P. Warzanowski , N. Borgwardt , K. Hopfer , T. C. Koethe , P. Becker , V. Tsurkan , A Loidl , M. Hermanns , P. H. M. van Loosdrecht , M. Grüninger

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

Due to the combination of a substantial spin-orbit coupling and correlation effects, iridium oxides hold a prominent place in the search for novel quantum states of matter, including, e.g., Kitaev spin liquids and topological Weyl states.…

Strongly Correlated Electrons · Physics 2017-07-11 Vamshi M. Katukuri , Ravi Yadav , Liviu Hozoi , Satoshi Nishimoto , Jeroen van den Brink

We discuss magnetically ordered states, arising in Heisenberg-Kitaev and related spin models, on three-dimensional (3D) harmonic honeycomb lattices. For large classes of ordered states, we show that they can be mapped onto two-dimensional…

Strongly Correlated Electrons · Physics 2020-01-29 Wilhelm G. F. Krüger , Matthias Vojta , Lukas Janssen

In this computational study, we explore a viable route to access the Kitaev-Quantum Spin Liquid (QSL) state in recently synthesized monolayer of a so-called spin-orbit assisted Mott insulator OsCl$_3$. In addition to other magnetic ground…

Strongly Correlated Electrons · Physics 2025-01-14 Qiangqiang Gu , Shishir Kumar Pandey , Yihao Lin

The exactly solvable Kitaev model on the honeycomb lattice has recently received enormous attention linked to the hope of achieving novel spin-liquid states with fractionalized Majorana-like excitations. In this review, we analyze the…

The Kitaev interaction in a honeycomb lattice with higher-spin $S$ has been one of the central attractions, as it may offer quantum spin liquids. A microscopic theory showed that when the Hund's coupling at the transition metal generates…

Strongly Correlated Electrons · Physics 2024-01-23 Jiefu Cen , Hae-Young Kee

A polycrystalline sample of the hyperhoneycomb iridate $\beta$-ZnIrO$_3$ was synthesized via a topochemical reaction, and its structural, magnetic, and thermodynamic properties were investigated. The magnetization and heat capacity data…

Strongly Correlated Electrons · Physics 2022-02-17 Yuya Haraguchi , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

Spin liquid ground states are predicted to arise within several distinct scenarios in condensed matter physics. The observation of these disordered magnetic states is particularly pervasive amongst a class of materials known as frustrated…

We report magnetization and neutron diffraction studies on crystal and magnetic structures of Ir- and Rh-substituted honeycomb lattice $\alpha$-RuCl$_3$. The iridium or rhodium atoms are distributed at the Ru site with little structural…

Materials Science · Physics 2023-10-05 Zachary Morgan , Iris Ye , Colin L. Sarkis , Xiaoping Wang , Stephen Nagler , Jiaqiang Yan

The search for a Kitaev quantum spin liquid in crystalline magnetic materials has fueled intense interest in the two-dimensional honeycomb systems. Many promising candidate Kitaev systems are characterized by a long range ordered magnetic…

Strongly Correlated Electrons · Physics 2024-10-16 V. Ovidiu Garlea , Colin L. Sarkis

The layered honeycomb magnet $\alpha$-RuCl$_3$ has emerged as a promising candidate for realizing a Kitaev quantum spin liquid. Previous studies have reported oscillation-like anomalies in the longitudinal thermal conductivity and…

Strongly Correlated Electrons · Physics 2025-04-01 Y. Xing , R. Namba , K. Imamura , K. Ishihara , S. Suetsugu , T. Asaba , K. Hashimoto , T. Shibauchi , Y. Matsuda , Y. Kasahara

The honeycomb-lattice cobaltate Na$_3$Co$_2$SbO$_6$ has recently been proposed to be a proximate Kitaev quantum spin liquid~(QSL) candidate. However, non-Kitaev terms in the Hamiltonian lead to a zigzag-type antiferromagnetic~(AFM) order at…

Maximizing the ratio between Kitaev and residual Heisenberg interactions is a major goal in nowadays research on Kitaev-Heisenberg quantum magnets. Here we investigate Kitaev-Heisenberg exchange in a recently discovered crystalline phase of…

Strongly Correlated Electrons · Physics 2023-12-15 Pritam Bhattacharyya , Liviu Hozoi , Quirin Stahl , Jochen Geck , Nikolay A. Bogdanov

Quantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T = 0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin…

Strongly Correlated Electrons · Physics 2020-11-20 C. Wessler , B. Roessli , K. W. Krämer , B. Delley , O. Waldmann , L. Keller , D. Cheptiakov , H. B. Braun , M. Kenzelmann

Competition and cooperation between electron correlation and relativistic spin-orbit coupling give rise to diverse exotic quantum phenomena in solids. An illustrative example is spin-orbit entangled quantum liquids, which exhibit remarkable…

Strongly Correlated Electrons · Physics 2024-03-15 Yi-Feng Zhao , Seong-Hoon Jang , Yukitoshi Motome
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