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Ion flow in charged nanopores is strongly influenced by the ratio of the Debye length to the pore radius. We investigate the asymptotic behaviour of solutions to the Poisson-Nernst-Planck (PNP) system in narrow pore like geometries and…

Analysis of PDEs · Mathematics 2019-04-10 B. Matejczyk , J. -F. Pietschmann , G. Richardson , M. -T. Wolfram

Based on ab initio density-functional-theory using generalized gradient approximation, we systematically study the optical and electronic properties of the insulating dense sodium phase (Na-hp4) reported recently [Ma \textit{et al.}, Nature…

Materials Science · Physics 2015-05-18 Dafang Li , Hanyu Liu , Bao-Tian Wang , Hongliang Shi , Shao-Ping Zhu , Jun Yan , Ping Zhang

An appropriate model Hamiltonian based formalism is proposed for a random adsorbate layer with arbitrary coverage and the ensuing two-dimensional band formation by metallic adsorbates in the monolayer regime. The coherent potential…

Chemical Physics · Physics 2007-05-23 A. K. Mishra

In this report we present systematic magnetic studies of pure iron oxide nanoparticles and gold iron oxide nanocomposite with increasing Au particle size/content. For the magnetic studies of these samples we have measured: (1) zero field…

Materials Science · Physics 2009-10-26 S. Banerjee , S. O. Raja , M. Sardar , N. Gayathri , B. Ghosh , A. Dasgupta

Mean-field theory is used to model polyelectrolyte adsorption and the possibility of overcompensation of charged surfaces. For charged surfaces that are also chemically attractive, the overcharging is large in high salt conditions,…

Soft Condensed Matter · Physics 2009-11-10 Adi Shafir , David Andelman

Fundamental understanding of ionic transport at the nanoscale is essential for developing biosensors based on nanopore technology and new generation high-performance nanofiltration membranes for separation and purification applications. We…

Explicit molecular dynamics simulations were applied to a pair of amorphous silica nanoparticles in aqueous solution, of diameter 4.4 nm with four different background electrolyte concentrations, to extract the mean force acting between the…

Chemical Physics · Physics 2009-11-13 S. Jenkins , S. R. Kirk , M. Persson , J. Carlen , Z. Abbas

The ionic selectivity of nanopores is crucial for the energy conversion based on nanoporous membranes. It can be significantly affected by various parameters of nanopores and the applied fields driving ions through porous membranes. Here,…

Soft Condensed Matter · Physics 2024-10-29 Chao Zhang , Mengnan Guo , Hongwen Zhang , Xiuhua Ren , Yinghao Gao , Yinghua Qiu

Pd nanoalloys show great potential as hysteresis-free, reliable hydrogen sensors. Here, a multi-scale modeling approach is employed to determine optimal conditions for optical hydrogen sensing using the Pd-Au-H system. Changes in hydrogen…

In this study nanoscale structure and associated energy dissipation behavior of nanoparticulates of tungsten disulphide (WS2) and nanoparticles of gold (Au) were investigated by advanced scanning probe and electron microscopy techniques.…

Mesoscale and Nanoscale Physics · Physics 2013-11-13 D. Devaprakasam

The present paper deals with the systematic growth of plasmonic gold nanoparticles (Au NPs) on molybdenum disulphide (MoS$_2$) nanosheets as well as the effect of Au NPs on the optical and magnetic properties. The crystalline nature of the…

Materials Science · Physics 2020-01-30 Anjali Rani , Arun Singh Patel , Anirban Chakraborti , Kulvinder Singh , Prianka Sharma

We have employed the highly accurate complex absorbing potential based ionization potential equation-of-motion coupled cluster singles and doubles (CAP-IP-EOM-CCSD) method to study the various intermolecular decay processes in ionized…

Chemical Physics · Physics 2022-08-05 Ravi Kumar , Aryya Ghosh , Nayana Vaval

Nanoscopic heterogeneities in composition and structure are quintessential for the properties of electrocatalyst materials. Here, we present a semiclassical model to study the electrochemical properties of supported electrocatalyst…

Materials Science · Physics 2025-02-27 Yufan Zhang , Tobias Binninger , Jun Huang , Michael Eikerling

The specific role played by small gold nanoparticles supported on the rutile TiO2(110) surface in the processes of adsorption and dissociation of H2 is discussed. It is demonstrated that the molecular and dissociative adsorption of H2 on…

Atomic and Molecular Clusters · Physics 2011-08-18 Andrey Lyalin , Tetsuya Taketsugu

Ion hydration and interfacial water play crucial roles in numerous phenomena ranging from biological to industrial systems. Although biologically relevant (and mostly smaller) ions have been studied extensively in this context, very little…

Soft Condensed Matter · Physics 2019-01-01 William Rock , Baofu Qiao , Tiecheng Zhou , Aurora E. Clark , Ahmet Uysal

We report the results of molecular dynamics simulations of the properties of a pseudo-atom model of dodecane thiol ligated 5-nm diameter gold nanoparticles (AuNP) in vacuum as a function of ligand coverage and particle separation in three…

Chemical Physics · Physics 2019-02-20 Christopher Liepold , Alex Smith , Binhua Lin , Juan de Pablo , Stuart A. Rice

A series of well-defined hydrophilic and hydrophobic polyelectrolytes of various chain lengths $N$ and effective charge fractions $f_{eff}$ have been adsorbed onto oppositely charged solid surfaces immersed in aqueous solutions. \emph{In…

Sorbent materials are a promising alternative to advance hydrogen storage technologies. The general disadvantage is the relatively weak solid-gas interaction and adsorption energy, providing low gravimetric and volumetric capacities and…

Materials Science · Physics 2022-11-28 Shima Rezaie , David M. J. Smeulders , Azahara Luna-Triguero

This article describes the optical properties of nanostructures composed of silver particles embedded into a gold matrix. In previous studies these materials were shown to exhibit temperature dependent transitions to a highly conductive and…

Understanding the local structure of water at the interfaces of metallic electrodes is a key problem in aqueous-based electrochemistry. Nevertheless, a realistic simulation of such setup is challenging, particularly when the electrodes are…

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