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We introduce a new parallelized approach to photothermal microscopy that utilizes mid-infrared dual-comb lasers, enabling simultaneous measurements at hundreds of wavelengths. This technology allows for high-speed, label-free chemical…

We report on a mode-locked laser design using Yb-doped fiber lasers for low-noise frequency-comb generation. The frequency comb covers the spectral range from $700$ to $1400$ nm. Although this range is more practical for many measurements…

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for…

Atomic Physics · Physics 2018-06-13 Bachana Lomsadze , Steven T. Cundiff

We describe methods using frequency combs and optical resonators for recording two-dimensional (2D) ultrafast spectroscopy signals with high sensitivity. By coupling multiple frequency combs to higher-order modes of one or more optical…

Optics · Physics 2017-01-25 Thomas K. Allison

Mid-infrared laser frequency combs are compelling sources for precise and sensitive metrology with applications in molecular spectroscopy and spectro-imaging. The infrared atmospheric window between 3-5.5 $\mu$m in particular provides vital…

Broadband dual-comb spectroscopy has attracted increasing interests due to its unique advantages in high spectral resolution, fast detection, and so on. Although the dual-comb technique is relatively mature in the infrared wavelengths, it…

Dual-comb interferometry harnesses the interference of two laser frequency combs to provide unprecedented capability in spectroscopy applications. In the past decade, the state-of-the-art systems have reached a point where the…

Quantum Physics · Physics 2023-09-20 Haowei Shi , Zaijun Chen , Scott E. Fraser , Mengjie Yu , Zheshen Zhang , Quntao Zhuang

The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

The interferometric signals produced in conventional dual-comb laser ranging require femtosecond lasers with long-term f_CEO stability, and are limited to an upper sampling rate by radio-frequency aliasing considerations. By using…

Instrumentation and Detectors · Physics 2021-08-24 Hollie Wright , Jinghua Sun , David McKendrick , Nick Weston , Derryck T. Reid

Mode-resolved dual-comb spectroscopy (DCS) is an emerging spectroscopic tool with the potential to simultaneously achieve a broad spectral coverage and ultrahigh spectral resolution in terahertz (THz) spectroscopy. However, the need for two…

Instrumentation and Detectors · Physics 2020-06-02 Jie Chen , Kazuki Nitta , Xin Zhao , Takahiko Mizuno , Takeo Minamikawa , Francis Hindle , Zheng Zheng , Takeshi Yasui

Laser dynamics underpin a broad range of modern photonic technologies and continue to reveal rich nonlinear behaviors. However, existing spectroscopic tools, most notably time-stretched dispersive Fourier transform spectroscopy (TS-DFT),…

Continuous wave (CW) lasers are the enabling technology for producing ultracold atoms and molecules through laser cooling and trapping. The resulting pristine samples of slow moving particles are the de facto starting point for both…

Atomic Physics · Physics 2016-10-19 A. M. Jayich , X. Long , W. C. Campbell

A multichannel dual-comb spectroscopy (DCS) approach for high-resolution, broadband spectral measurements is presented, demonstrating its effectiveness in studying complex atomic systems. By implementing a photodetector array, we enhance…

Atomic Physics · Physics 2025-03-14 R. Aramyan , O. Tretiak , S. S. Sahoo , D. Budker

We report ultra-low phase-noise microwave generation at a 9.6 GHz carrier frequency from optical frequency combs based on diode-pumped solid-state lasers emitting at telecom wavelength and referenced to a common cavity-stabilized…

We report molecular detection using dual frequency-comb spectroscopy with highly coherent broadband (6.6-11.4 {\m}m) long-wavelength infrared (LWIR) combs. The combs were produced via intra-pulse difference frequency generation (IDFG) in…

Dual-comb interferometry is based on self-heterodyning two optical frequency combs, with corresponding mapping of the optical spectrum into the radio-frequency domain. The dual-comb enables diverse applications, including metrology, fast…

We present a simple method for fully-stabilized mid-infrared optical frequency comb generation based on single-pass femtosecond optical parametric generation that is seeded by a continuous-wave laser. We have implemented the method in a…

Optics · Physics 2024-06-12 Mikhail Roiz , Krishna Kumar , Juho Karhu , Markku Vainio

Optical frequency combs based on semiconductor lasers are a promising technology for monolithic integration of dual-comb spectrometers. However, the stabilization of the offset frequency fceo remains a challenging feat due the lack of…

We present a compact, reliable, and robust free-running all-polarization-maintaining erbium (Er) single-cavity dual-comb laser generated via polarization multiplexing with gain sharing. Polarization multiplexing exploits the fast and slow…

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