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We report on a combined experimental and theoretical study on CrI3 single crystals by employing the polarization dependence of resonant inelastic X-ray scattering (RIXS). Our investigations reveal multiple Cr 3d orbital splitting (dd…

Density functional theory augmented with Hubbard-$U$ corrections (DFT+$U$) is currently one of the widely used methods for first-principles electronic structure modeling of insulating transition metal oxides (TMOs). Since $U$ is relatively…

Computational Physics · Physics 2018-05-09 Samara Keshavarz , Johan Schött , Andrew J. Millis , Yaroslav O. Kvashnin

We extend density matrix embedding theory to periodic systems, resulting in an electronic band structure method for solid-state materials. The electron correlation can be captured by means of a local impurity model using various choices of…

Strongly Correlated Electrons · Physics 2019-09-27 Hung Q. Pham , Matthew R. Hermes , Laura Gagliardi

Streamlined prediction of the electronic properties of photoactive materials warrants a Density Functional Theory (DFT) based approach that (i) yields reliable bandgaps, (ii) is free of empirically tuned parameters, and (iii) exhibits low…

Materials Science · Physics 2025-12-17 Andrew C. Burgess , Lórien MacEnulty , Ethan D'Arcy , David Gavin , David D. O'Regan

Ab initio calculation of the electronic properties of materials is a major challenge for solid state theory. Whereas the experience of forty years has proven density functional theory (DFT) in a suitable, e.g. local approximation (LDA) to…

Strongly Correlated Electrons · Physics 2009-11-13 K. Held , O. K. Andersen , M. Feldbacher , A. Yamasaki , Y. -F. Yang

Oxide heterostructures allow for detailed studies of 2D electronic transport phenomena. Herein, different facets of magnetotransport in selected spin-orbit-coupled systems are analyzed and characterized by their single-band and multiband…

Mesoscale and Nanoscale Physics · Physics 2021-10-14 Robert Bartel , Elias Lettl , Patrick Seiler , Thilo Kopp , German Hammerl

The latest discovery of ferromagnetism in atomically thin films of semiconductors Cr$_2$Ge$_2$Te$_6$ and CrI$_3$ has unleashed numerous opportunities for fundamental physics of magnetism in two-dimensional (2D) limit and also for…

Mesoscale and Nanoscale Physics · Physics 2019-05-09 Vijay Kumar Gudelli , Guang-Yu Guo

The effect of on-site electron-electron repulsion $U$ in a band insulator is explored for a bilayer Hubbard Hamiltonian with opposite sign hopping in the two sheets. The ground state phase diagram is determined at half-filling in the plane…

Strongly Correlated Electrons · Physics 2013-04-09 Axel Euverte , Simone Chiesa , Richard . T. Scalettar , George G. Batrouni

The dynamical mean-field theory together with the non-crossing approximation is used to set up a novel scheme to study the electronic structure of strongly correlated electron systems. The non-interacting band structure is obtained from a…

Strongly Correlated Electrons · Physics 2007-05-23 M. B. Zoelfl , Th. Pruschke , J. Keller , A. I. Poteryaev , I. A. Nekrasov , V. I. Anisimov

Using density functional theory (DFT), Hartree-Fock, exact diagonalization, and numerical renormalization group methods we study the electronic structure of diluted hydrogen atoms chemisorbed on graphene. A comparison between DFT and…

Mesoscale and Nanoscale Physics · Physics 2012-03-07 J. O. Sofo , Gonzalo Usaj , P. S. Cornaglia , A. M. Suarez , A. D. Hernández-Nieves , C. A. Balseiro

The magnetic ground states of $R_2$Ru$_2$O$_7$ and $A_2$Ru$_2$O$_7$ with $R=$ Pr, Gd, Ho, and Er, as well as $A=$ Ca, Cd are predicted devising a combination of the cluster-multipole (CMP) theory and spin-density-functional theory (SDFT).…

Strongly Correlated Electrons · Physics 2022-02-22 Marie-Therese Huebsch , Yuske Nomura , Shiro Sakai , Ryotaro Arita

Optical spectroscopy, X-ray diffraction measurements, density functional theory (DFT) and density functional theory + embedded dynamical mean field theory (DFT+eDMFT) have been used to characterize structural and electronic properties of…

Strongly Correlated Electrons · Physics 2020-09-23 T. N. Stanislavchuk , G. L. Pascut , A. P. Litvinchuk , Z. Liu , S. Choi , M. J. Gutmann , B. Gao , K. Haule , V. Kiryukhin , S. -W. Cheong , A. A. Sirenko

Using density functional theory plus Hubbard-U (DFT+U) approach, we find that quasi one-dementation(1D) 3d transition metal(TM) zigzag nanowire can be constructed by TM adsorbed on the surface of graphyne sheet. The results show that the TM…

Materials Science · Physics 2013-05-22 Junjie He , Pan Zhou , N. Jiao , S. Y. Ma , K. W. Zhang , R. Z. Wang , L. Z. Sun

We employ density-functional theory (DFT) in the generalized gradient approximation (GGA) and its extensions GGA+$U$ and GGA+Gutzwiller to calculate the magnetic exchange couplings between pairs of Mn ions substituting Cd in a CdTe crystal…

Strongly Correlated Electrons · Physics 2017-02-01 Thorben Linneweber , Jörg Bünemann , Ute Löw , Florian Gebhard , Frithjof Anders

A systematic density functional theory (DFT)+U study is conducted to investigate the electron correlation and spin-orbit coupling (SOC) effects in US3 and USe3. Our calculations reveal that inclusion of the U term is essential to get energy…

Strongly Correlated Electrons · Physics 2012-12-13 Yu Yang , Wei Yang , Ping Zhang

We conduct a comprehensive study of three different magnetic semiconductors, CrI$_3$, CrBr$_3$, and CrCl$_3$, by incorporating both few- and bi-layer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering,…

We experimentally measure the band dispersions of topological Dirac semimetal Na3Bi using Fourier-transform scanning tunneling spectroscopy to image quasiparticle interference on the (001) surface of molecular-beam epitaxy-grown Na3Bi thin…

Materials Science · Physics 2020-08-26 I. Di Bernardo , J. Collins , W. Wu , J. Zhou , S. A. Yang , S. Ju , M. T. Edmonds , M. S. Fuhrer

We investigate the magnetotransport properties of the one-band Hubbard-Holstein model at half-filling in three dimensions (3D) using exact diagonalization based semi-classical Monte Carlo simulations with phonons treated in the adiabatic…

Strongly Correlated Electrons · Physics 2026-04-21 Sandip Halder , Moshe Schechter

The development of room-temperature magnetic semiconductors is critical for advancing spintronic technologies, yet van der Waals magnets like CrI3 exhibit intrinsically low Curie temperatures (Tc = 45 K). This study employs first-principles…

Materials Science · Physics 2025-08-12 Qing-Han Yang , Jia-Wen Li , Xin-Wei Yi , Xiang Li , Jing-Yang You , Gang Su , Bo Gu

By means of ab initio calculations within the density functional theory (DFT) electronic and magnetic properties of BaTiO3/LaMnO3 interface were investigated. An impact of ferroelectric overlayer thickness onto the interface properties was…

Materials Science · Physics 2022-06-07 Irina Piyanzina , Rinat Mamin