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Glasses are solid materials whose constituent atoms are arranged in a disordered manner. The transition from a liquid to a glass remains one of the most poorly understood phenomena in condensed matter physics, and still no fully microscopic…

Statistical Mechanics · Physics 2015-11-12 Liesbeth M. C. Janssen , David R. Reichman

We present Molecular Dynamics simulations of the thermal glass transition in a dense model polymer liquid. We performed a comparative study of both constant volume and constant pressure cooling of the polymer melt. Great emphasis was laid…

Statistical Mechanics · Physics 2009-10-30 C. Bennemann , W. Paul , K. Binder , B. Duenweg

The dynamical glass transition is typically taken to be the temperature at which a glassy liquid is no longer able to equilibrate on experimental timescales. Consequently, the physical properties of these systems just above or below the…

Soft Condensed Matter · Physics 2017-03-08 Samuel S. Schoenholz , Ekin D. Cubuk , Efthimios Kaxiras , Andrea J. Liu

A liquid can form under cooling a glassy state either as a result of a continuous slowing down or by a first order polyamorphous phase transition. The second scenario has so far always been observed below the melting point where it…

Soft Condensed Matter · Physics 2010-04-16 Måns Elenius , Tomas Oppelstrup , Mikhail Dzugutov

We compute for an archetypical glass-forming system the excess of particle mobility distributions over the corresponding distribution of dynamic propensity, a quantity that measures the tendency of the particles to be mobile and reflects…

Statistical Mechanics · Physics 2014-04-01 Rodriguez Fris J. Ariel , Frechero M. , Appignanesi Gustavo

We give evidence of a clear structural signature of the glass transition, in terms of a static correlation length with the same dependence on the system size which is typical of critical phenomena. Our approach is to introduce an external,…

Statistical Mechanics · Physics 2010-06-25 Majid Mosayebi , Emanuela Del Gado , Patrick Ilg , Hans Christian Ottinger

We report a molecular dynamics (MD) study of the collective dynamics of a simple monatomic liquid -interacting through a two body potential that mimics that of lithium- across the liquid-glass transition. In the glassy phase we find…

Disordered Systems and Neural Networks · Physics 2009-11-07 T. Scopigno , G. Ruocco , F. Sette , G. Viliani

We address the relaxation dynamics in hydrogen-bonded super-cooled liquids near the glass transition, measured via Broad-Band Dielectric Spectroscopy (BDS). We propose a theory based on decomposing the relaxation of the macroscopic dipole…

Soft Condensed Matter · Physics 2009-11-13 H. G. E. Hentschel , Itamar Procaccia

We introduce a three-dimensional lattice gas model to study the glass transition. In this model the interactions come from the excluded volume and particles have five arms with an asymmetrical shape, which results in geometric frustration…

Statistical Mechanics · Physics 2007-05-23 Anastasio Díaz-Sánchez

Due to high viscosity, glassy systems evolve slowly to the ordered state. Results of molecular dynamics simulation reveal that the structural ordering in glasses becomes observable over "experimental" (finite) time-scale for the range of…

Materials Science · Physics 2015-06-24 Anatolii V. Mokshin , Bulat N. Galimzyanov

We report the combined results of molecular dynamics simulations and theoretical calculations concerning various dynamical arrest transitions in a model system representing a dipolar fluid, namely, N (softcore) rigid spheres interacting…

A model of low-temperature polar liquids is constructed that accounts for configurational heat capacity, entropy, and the effect of a strong electric field on the glass transition. The model is based on Pad{\'e}-truncated perturbation…

Soft Condensed Matter · Physics 2016-08-03 D. V. Matyushov

We obtain evidence that the dynamics of glassy systems below the glass transition is characterized by self-organized criticality. Using molecular dynamics simulations of a model glass-former we identify clusters of cooperatively jumping…

Disordered Systems and Neural Networks · Physics 2015-06-25 Katharina Vollmayr-Lee , Elizabeth A. Baker

The configurational entropy is among the key observables to characterize experimentally the formation of a glass. Physically, it quantifies the multiplicity of metastable states in which an amorphous material can be found at a given…

Statistical Mechanics · Physics 2014-08-21 Ludovic Berthier , Daniele Coslovich

The breakdown of the time-temperature superposition (TTS) near its glass transition temperature (Tg) in simple bead-spring polymer melts with and without the chain angle potential was numerically investigated. The stress relaxation modulus…

Soft Condensed Matter · Physics 2014-10-07 Tamio Yamazaki

It is presented a theory that describes a spin glass phase at finite temperatures in Kondo lattice systems with an additional RKKY interaction represented by long range, random couplings among localized spins like in the Sherrington-…

Statistical Mechanics · Physics 2009-10-31 Alba Theumann , B. Coqblin , S. G. Magalhaes , A. A. Schmidt

We show that a fluid under strong spatially periodic confinement displays a glass transition within mode-coupling theory (MCT) at a much lower density than the corresponding bulk system. We use fluctuating hydrodynamics, with confinement…

Soft Condensed Matter · Physics 2013-03-14 Saroj Kumar Nandi , Sarika Maitra Bhattacharyya , Sriram Ramaswamy

We have studied the low-frequency dynamics of the charge carriers in different organic charge-transfer salts $\kappa$-(BEDT-TTF)$_2$X with polymeric anions X by using resistance noise spectroscopy. Our aim is to investigate the structural,…

Strongly Correlated Electrons · Physics 2015-09-30 J. Müller , B. Hartmann , R. Rommel , J. Brandenburg , S. M. Winter , J. A. Schlueter

We introduce a new quantity to probe the glass transition. This quantity is a linear generalized compressibility which depends solely on the positions of the particles. We have performed a molecular dynamics simulation on a glass forming…

Disordered Systems and Neural Networks · Physics 2009-11-07 Herve M. Carruzzo , Clare C. Yu

There is a growing belief that the mode coupling theory is the proper microscopic theory for the dynamics of the undercooled liquid above a critical temperature T_c. In addition, there is some evidence that the system leaves the…

Disordered Systems and Neural Networks · Physics 2009-11-07 U. Buchenau
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