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Thermal relaxation of nanoscale magnetic islands, mimicking Ising macrospins, is indispensable for studies of geometrically frustrated artificial spin systems and low-energy nanomagnetic computation. Currently-used heating schemes based on…
Highly nonlinear optical processes, such as multiphoton photoemission, require high intensities, typically achieved with ultrashort laser pulses and, hence, were first observed with the advent of picosecond laser technology. An alternative…
It has recently been shown that holographically nanostructured surfaces can be employed to control the wavefront of (predominantly plasmonic) optical-frequency light emission generated by the injection of medium-energy electrons into a gold…
We present a novel procedure for manipulating the near-field of plasmonic nanoantennas using neural network-controlled laser pulse-shaping. As model systems we numerically studied the spatial distribution of the second harmonic response of…
Nanoparticle surface structural dynamics is believed to play a significant role in regulating functionalities such as diffusion, reactivity, and catalysis but the atomic-level processes are not well understood. Atomic resolution…
Nanostructured plasmonic metal systems are known to enhance greatly variety of radiative and nonradiative optical processes, both linear and nonlinear, which are due to the interaction of an electron in a molecule or semiconductor with the…
We describe a strategy for conversion of optical power into DC electrical power using resonant absorption in plasmonic nanostructures. A thermodynamic analysis of the underlying mechanism motivates our description of the phenomenon, which…
The observation and electrical manipulation of infrared surface plasmons in graphene have triggered a search for similar photonic capabilities in other atomically thin materials that enable electrical modulation of light at visible and…
Light emission of europium (Eu3+) ions placed in the vicinity of optically resonant nanoantennas is usually controlled by tailoring the local density of photon states (LDOS). We show that the polarization and shape of the excitation beam…
We analyse recently measured nonlinear photoemission spectra from Ag surfaces that reveal resonances whose energies do not scale with the applied photon energy but stay pinned to multiples of bulk plasmon energy $\hbar\omega_p$ above the…
Controlling quantum light-matter interactions at scales smaller than the diffraction limit at the single quantum emitter level is a critical challenge to the goal of advancing quantum technologies. We introduce a novel material platform…
Optical metasurfaces composed of metallic or dielectric scatterers (meta-atoms) promise a powerful way of tailoring light-matter interactions. Phase-change materials (PCMs) are prime candidates for non-volatile resonance tuning of…
Recently in nanophotonics, a rigorous evolution from passive to active metasurfaces has been witnessed. This advancement not only brings forward interesting physical phenomena but also elicits opportunities for practical applications.…
We study the plasmonic properties of arrays of atomic chains which comprise noble (Cu, Ag, and Au) and transition (Pd, Pt) metal atoms using time-dependent density-functional theory. We show that the response to the electromagnetic…
Alloy nanocatalysts have found broad applications ranging from fuel cells to catalytic converters and hydrogenation reactions. Despite extensive studies, identifying the active sites of nanocatalysts remains a major challenge due to the…
Metasurfaces enable manipulation of light propagation at an unprecedented level, benefitting from a number of merits unavailable to conventional optical elements, such as ultracompactness, precise phase and polarization control at deep…
Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…
Multiexcitonic transitions and emission of several photons per excitation comprise a very attractive feature of semiconductor quantum dots for optoelectronics applications. However, these higher-order radiative processes are usually…
Physical mechanisms of electron emission from fibre optic nanotips, namely, tunnelling, multi-photon, and thermionic emission, either prevent fast switching or require intense laser fields. Time-resolved electron emission from nano-sized…
We propose a method that enables strong, coherent coupling between individual optical emitters and electromagnetic excitations in conducting nano-structures. The excitations are optical plasmons that can be localized to sub-wavelength…