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In most single-photon defect emitters, such as those in SiC and diamond, interaction with low-energy acoustic phonons determines the temperature dependence of the decoherence rate and the resulting broadening of the ZPL with the temperature…

Materials Science · Physics 2023-10-09 Yifei Geng , Jialun Luo , Len van Deurzen , Huili , Xing , Debdeep Jena , Gregory David Fuchs , Farhan Rana

The anharmonic lattice dynamics of rock-salt thermoelectric compounds SnTe and PbTe are investigated with inelastic neutron scattering (INS) and first-principles calculations. The experiments show that, surprisingly, although SnTe is closer…

Materials Science · Physics 2015-06-18 C. W. Li , O. Hellman , J. Ma , A. F. May , H. B. Cao , X. Chen , A. D. Christianson , G. Ehlers , D. J. Singh , B. C. Sales , O. Delaire

We report the first experiments on the high pressure phonon spectra of transition-metal nitrides HfN, ZrN, and NbN, obtained by Raman scattering measurements. Two pronounced bands, which are related to the acoustic part at low frequency…

$\beta-Ga_2O_3$ is a promising material candidate for next-generation high power devices even as its low thermal conductivity ($\kappa$) limits utilization due to an inability to sufficiently dissipate heat. Despite its importance, a…

Materials Science · Physics 2024-10-16 Abdulaziz Alkandari , Zherui Han , Ziqi Guo , Thomas Beechem , Xiulin Ruan

We study the role of anharmonicity at interfaces with an added intermediate layer designed to facilitate interfacial phonon transport. Our results demonstrate that while in the harmonic limit the bridge may lower the conductance due to…

Temperature-dependent FAR-infrared reflectivity spectra of partially ordered magnetodielectric La2CoMnO6 is presented, from room temperature up to 675 K. A clear first-ordered structural phase transition (SPT) from a monoclinic structure…

Materials Science · Physics 2018-02-22 R. X. Silva , A. Nonato , R. L. Moreira , R. M. Almeida , C. W. A. Paschoal

We present a first-principles study of the temperature- and density-dependent intrinsic electrical resistivity of graphene. We use density-functional theory and density-functional perturbation theory together with very accurate Wannier…

Contradictory experiments have been reported about the dimensionality effect on the charge-density-wave transition in 2H NbSe$_2$. While scanning tunnelling experiments on single layers grown by molecular beam epitaxy measure a…

Mesoscale and Nanoscale Physics · Physics 2020-09-02 Raffaello Bianco , Lorenzo Monacelli , Matteo Calandra , Francesco Mauri , Ion Errea

We employ polarization-resolved Raman spectroscopy to study the lattice dynamics of the polar charge density wave phase of the superconductor Mo$_3$Al$_2$C with structural chirality. We show the phononic signatures of the charge density…

Superconductivity · Physics 2025-06-12 Shangfei Wu , Xianghan Xu , Fei-Ting Huang , Turan Birol , Sang-Wook Cheong , Girsh Blumberg

Recent theory has predicted large temperature differences between the in-plane (LA and TA) and out-of-plane (ZA) acoustic phonon baths in locally-heated suspended graphene. To verify these predictions, and their implications for…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Robin J. Dolleman , Gerard J. Verbiest , Yaroslav M. Blanter , Herre S. J. van der Zant , Peter G. Steeneken

The features of phonon spectra and their effect on the vibrational heat capacity of linear chains of inert gas atoms adsorbed onto a substrate, which is the surface of nanotubes bound to a nanobundle. The influence of the substrate results…

Mesoscale and Nanoscale Physics · Physics 2025-06-26 E. V. Manzhelii , S. B. Feodosyev , I. A. Gospodarev

The detailed optical properties of BaFe2As2 have been determined over a wide frequency range above and below the structural and magnetic transition at T_N = 138 K. A prominent in-plane infrared-active mode is observed at 253 cm^{-1} (31.4…

Strongly Correlated Electrons · Physics 2009-11-20 A. Akrap , J. J. Tu , L. J. Li , G. H. Cao , X. A. Xu , C. C. Homes

The understanding and modeling of inelastic scattering of thermal phonons at a solid/solid interface remain an open question. We present a fully quantum theoretical scheme to quantify the effect of anharmonic phonon-phonon scattering at an…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 Yangyu Guo , Zhongwei Zhang , Marc Bescond , Shiyun Xiong , Masahiro Nomura , Sebastian Volz

We report on polarized infrared reflectivity measurements of multiferroic, monoclinic MnWO4 between 10K and 295K. The full dielectric tensor and the frequency dependence of the orientation of the principal axes have been determined in the…

Strongly Correlated Electrons · Physics 2014-10-08 T. Möller , P. Becker , L. Bohaty , J. Hemberger , M. Grüninger

We report on the temperature dependence of the anharmonic decay rate of zone-center (G mode) optical phonons in both single-walled carbon nanotubes and graphite. The measurements are performed using a pump-probe Raman scattering scheme with…

Materials Science · Physics 2011-06-09 Ioannis Chatzakis , Hugen Yan , Daohua Song , Stéphane Berciaud , Tony F. Heinz

We develop a theoretical framework for probing moir\'e phonon modes using Raman spectroscopy, and illustrate it with the example of twisted bilayer graphene (TBG). These moir\'e phonons arise from interlayer sliding motion in twisted 2D…

Strongly Correlated Electrons · Physics 2025-06-24 Vitor Dantas , Héctor Ochoa , Rafael M. Fernandes , Natalia B. Perkins

The effect of electron-phonon scattering processes over the thermoelectric properties of extrinsic graphene was studied. Electrical and thermal resistivity, as well as the thermopower, were calculated within the Bloch theory approximations.…

Mesoscale and Nanoscale Physics · Physics 2012-08-02 Enrique Muñoz

We have observed the characteristic temperature dependence of the intermolecular phonon spectrum in the organic dimer Mott insulator kappa-(ET)2Cu2(CN)3 exhibiting a dielectric anomaly at 30 K. The anomalous spectral narrowing of the 55…

Strongly Correlated Electrons · Physics 2015-06-16 K. Itoh , H. Itoh , S. Saito , I. Hosako , Y. Nakamura , H. Kishida , N. Yoneyama , T. Sasaki , S. Ishihara , S. Iwai

We use first-principles density-functional calculations to determine the frequency shift of the A$'_1$-${\bf K}$ phonon (Raman D band) in monolayer graphene, as a function of the charge doping. A detailed DFT study on the electron-phonon…

Materials Science · Physics 2007-05-23 Srijan Kumar Saha , U. V. Waghmare , H. R. Krishnamurthy , A. K. Sood

We investigate three dimensional anharmonic phonons in tetrahedral symmetry and superconductivity mediated by these phonons. Three dimensional anharmonic phonon spectra are calculated directly by solving Schr\"odinger equation and the…

Superconductivity · Physics 2015-05-18 Kazumasa Hattori , Hirokazu Tsunetsugu
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