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In this article we present an algorithm to efficiently evaluate the exchange matrix in periodic systems when Gaussian basis set with pseudopotentials are used. The usual algorithm for evaluating exchange matrix scales cubically with the…

Strongly Correlated Electrons · Physics 2022-11-11 Sandeep Sharma , Alec F. White , Gregory Beylkin

The inverse Kohn-Sham density-functional theory (inv-KS) for the electron density of the Hartree-Fock (HF) wave function was revisited within the context of the optimized effective potential (HF- OEP). First, it is proved that the exchange…

Chemical Physics · Physics 2024-03-05 Hideaki Takahashi

We devise an efficient practical method for computing the Kohn-Sham exchange-correlation potential corresponding to a Hartree-Fock electron density. This potential is almost indistinguishable from the exact-exchange optimized effective…

Chemical Physics · Physics 2013-07-09 Ilya G. Ryabinkin , Alexei A. Kananenka , Viktor N. Staroverov

Scaling deep neural network (DNN) training to more devices can reduce time-to-solution. However, it is impractical for users with limited computing resources. FOSI, as a hybrid order optimizer, converges faster than conventional optimizers…

Machine Learning · Computer Science 2025-08-05 Shunxian Gu , Chaoqun You , Bangbang Ren , Lailong Luo , Junxu Xia , Deke Guo

In this paper, an efficient divide-and-conquer (DC) algorithm is proposed for the symmetric tridiagonal matrices based on ScaLAPACK and the hierarchically semiseparable (HSS) matrices. HSS is an important type of rank-structured…

Mathematical Software · Computer Science 2016-12-27 Shengguo Li , Francois-Henry Rouet , Jie Liu , Chun Huang , Xingyu Gao , Xuebin Chi

Exchange interactions are a manifestation of the quantum mechanical nature of the electrons and play a key role in predicting the properties of materials from first principles. In density functional theory (DFT), a widely used approximation…

Materials Science · Physics 2020-03-27 Marco Bernardi

In the present work, a high order finite element type residual distribution scheme is designed in the framework of multidimensional compressible Euler equations of gas dynamics. The strengths of the proposed approximation rely on the…

Numerical Analysis · Mathematics 2023-01-16 Remi Abgrall , Paola Bacigaluppi , Tokareva Svetlana

We report the results of intensive numerical calculations for four atomic H2+H2 energy transfer collision. A parallel computing technique based on LAM/MPI functions is used. In this algorithm, the data is distributed to the processors…

Chemical Physics · Physics 2007-05-23 Renat A. Sultanov , Mark Nordby , Dennis Guster

We introduce a data distribution scheme for $\mathcal{H}$-matrices and a distributed-memory algorithm for $\mathcal{H}$-matrix-vector multiplication. Our data distribution scheme avoids an expensive $\Omega(P^2)$ scheduling procedure used…

Numerical Analysis · Mathematics 2020-09-23 Yingzhou Li , Jack Poulson , Lexing Ying

The Interstellar Boundary Explorer (IBEX) has been measuring fluxes of the Energetic Neutral Atoms (ENAs) using the IBEX-Hi (0.3 -- 6 keV) instrument since 2008. We have developed a numerical time-depended code to calculate globally…

Space Physics · Physics 2020-10-01 I. I. Baliukin , V. V. Izmodenov , D. B. Alexashov

With the widespread use of self-consistent field methods, including Hartree-Fock and Density Functional Theory, the implications of accelerating these methods are immense. To this end, we develop a tensor hypercontraction construction with…

Chemical Physics · Physics 2025-08-27 Andreas Erbs Hillers-Bendtsen , Todd J. Martínez

Recent theoretical work has provided evidence that hybrid functionals, which include a fraction of exact (Hartree Fock) exchange in the density functional theory (DFT) exchange and correlation terms, significantly improve the description of…

Materials Science · Physics 2015-05-13 Xifan Wu , Eric J. Walter , Andrew M. Rappe , Roberto Car , Annabella Selloni

We present an accurate, efficient and massively parallel finite-element code, DFT-FE, for large-scale ab-initio calculations (reaching $\sim 100,000$ electrons) using Kohn-Sham density functional theory (DFT). DFT-FE is based on a local…

Computational Physics · Physics 2020-01-08 Phani Motamarri , Sambit Das , Shiva Rudraraju , Krishnendu Ghosh , Denis Davydov , Vikram Gavini

This paper considers the dynamic economic dispatch problem for a group of distributed energy resources (DERs) with storage that communicate over a weight-balanced strongly connected digraph. The objective is to collectively meet a certain…

Optimization and Control · Mathematics 2016-05-04 Ashish Cherukuri , Jorge Cortes

This paper investigates the system achievable rate and optimization for the multiple-input multiple-output (MIMO)-orthogonal frequency division multiplexing (OFDM) system with an energy harvesting (EH) relay. Firstly we propose a time…

Information Theory · Computer Science 2015-01-06 Guanyao Du , Zhilong Dong , Ke Xiong , Zhengding Qiu

We present an implementation of the multiconfiguration time-dependent Hartree-Fock method based on the adaptive finite element method for molecules under intense laser pulses. For efficient simulations, orbital functions are propagated by a…

Quantum Physics · Physics 2023-01-09 Yuki Orimo , Takeshi Sato , Kenichi L. Ishikawa

We present a distributed-memory library for computations with dense structured matrices. A matrix is considered structured if its off-diagonal blocks can be approximated by a rank-deficient matrix with low numerical rank. Here, we use…

Mathematical Software · Computer Science 2015-06-29 François-Henry Rouet , Xiaoye S. Li , Pieter Ghysels , Artem Napov

High performance computing (HPC) is a powerful tool to accelerate the Kohn-Sham density functional theory (KS-DFT) calculations on modern heterogeneous supercomputers. Here, we describe a massively extreme-scale parallel and portable…

Computational Physics · Physics 2020-04-20 Wei Hu , Xinming Qin , Caiqing Jiang , Junshi Chen , Hong An , Weile Jia , Fang Li , Xin Liu , Dexun Chen , Jinlong Yang

A two-parameter extension of the density-scaled double hybrid approach of Sharkas et al. [J. Chem. Phys. 134, 064113 (2011)] is presented. It is based on the explicit treatment of a fraction of multideterminantal exact exchange. The…

Chemical Physics · Physics 2012-01-12 Emmanuel Fromager

Noncollinear (NC) magnetism and spin-orbit coupling (SOC) are indispensable for predictive ab initio materials simulations with pronounced relativistic effects and magnetic frustration, yet they significantly increase the cost of…