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Optical polaritons appear when a material excitation strongly couples to the optical mode. Such strong coupling between molecular transitions and optical cavities results in far-reaching opportunities in modifying fundamental properties of…

Mirror symmetry is among the most fundamental concepts of physics and its spontaneous breaking at the molecular level allows chiral molecules to exist in two enantiomers that are mirror images of each other. The majority of chiro-optical…

Optics · Physics 2021-09-29 Alessandro Ciattoni

Chiroptical effects, characterized by different optical responses for left- (LCP) and right- handed circularly polarized light (RCP), are powerful and valuable tools in optics with wide applications in polarization resolved imaging and…

Optics · Physics 2018-05-02 Weimin Ye , Xiaodong Yuan , Chucai Guo , Jianfa Zhang , Biao Yang , Shuang Zhang

Strongly coupled plasmon-exciton systems offer promising applications in nanooptics. The classification of the coupling regime is currently debated both from experimental and theoretical perspectives. We present a method to unambiguously…

Mesoscale and Nanoscale Physics · Physics 2023-07-19 Felix Stete , Wouter Koopman , Matias Bargheer

We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling…

Mesoscale and Nanoscale Physics · Physics 2012-08-17 Adi Salomon , Robert J. Gordon , Yehiam Prior , Tamar Seideman , Maxim Sukharev

Quantum emitters near the surface of silver nanoparticles undergo Rabi oscillations in electronic population dynamics due to strong coupling with near-field multipole modes that are not radiative. Low-frequency nanoparticle dipole modes are…

Quantum Physics · Physics 2026-03-19 Athul S. Rema , Adrián E. Rubio López , Felipe Herrera

Recent activity in the area of chiroptical phenomena has been focused on the connection between structural asymmetry, electron spin configuration and light matter interactions in chiral semiconductors. In these systems, spin-splitting…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 Peter C. Sercel , Matthew P. Hautzinger , Ruyi Song , Volker Blum , Matthew C. Beard

The optical responses of structured array of noble-metal nanoparticle dimers immersed in a glass matrix are investigated theoretically, motivated by the recent experimental observation of the splitting of the surface plasmon bands in silver…

Optics · Physics 2007-05-23 J. J. Xiao , J. P. Huang , K. W. Yu

Chiral excited electronic states of molecules have an intrinsic sense of handedness, or twist, and are the active component in energy efficient display technologies and in new photosynthetic routes to produce pharmaceuticals. Creating…

We present a comprehensive review of recent developments in the field of chiral plasmonics. Significant advances have been made recently in understanding the working principles of chiral plasmonic structures. With advances in micro- and…

We investigate theoretically the effects of interaction between an optical dipole (semiconductor quantum dot or molecule) and metal nanoparticles. The calculated absorption spectra of hybrid structures demonstrate strong effects of…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Jie-Yun Yan , Wei Zhang , Suqing Duan , Xian-Geng Zhao , Alexander O. Govorov

Van der Waals heterostructures of atomically thin layers with rotational misalignments, such as twisted bilayer graphene, feature interesting structural moir\'e superlattices. Due to the quantum coupling between the twisted atomic layers,…

Peculiar ring gap modes on the surface of disk close to the metallic thin film are excited in the visible light regime. We apply plasmon hybridization method to illustrate the ring gap modes arising from the interaction between localized…

Optics · Physics 2021-02-02 Guodong Zhu , Linhong Qv , Yangzhe Guo , Yurui Fang

Chiral response is of tremendous importance to many fields, such as analytical chemistry, polarization manipulation and biological sensing. Here, a chiral metasurface based on rectangular holes is systematically investigated. The results…

Optics · Physics 2021-12-07 Biyuan Wu , Mingjun Wang , Yasong Sun , Feng Wu , Zhangxing Shi , Xiaohu Wu

Strong coupling typically occurs between two separate objects or between an object and its environment (such as an atom and a cavity). However, it can also occur between two different excitations within the same object, a situation that has…

Light scattering from chiral plasmonic structures can create near fields with an asymmetry greater than the equivalent circularly polarised light, a property sometimes referred to as superchirality. These near fields with enhanced chiral…

From the high vibrational dipolar strength offered by molecular liquids, we demonstrate that a molecular vibration can be ultra-strongly coupled to multiple IR cavity modes, with Rabi splittings reaching $24\%$ of the vibration frequencies.…

Localized plasmonic modes of metallic nanoparticles may hybridize like those of atoms forming a molecule. However, the rapid decay of the plasmonic fields outside the metal severely limits the range of these interactions to tens of…

Optics · Physics 2013-03-05 Adi Salomon , Yehiam Prior , Radoslaw Kolkowski , Joseph Zyss

It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…

Optics · Physics 2020-04-14 David Ayuso , Andres Ordonez , Piero Decleva , Misha Ivanov , Olga Smirnova

The strong coupling between two subsystems consisting of quantum emitters and photonic modes, at which the level splitting of mixed quantum states occurs, has been a central subject of quantum physics and nanophotonics due to various…

Optics · Physics 2021-06-30 Renming Liu , Yi-Cong Yu , Xue-Hua Wang
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