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We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…

Atomic Physics · Physics 2015-06-19 Bin Zhang , Jianmin Yuan , Zengxiu Zhao

Considerable progress has been made in organic light-emitting diodes (OLEDs) to achieve high external quantum efficiency (EQE), among which the dipole orientation of OLED emitters has a remarkable effect. In most cases, EQE of the OLED…

Phase-of-the-phase spectroscopy using two-color colinearly polarized laser pulses has been introduced and experimentally applied to strong-field tunneling ionization in S. Skruszewicz et al., Phys. Rev. Lett. 115, 043001 (2015) and recently…

Atomic Physics · Physics 2018-12-05 V. Tulsky , M. A. Almajid , D. Bauer

We consider the final stage of multiple ionization of atoms in a strong linearly polarized laser field within a classical model. We propose that non-sequential multiple ionization is dominated by symmetric escape from a highly excited…

Atomic Physics · Physics 2007-05-23 Krzysztof Sacha , Bruno Eckhardt

The total photodetachment cross section of a linear triatomic negative ion using plane polarized laser light parallel to the axis of the molecular ion is derived. The cross section shows strong oscillations in contrast to the recently…

Atomic Physics · Physics 2010-01-26 A. Afaq , Iftikhar Ahmad

The transition between two distinct mechanisms for the laser-induced field-free orientation of CO molecules is observed via measurements of orientation revival times and subsequent comparison to theoretical calculations. In the first…

Fully relativistic approach to evaluate the correlation effects in highly charged ions is presented. The interelectronic-interaction contributions of first and second orders in $1/Z$ are treated rigorously within the framework of…

Atomic Physics · Physics 2019-12-18 Y. S. Kozhedub , A. V. Malyshev , D. A. Glazov , V. M. Shabaev , I. I. Tupitsyn

We extend the recently-developed theory of bulk orbital magnetization to finite electric fields, and use it to calculate the orbital magnetoelectric response of periodic insulators. Working in the independent-particle framework, we find…

Mesoscale and Nanoscale Physics · Physics 2010-05-28 Andrei Malashevich , Ivo Souza , Sinisa Coh , David Vanderbilt

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

We present a simple and general coherence model for multiorbital tunnel ionization of molecules, which we incorporate into our previously developed density matrix approach for sequential double ionization [Yuen and Lin, Phys. Rev. A 106,…

Atomic Physics · Physics 2023-09-07 C. H. Yuen , C. D. Lin

For a given many-electron molecule, it is possible to define a corresponding one-electron Schr\"odinger equation, using potentials derived from simple atomic densities, whose solution predicts fairly accurate molecular orbitals for single-…

Chemical Physics · Physics 2022-05-16 Fariba Nazari , Jerry L. Whitten

Formal expressions are derived for the multipole expansion of the structure functions of a general polarization observable of exclusive electrodisintegration of the deuteron using a longitudinally polarized beam and/or an oriented target.…

Nuclear Theory · Physics 2007-05-23 Hartmuth Arenhoevel , Winfried Leidemann , Edward L. Tomusiak

We consider emission of a photon by an electron in the field of a strong laser wave. A probability of this process for circularly or linearly polarized laser photons and for arbitrary polarization of all other particles is calculated. We…

High Energy Physics - Phenomenology · Physics 2007-05-23 D. Yu. Ivanov , G. L. Kotkin , V. G. Serbo

We have experimentally and theoretically investigated the mixed-field orientation of rotational-state-selected OCS molecules and we achieve strong degrees of alignment and orientation. The applied moderately intense nanosecond laser pulses…

Electron-electron correlation effects play an instrumental role in our understanding of sequential (SDI) and non-sequential double ionization (NSDI) mechanisms. Here, we present a theoretical study of NSDI driven by plasmonic-enhanced…

In this work we propose a novel composite method for accurate calculation of the energies of many-electron atoms. The dominant contribution to the energy (pair energies) are calculated by using explicitly correlated factorisable coupled…

Atomic Physics · Physics 2018-12-12 Michal Przybytek , Michal Lesiuk

We investigate the discrete orbital angular momentum (OAM) of photoelectrons freed in strongfield ionization. We use these `twisted' electrons to provide an alternative interpretation on existing experimental work of vortex interferences…

Using perturbed relativistic coupled-cluster (PRCC) theory we compute the ground state electric dipole polarizability, $\alpha$, of doubly ionized alkaline earth metal ions $\rm{Mg}^{2+}$, $\rm{Ca}^{2+}$, $\rm{Sr}^{2+}$, $\rm{Ba}^{2+}$ and…

Atomic Physics · Physics 2013-06-14 S. Chattopadhyay , B. K. Mani , D. Angom

The Schr\"odinger equation is solved for the wave function of an electron moving in a superposition of external constant and uniform electric and magnetic fields at an arbitrary angle between the field directions. The changing of the…

Quantum Physics · Physics 2017-02-10 S. O. Lebedynskyi , V. I. Miroshnichenko , R. I. Kholodov , V. A. Baturin

We present angular distributions of photoelectrons of atomic model systems excited by intense linearly polarized laser pulses in the VUV- and XUV-regime. We solve the multi-dimensional time-dependent Schr\"odinger equation for one particle…

Atomic Physics · Physics 2010-03-16 S. Bauch , M. Bonitz