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We investigate the orientation dependence of Enhanced Ionization (EI) during strong-field-driven nuclear motion in acetylene (C$_2$H$_2$). Here, we both initiate and probe molecular dynamics in acetylene with intense 6-fs cross-polarized…

Atomic Physics · Physics 2024-11-08 S. A. Mohideen , A. J. Howard , C. Cheng , I. Gabalski , A. M. Ghrist , E. Weckwerth , P. H. Bucksbaum

The ionization dynamics of a two-electron atom in an attosecond XUV-infrared pump-probe experiment is simulated by solving the time-dependent two-electron Schr\"odinger equation. A dramatic change of the double ionization (DI) yield with…

Atomic Physics · Physics 2010-11-29 S. Bauch , K. Balzer , M. Bonitz

We explore the possibility of forming a oriented polar molecule directly from a pair of colliding atoms. The process comprises the photoassociation and vibrational stabilization along with the molecular orientation. These processes are…

Quantum Physics · Physics 2026-01-14 Murilo D. Forlevesi , Edson Denis Leonel , Emanuel F. de Lima

The screened electron-electron interaction in a multi-band electron system is calculated within the random phase approximation and in the tight-binding representation. The obtained dielectric matrix contains, beside the usual site-site…

Condensed Matter · Physics 2009-10-28 P. Zupanovic , A. Bjelis , S. Barisic

We investigate the strong-field ionization of atomic hydrogen in a few-cycle elliptically polarized infrared pulse by solving the time-dependent Schr\"odinger equation. The dependence of the photoelectron momentum distribution on the pulse…

Atomic Physics · Physics 2022-11-30 Nicolas Douguet , Klaus Bartschat

We study the ionization dynamics of oriented HeH$^+$ in strong linearly-polarized laser fields by numerically solving the time-dependent Schr\"{o}dinger equation. The calculated photoelectron momentum distributions for parallel orientation…

Atomic Physics · Physics 2020-11-11 S. Wang , J. Y. Che , C. Chen , G. G. Xin , Y. J. Chen

We analyze, quantum mechanically, the dynamics of ionization with a strong, circularly polarized, laser field. We show that the main source for non-adiabatic effects is connected to an effective barrier lowering due to the laser frequency.…

Atomic Physics · Physics 2014-09-26 Francois Mauger , A. D. Bandrauk

We experimentally demonstrated strong adiabatic mixed-field orientation of carbonyl sulfide molecules (OCS) in their absolute ground state of $\text{N}_{\text{up}}/\text{N}_{\text{tot}}=0.882$. OCS was oriented in combined non-resonant…

Deep understanding of photon polarization impact on pair production is essential for the efficient creation of laser driven polarized positron beams, and demands a complete description of polarization effects in strong-field QED processes.…

We perform time-dependent calculations of strong-field ionization of He by elliptically polarized light in configuration of recent attoclock measurements of Boge {\em et al} [PRL {\bf 111}, 103003 (2013)]. By solving a 3D time-dependent…

Atomic Physics · Physics 2026-03-03 I. A. Ivanov , A. S. Kheifets

The exact quantum time-dependent optical response of hydrogen under strong field near infrared excitation is investigated and compared to the perturbative model widely used for describing the effective atomic polarization induced by intense…

Formulas for the contribution of the conduction electrons to the polarization and magnetization are derived for disordered systems and within a one-particle framework. These results generalize known formulas for Bloch electrons and the…

Mathematical Physics · Physics 2014-01-10 Hermann Schulz-Baldes , Stefan Teufel

We present a combined experimental and theoretical study on strong-field ionization of a three-dimensionally oriented asymmetric top molecule, benzonitrile (C$_7$H$_5$N), by circularly polarized, nonresonant femtosecond laser pulses. Prior…

We give examples showing that two well-known versions of the S-matrix theory, which describes a nonresonant multiphoton ionization of atoms and ions in intense laser fields, lead to qualitatively different results. The latter refer not only…

Atomic Physics · Physics 2015-05-28 J. H. Bauer

We present a wave-function based method to solve the time-dependent many-electron Schr\"odinger equation (TDSE) with special emphasis on strong-field ionization phenomena. The theory builds on the configuration-interaction (CI) approach…

Quantum Physics · Physics 2014-12-11 Sebastian Bauch , Lasse Kragh Sørensen , Lars Bojer Madsen

We present an ab initio approach to solve the time-dependent Schr\"odinger equation to treat electron and photon impact multiple ionization of atoms or molecules. It combines the already known time scaled coordinate method with a new high…

Electrons colliding with spatially fixed ions in strong laser fields are investigated by solving the time-dependent Schr\"odinger equation. Considering first simple one-dimensional model systems, the mechanisms and energy spectra of fast…

Atomic Physics · Physics 2015-10-28 S. Bauch , M. Bonitz

Under quite generic assumptions the general expression is derived for the probability of circularly polarized photon emission from the longitudinally polarized electron and for the probability of pair creation of longitudinally polarized…

High Energy Physics - Phenomenology · Physics 2007-05-23 V. N. Baier , V. M. Katkov

Multivalent ions in solutions with polyelectrolytes (PE) induce electrostatic correlations that can drastically change ion distributions around the PEs and their mutual interactions. Using coarse-grained molecular dynamics simulations, we…

Soft Condensed Matter · Physics 2023-04-26 Hossein Vahid , Alberto Scacchi , Maria Sammalkorpi , Tapio Ala-Nissila

We study the ellipticity of high-order harmonics emitted from CO$_2$ molecule driven by linearly polarized laser fields using numerical simulations within the time-dependent density functional theory. We find that the overall ellipticity of…

Atomic and Molecular Clusters · Physics 2024-09-17 Andres Mora , Lauren Bauerle , Yuqing Xia , Agnieszka Jaron