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One challenge of using nonlinear optical phenomena for practical applications is the need to perform phase-matching. Recently, epsilon-near-zero materials have been shown to demonstrate strong optical nonlinearities, in addition to their…

Optics · Physics 2024-07-30 Kyle Wynne , Marjan Bazian , Mark C. Harrison

We combine modeling and experiments to investigate second- and third-harmonic generation (SHG/THG) in metal-indium tin oxide (ITO) metasurfaces. Linear optics at normal incidence show moderate field enhancement near the ITO…

We investigate, theoretically and numerically, the dependence of a material's nonlinear-optical response on the linear relative electric permittivity $\epsilon$ and magnetic permeability $\mu$. The conversion efficiency of low-order…

Optics · Physics 2025-09-24 Diego M. Solís , Robert W. Boyd , Nader Engheta

Light in the mid-infrared (mid-IR) spans wavelengths from 3-8 $\mu$m and is important to many applications such as gas sensing and thermal imaging. Due to materials challenges, there is currently a lack of mid-IR reconfigurable optical…

The transparent and conductive properties of indium tin oxide (ITO) thin films, make them an attractive coating for optically integrated ion traps. However, the relatively low transmittance for wavelengths $<$ 400 nm, high scattering and…

Tunable optical material properties enable novel applications in both versatile metamaterials and photonic components including optical sources and modulators. Transparent conductive oxides (TCOs) are able to highly tune their optical…

Similar to radiation pressure, photothermal effects connect the optical path length to an intracavity field, resulting in nonlinear behavior of the resonator due to thermal effects. Here, we theoretically investigate the nonlinear optics…

Optics · Physics 2023-03-07 Akhtar Munir

Low electron density Drude (LEDD) materials such as indium tin oxide (ITO) are receiving considerable attention because of their combination of CMOS compatibility, unique epsilon-near-zero (ENZ) behavior, and giant ultrafast nonlinear…

Optics · Physics 2024-04-15 Ieng Wai Un , Subhajit Sarkar , Yonatan Sivan

Ultrathin plasmonic films that approach the trans-dimensional (TD) thickness limit provide a promising route for light_matter interaction control and manipulation, yet their nonlinear optical response near the epsilon_near_zero (ENZ)…

We show that the third order optical nonlinearity of 15-atom gold clusters is significantly enhanced when in contact with indium tin oxide (ITO) conducting film. Open and close aperture z-scan experiments together with non-degenerate…

Mesoscale and Nanoscale Physics · Physics 2013-04-02 Sunil Kumar , E. S. Shibu , T. Pradeep , A. K. Sood

Transparent conducting oxides (TCOs) play an essential role in modern optoelectronic devices through their combination of electrical conductivity and optical transparency. We review recent progress in our understanding of multi-component…

Materials Science · Physics 2013-09-18 Aron Walsh , Juarez L. F. Da Silva , Su-Huai Wei

For decades, nonlinear optics has been used to control the frequency and propagation of light in unique ways enabling a wide range of applications such as ultrafast lasing, sub-wavelength imaging, and novel sensing methods. Through this, a…

Optics · Physics 2020-04-02 Ray Secondo , Jacob B. Khurgin , Nathaniel Kinsey

Non-linear and bistable optical systems are a key enabling technology for the next generation optical networks and photonic neural systems with many potential applications in optical logic and information processing. Here, we propose a…

Optics · Physics 2022-09-20 J. Gosciniak , Z. Hu , M. Thomaschewski , V. Sorger , J. B. Khurgin

Controlling light polarization is one of the most essential routines in modern optical technology. Since the demonstration of optical pulse shaping by spatial light modulators and its potential in controlling the quantum reaction pathways,…

Experiments on Indium Tin Oxide (ITO) have revealed that a relatively broad 200THz pump pulse, roughly 30 cycles in width, can switch ITO from a transparent to a reflecting state within one or two optical cycles, a few Femtoseconds. So far…

Optics · Physics 2024-07-12 J. B. Pendry

Epsilon near zero (ENZ) materials can contribute significantly to the advancement of spectrally selective coatings aimed at enhancing efficient use of solar radiation and thermal energy management. Here, we demonstrate a subwavelength…

Optics · Physics 2024-02-13 Sraboni Dey , Kirandas P S , Deepshikha Jaiswal Nagar , Joy Mitra

Nonlinear optics experiments measuring phase shifts induced in a weak probe pulse by a strong pump pulse must account for coherent effects that only occur when the pump and probe pulses are temporally overlapped. It is well known that a…

An optically-induced thermal non-linear effect in a nematic liquid-crystal (E7) cell is evidenced through weak light-absorption by the ITO coating of an infrared pulsed femtosecond laser (m). Strong spatial self-phase modulation is…

This work describes the experimental and theoretical study of the nonlinear optical properties of the imidazolium cation based ionic liquids and the corresponding thermo-optical parameters. Experimental results of nonlinear optical…

Realizing remarkable tunability in optical properties without sacrificing speed is critical to obtain all optical ultrafast devices. In this work, we investigate the ultrafast temporal behavior of optically tunable epsilon-near-zero (ENZ)…