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Accurate molecular crystal structure prediction is a fundamental goal in academic and industrial condensed matter research and polymorphism is arguably the biggest obstacle on the way. We tackle this challenge in the difficult case of the…

Materials Science · Physics 2016-05-04 Cong Huy Pham , Emine Kucukbenli , Stefano de Gironcoli

Polymorphs in molecular crystals are often very close in energy, yet they may possess markedly different physical and chemical properties. The understanding and prediction of polymorphism is of paramount importance for a variety of…

We demonstrate a smart laser-diffraction analysis technique for particle mixture identification. We retrieve information about the size, geometry, and ratio concentration of two-component heterogeneous particle mixtures with an efficiency…

Image and Video Processing · Electrical Eng. & Systems 2022-02-03 Arturo Villegas , Mario A. Quiroz-Juarez , Alfred U'Ren , Juan P. Torres , Roberto de J. Leon-Montiel

This paper explores optimal methods for obtaining one-dimensional (1D) powder pattern intensities from two-dimensional (2D) planar detectors with good estimates of their standard deviations. We describe methods to estimate uncertainties…

Materials Science · Physics 2014-09-12 Xiaohao Yang , Pavol Juhas , Simon J. L. Billinge

We calculate the optical diffraction radiation generated by a bunch of high energy particles as they pass through a round hole within an annular metallic ring. We derive expressions for the differential angular spectrum in the far-field and…

Accelerator Physics · Physics 2008-08-29 Tanaji Sen

(short version) Accurate determination of the coherent static structure factor of disordered materials containing proton nuclei is prohibitively difficult by neutron diffraction, due to the large incoherent cross section of $^1$H. This…

Soft Condensed Matter · Physics 2021-01-28 László Temleitner , Anne Stunault , Gabriel Cuello , László Pusztai

Transmission electron diffraction is a powerful and versatile structural probe for the characterization of a broad range of materials, from nanocrystalline thin films to single crystals. With recent developments in fast electron detectors…

Materials Science · Physics 2021-10-06 Jian-Min Zuo , Renliang Yuan , Yu-Tsun Shao , Haw-Wen Hsiao , Saran Pidaparthy , Yang Hu , Qun Yang , Jiong Zhang

We describes a new approach for performing quantitative structure-factor analysis and density measurements of liquids using x-ray diffraction with a pink-spectrum x-ray source. The methodology corrects for the pink beam effect by performing…

The implementation and reliability of a quadratic diffusion Monte Carlo method for the study of ground-state properties of atoms are discussed. We show in the simple yet non-trivial calculation of the binding energy of the Li atom that the…

Condensed Matter · Physics 2009-11-07 A. Sarsa , J. Boronat , J. Casulleras

The diffusion path and diffusivity of oxygen in crystalline silicon are computed using an empirical interatomic potential which was recently developed for modelling the interactions between oxygen and silicon atoms. The diffusion path is…

mtrl-th · Physics 2008-02-03 Z. Jiang , R. A. Brown

Atoms and molecules can serve as sensitive probes of a possible variation of the fine structure constant $\alpha$ and electron-to-proton mass ratio $\mu$. Two types of sensitivity coefficients are often used to quantify and compare the…

Atomic Physics · Physics 2018-12-06 M. G. Kozlov , D. Budker

We present an analysis of atomic diffraction due to the interaction of an atomic beam with a pair of Gaussian light pulses. We derive a simple analytical expression for the populations in different diffraction orders. The validity of the…

Quantum Physics · Physics 2009-11-13 Tapio P. Simula , Atom Muradyan , Klaus Molmer

A single crystal of GdBaCo2O5.47(2) has been studied by means of X-ray diffraction. Appearance of superstructure reflections at T = 341.5(7) K gives an evidence of continuous transition to the phase with unit cell doubled along the shortest…

Materials Science · Physics 2009-11-10 Yu. P. Chernenkov , V. P. Plakhty , V. I. Fedorov , S. N. Barilo , S. V. Shiryaev , G. L. Bychkov

These tutorials introduce some basics of imaging with coherent X-rays, focusing on phase contrast. We consider the transport-of-intensity equation, as one particular method for X-ray phase contrast imaging among many, before passing on to…

Image and Video Processing · Electrical Eng. & Systems 2019-02-28 David M. Paganin , Daniele Pelliccia

Cross-spectral analysis is a mathematical tool for extracting the power spectral density of a correlated signal from two time series in the presence of uncorrelated interfering signals. We demonstrate and explain a set of conditions where…

Instrumentation and Detectors · Physics 2013-07-26 Craig W. Nelson , Archita Hati , David A. Howe

This article considers the computational (acoustic) wave propagation in strongly heterogeneous structures beyond the assumption of periodicity. A high contrast between the constituents of microstructured multiphase materials can lead to…

Numerical Analysis · Mathematics 2020-01-29 Daniel Peterseim , Barbara Verfürth

Here we show that the low temperature phase of magnetite is associated with an effective, although fractional, ordering of the charge. Evidence and a quantitative evaluation of the atomic charges are achieved by using resonant x-ray…

Strongly Correlated Electrons · Physics 2009-11-11 E. Nazarenko , J. E. Lorenzo , Y. Joly , J. L. Hodeau , D. Mannix , C. Marin

Classifying a crystalline solid's phase using X-ray diffraction (XRD) is a challenging endeavor, first because this is a poorly constrained problem as there are nearly limitless candidate phases to compare against a given experimental…

Applied Physics · Physics 2025-05-15 Kangyu Ji , Fang Sheng , Tianran Liu , Basita Das , Tonio Buonassisi

The surface diffusion potential landscape plays an essential role in a number of physical and chemical processes such as self-assembly and catalysis. Diffusion energy barriers can be calculated theoretically for simple systems, but there is…

Mesoscale and Nanoscale Physics · Physics 2019-05-28 Renan Villarreal , Christopher J. Kirkham , Alessandro Scarfato , David R. Bowler , Christoph Renner

The chiral structure of liquid crystalline phases arises due to the intrinsic chirality of the constituent mesogens. While it is seemingly straightforward to quantify the macroscopic chirality by using, for instance, the cholesteric pitch…

Soft Condensed Matter · Physics 2007-05-23 Randall D. Kamien