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Mapping an atomistic configuration to an $N$-point correlation of a field associated with the atomic positions (e.g. an atomic density) has emerged as an elegant and effective solution to represent structures as the input of…

Chemical Physics · Physics 2020-10-07 Jigyasa Nigam , Sergey Pozdnyakov , Michele Ceriotti

We introduce a fresh scheme based on the local hidden variable models to quantify nonlocality for arbitrarily high-dimensional quantum systems. Our scheme explores the minimal amount of white noise that must be added to the system in order…

Quantum Physics · Physics 2009-11-09 Dong-Ling Deng , Jing-Ling Chen , Zi-Sui Zhou

Utilising dynamic electromagnetic field control over charged particles serves as the basis for a quantum machine learning platform that operates on observables rather than directly on states. Such a platform can be physically realised in…

Quantum Physics · Physics 2024-06-12 Jesús Fuentes

Predicting and enhancing inherent properties based on molecular structures is paramount to design tasks in medicine, materials science, and environmental management. Most of the current machine learning and deep learning approaches have…

Machine Learning · Computer Science 2024-04-08 Zachary R. Fox , Ayana Ghosh

An important yet challenging aspect of atomistic materials modeling is reconciling experimental and computational results. Conventional approaches involve generating numerous configurations through molecular dynamics or Monte Carlo…

Materials Science · Physics 2024-12-23 Tigany Zarrouk , Rina Ibragimova , Albert P. Bartók , Miguel A. Caro

By adopting a perspective informed by contemporary liquid state theory, we consider how to train an artificial neural network potential to describe inhomogeneous, disordered systems. We find that neural network potentials based on local…

Chemical Physics · Physics 2021-11-10 Samuel P. Niblett , Mirza Galib , David T. Limmer

In machine learning energy potentials for atomic systems, forces are commonly obtained as the negative derivative of the energy function with respect to atomic positions. To quantify aleatoric uncertainty in the predicted energies, a widely…

Machine Learning · Statistics 2023-12-08 Peter Bjørn Jørgensen , Jonas Busk , Ole Winther , Mikkel N. Schmidt

Real-world applications of machine learning models are often subject to legal or policy-based regulations. Some of these regulations require ensuring the validity of the model, i.e., the approximation error being smaller than a threshold. A…

Machine Learning · Statistics 2024-06-18 Sven Lämmle , Can Bogoclu , Robert Voßhall , Anselm Haselhoff , Dirk Roos

The non-equilibrium response of a quantum many-body system defines its fundamental transport properties and how initially localized quantum information spreads. However, for long-range-interacting quantum systems little is known. We address…

Quantum Physics · Physics 2013-11-15 Philipp Hauke , Luca Tagliacozzo

Measurements are essential for the processing and protection of information in quantum computers. They can also induce long-range entanglement between unmeasured qubits. However, when post-measurement states depend on many non-deterministic…

Laser-driven rescattering of electrons is the basis of many strong-field phenomena in atoms and molecules. Here, we will show how this mechanism operates in extended atomic systems, giving rise to effective energy absorption. Rescattering…

Atomic and Molecular Clusters · Physics 2008-04-07 Ulf Saalmann , Jan M. Rost

We demonstrate how to construct a lorentz-invariant, hidden-variable interpretation of relativistic quantum mechanics based on particle trajectories. The covariant theory that we propose employs a multi-time formalism and a…

Quantum Physics · Physics 2009-11-07 George Horton , Chris Dewdney

Can a large system be fully characterized using its subsystems via inductive reasoning? Is it possible to completely reduce the behavior of a complex system to the behavior of its simplest "atoms"? In the following paper we answer these…

Quantum Physics · Physics 2018-11-19 Yakir Aharonov , Eliahu Cohen , Jeff Tollaksen

A common pipeline in learning-based control is to iteratively estimate a model of system dynamics, and apply a trajectory optimization algorithm - e.g.~$\mathtt{iLQR}$ - on the learned model to minimize a target cost. This paper conducts a…

Machine Learning · Computer Science 2023-05-17 Daniel Pfrommer , Max Simchowitz , Tyler Westenbroek , Nikolai Matni , Stephen Tu

A cardinal obstacle to understanding and predicting quantitatively the properties of solids and large molecules is that, for these systems, it is very challenging to describe beyond the mean-field level the quantum-mechanical interactions…

Strongly Correlated Electrons · Physics 2020-09-14 Nicola Lanatà

We study the problem of selecting covariates for unbiased estimation of the total causal effect.Existing approaches typically rely on global causal structure learning over all variables, or on strong assumptions such as causal sufficiency -…

Machine Learning · Statistics 2026-05-22 Zeyu Liu , Zheng Li , Feng Xie , Yan Zeng , Hao Zhang , Kun Zhang

Neural network force field (NNFF) is a method for performing regression on atomic structure-force relationships, bypassing expensive quantum mechanics calculation which prevents the execution of long ab-initio quality molecular dynamics…

Quantum many-body systems realise many different phases of matter characterised by their exotic emergent phenomena. While some simple versions of these properties can occur in systems of free fermions, their occurrence generally implies…

Strongly Correlated Electrons · Physics 2019-10-04 Samuel Spillard , Christopher J. Turner , Konstantinos Meichanetzidis

Encoding the electronic structure of molecules using 2-electron reduced density matrices (2RDMs) as opposed to many-body wave functions has been a decades-long quest as the 2RDM contains sufficient information to compute the exact molecular…

Chemical Physics · Physics 2022-08-11 David Pekker , Chungwen Liang , Sankha Pattanayak , Swagatam Mukhopadhyay

Data-based inference of directed interactions in complex dynamical systems is a problem common to many disciplines of science. In this work, we study networks of spatially separate dynamical entities, which could represent physical systems…

Statistical Mechanics · Physics 2024-03-15 Tim Hempel , Sarah A. M. Loos
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