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The giant exciton binding energy and the richness of degrees of freedom make monolayer transition metal dichalcogenide an unprecedented playground for exploring exciton physics in 2D systems. Thanks to the well energetically separated…

Mesoscale and Nanoscale Physics · Physics 2023-07-26 Bairen Zhu , Ke Xiao , Siyuan Yang , Kenji Watanabe , Takashi Taniguchi , Xiaodong Cui

Monolayer group VI transition metal dichalcogenides have recently emerged as semiconducting alternatives to graphene in which the true two-dimensionality (2D) is expected to illuminate new semiconducting physics. Here we investigate…

Mesoscale and Nanoscale Physics · Physics 2014-03-05 Jason S Ross , Sanfeng Wu , Hongyi Yu , Nirmal J Ghimire , Aaron M Jones , Grant Aivazian , Jiaqiang Yan , David G. Mandrus , Di Xiao , Wang Yao , Xiaodong Xu

We study spatial photoluminescence characteristics of neutral and charged excitons across extended monolayer MoS$_2$ synthesized by chemical vapor deposition. Using two-dimensional hyperspectral photoluminescence mapping at cryogenic…

Mesoscale and Nanoscale Physics · Physics 2019-02-20 Andre Neumann , Jessica Lindlau , Manuel Nutz , Aditya D. Mohite , Hisato Yamaguchi , Alexander Högele

The quest for platforms to generate and control exotic excitonic states has greatly benefited from the advent of transition metal dichalcogenide (TMD) monolayers and their heterostructures. Among the unconventional excitonic states,…

The predicted formation of moire superlattices leading to confined excitonic states in heterostructures formed by stacking two lattice mismatched transition metal dichalcogenide (TMD) monolayers was recently experimentally confirmed. Such…

The rich optical properties of transition metal dichalcogenide monolayers (TMD-MLs) render these materials promising candidates for the design of new optoelectronic devices. Despite the large number of excitonic complexes in TMD-MLs, the…

Excitons with binding energies of a few hundreds of meV control the optical properties of transition metal dichalcogenide monolayers. Knowledge of the fine structure of these excitons is therefore essential to understand the optoelectronic…

Atomically thin materials such as graphene and monolayer transition metal dichalcogenides (TMDs) exhibit remarkable physical properties resulting from their reduced dimensionality and crystal symmetry. The family of semiconducting…

We present first-principles calculations of the optical response of monolayer molybdenum disulfide employing the GW-Bethe Salpeter equation (GW-BSE) approach including self-energy, excitonic, and electron-phonon effects. We show that…

Materials Science · Physics 2014-06-30 Diana Y. Qiu , Felipe H. da Jornada , Steven G. Louie

Excitons dominate the optical properties of monolayer transition metal dichalcogenides (TMDs). Besides optically accessible bright exciton states, TMDs exhibit also a multitude of optically forbidden dark excitons. Here, we show that…

Monolayer transition-metal dichalcogenides (TMDs) provide a platform for realizing Wigner crystals and enable their detection via exciton spectroscopy. We develop a microscopic theoretical model for excitons interacting with the localized…

Strongly Correlated Electrons · Physics 2025-12-22 Haydn S. Adlong , Eugen Dizer , Richard Schmidt , Atac Imamoglu , Arthur Christianen

We demonstrate the integration of a thin BaTiO$_3$ (BTO) membrane with monolayer MoSe$_2$ in a dual gate device that enables in-situ manipulation of the BTO ferroelectric polarization with a voltage pulse. While two-dimensional (2D)…

Semiconducting transition metal dichalcogenides (TMDs), such as MoSe$_2$ and WSe$_2$, exhibit unique optical and electronic properties. Vertical stacking of layers of one or more TMDs, to create heterostructures, has expanded the fields of…

The interactions between charges and excitons involve complex many-body interactions at high densities. The exciton-polaron model has been adopted to understand the Fermi sea screening of charged excitons in monolayer transition metal…

Mesoscale and Nanoscale Physics · Physics 2023-09-14 Xin Cong , Parisa Ali Mohammadi , Mingyang Zheng , Kenji Watanabe , Takashi Taniguchi , Daniel Rhodes , Xiao-Xiao Zhang

We report magneto-optical spectroscopy of gated monolayer MoS$_2$ in high magnetic fields up to 28T and obtain new insights on the many-body interaction of neutral and charged excitons with the resident charges of distinct spin and valley…

Excitons in two-dimensional semiconductors provide a novel platform for fundamental studies of many-body interactions. In particular, dipolar interactions between spatially indirect excitons may give rise to strongly correlated phases of…

Mesoscale and Nanoscale Physics · Physics 2022-09-14 Rafał Ołdziejewski , Alessio Chiocchetta , Johannes Knörzer , Richard Schmidt

Heterostructures of layered transition metal dichalcogenides (TMDs) host long-lived, tunable excitons, making them intriguing candidates for material-based quantum information applications. Light absorption in these systems induces a…

Materials Science · Physics 2023-08-25 Tomer Amit , Sivan Refaely-Abramson

In heterostructures consisting of different transition-metal dichalcogenide monolayers, a staggered band alignment can occur, leading to rapid charge separation of optically generated electron-hole pairs into opposite monolayers. These…

Transition metal dichalcogenide (TMDC) monolayer has recently emerged as an important two-dimensional semiconductor with promising potentials for electronic and optoelectronic devices. Unlike semi-metallic graphene, layered TMDC has a…

Mesoscale and Nanoscale Physics · Physics 2014-10-16 Ziliang Ye , Ting Cao , Kevin O'Brien , Hanyu Zhu , Xiaobo Yin , Yuan Wang , Steven G. Louie , Xiang Zhang

Atomically thin semiconductors such as transition metal dichalcogenide (TMD) monolayers exhibit a very strong Coulomb interaction, giving rise to a rich exciton landscape. This makes these materials highly attractive for efficient and…

Mesoscale and Nanoscale Physics · Physics 2022-11-02 Raul Perea-Causin , Daniel Erkensten , Jamie M. Fitzgerald , Joshua J. P. Thompson , Roberto Rosati , Samuel Brem , Ermin Malic