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New propagation regimes for light arise from the ability to tune the dielectric permittivity to extremely low values. Here we demonstrate a universal approach based on the low linear permittivity values attained in the epsilon-near-zero…

Optical materials with vanishing dielectric permittivity, known as epsilon-near-zero (ENZ) materials, have been shown to possess enhanced nonlinear optical responses in their ENZ region. These strong nonlinear optical properties have been…

For decades, nonlinear optics has been used to control the frequency and propagation of light in unique ways enabling a wide range of applications such as ultrafast lasing, sub-wavelength imaging, and novel sensing methods. Through this, a…

Optics · Physics 2020-04-02 Ray Secondo , Jacob B. Khurgin , Nathaniel Kinsey

Epsilon-near-zero (ENZ) materials such as indium tin oxide (ITO), have recently emerged as a new platform to enhance optical nonlinearities. Here we report a theoretical and experimental study on the origin of nonlinearities in ITO thin…

We extend our previous study of the polarization dependence of the nonlinear optical response to the case of magnetic surfaces and buried magnetic interfaces. We calculate for the longitudinal and polar configuration the nonlinear…

Condensed Matter · Physics 2009-10-28 W. Hubner , K. H. Bennemann

Recently, materials with vanishingly small permittivity, known as epsilon-near-zero (ENZ) media, emerged as promising candidates to achieve nonlinear optical effects of unprecedented magnitude on a solid-state platform. In particular, the…

Optics · Physics 2023-09-18 Tornike Shubitidze , Wesley A. Britton , Luca Dal Negro

Low electron density Drude (LEDD) materials such as indium tin oxide (ITO) are receiving considerable attention because of their combination of CMOS compatibility, unique epsilon-near-zero (ENZ) behavior, and giant ultrafast nonlinear…

Optics · Physics 2024-04-15 Ieng Wai Un , Subhajit Sarkar , Yonatan Sivan

We show that standard approximations in nonlinear optics are violated for situations involving a small value of the linear refractive index. Consequently, the conventional equation for the intensity-dependent refractive index, $n(I) = n_0 +…

Nanophotonic devices offer an unprecedented ability to concentrate light into small volumes which can greatly increase nonlinear effects. However, traditional plasmonic materials suffer from low damage thresholds and are not compatible with…

Ultrathin plasmonic films that approach the trans-dimensional (TD) thickness limit provide a promising route for light_matter interaction control and manipulation, yet their nonlinear optical response near the epsilon_near_zero (ENZ)…

Over the last few decades, extensive previous studies of the nonlinear response of metal nanoparticles report a wide variation of nonlinear coefficients, thus, revealing a highly confused picture of the underlying physics. This naturally…

Optics · Physics 2020-10-28 Ieng Wai Un , Yoatan Sivan

Epsilon-near-zero materials are exceptional candidates for studying electrodynamics and nonlinear optical processes at the nanoscale. We demonstrate that by alternating a metal and a highly doped conducting-oxide, the epsilon-near-zero…

We show that a nonlinear optical response associated with a resonant, atomically thin material can be dramatically enhanced by placing it in front of a partially reflecting mirror, rendering otherwise weakly nonlinear systems suitable for…

Mesoscale and Nanoscale Physics · Physics 2018-09-25 Dominik S. Wild , Ephraim Shahmoon , Susanne F. Yelin , Mikhail D. Lukin

Novel materials, with enhanced light-matter interaction capabilities, play an essential role in achieving the lofty goals of nonlinear optics. Recently, Epsilon-Near-Zero (ENZ) media have emerged as a promising candidate to enable the…

Optics · Physics 2020-07-14 Jacob B. Khurgin , Matteo Clerici , Nathaniel Kinsey

Self-mode-locking has become an emerging path to the generation of ultrashort pulses with vertical-external-cavity surface-emitting lasers. In our work, a strong Kerr nonlinearity that is so far assumed to give rise to mode-locked operation…

The nonlinear magneto-optical Kerr-effect (NOLIMOKE) is determined for freestanding Fe monolayers with several in-plane structures from first principles. Based on the theory of nonlinear magneto-optics by H\"ubner and Bennemann [Phys. Rev.…

Materials Science · Physics 2009-10-31 J. P. Dewitz , W. Hübner

Based on the momentum-resolved Boltzmann equation, we provide self-consistent numerical calculations of the dynamics of conduction electrons in thin noble metal films after linear and non-linear optical excitations with infrared and…

Mesoscale and Nanoscale Physics · Physics 2025-04-29 Jonas Grumm , Malte Selig , Holger Lange , Andreas Knorr

The promise of active nanophotonics technology relies on the confinement and control of light at the nanoscale. Confinement via plasmonics, dielectric resonators, and waveguides can be complemented with materials whose optical properties…

The pronounced dependence of the nonlinear parameters of both dielectric and semiconductor materials on the wavelength, and the nonlinear interaction between the ultra-short laser pulse and the material requires precise control of the…

We solve the nonlinear Maxwell equations in an InP-based dielectric metamaterial, considering both two-photon absorption and photo-induced free-carrier absorption. We obtain the intensity-dependent reflection, absorption, and effective…

Optics · Physics 2018-01-10 Brian Slovick , Lucas Zipp , Srini Krishnamurthy
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