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We report on the first streaking measurement of water-window attosecond pulses generated via high harmonic generation, driven by sub-2-cycle, CEP-stable, 1850 nm laser pulses. Both the central photon energy and the energy bandwidth far…

Infrared femtosecond laser pulses are important tools both in strong-field physics, driving X-ray high-harmonic generation, and as the basis for widely tuneable, if inefficient, ultrafast sources in the visible and ultraviolet. Although…

Optics · Physics 2020-10-14 Christian Brahms , Federico Belli , John C. Travers

Electronic correlations occur on attosecond timescales, dictating how chemical bonds form, energy flows, and materials respond to light. Capturing such many-body processes requires light pulses of similar duration. The soft X-ray water…

A new method to coherently control the electron dynamics is proposed using a few-cycle laser pulse in combination with a controlling field. It is shown that this method not only broadens the attosecond pulse bandwidth, but also reduces the…

Atomic Physics · Physics 2015-04-06 Pengfei Lan , Peixiang Lu , Wei Cao , Yuhua Li , Xinlin Wang

Sub-10-attosecond pulses with half-cycle electric fields provide exceptional options to detect and manipulate electrons in the atomic timescale. However, the availability of such pulses is still challenging. Here, we propose a method to…

Plasma Physics · Physics 2021-05-26 Yinren Shou , Ronghao Hu , Zheng Gong , Jinqing Yu , Jia erh Chen , Gerard Mourou , Xueqing Yan , Wenjun Ma

The interaction between an ultrastrong laser and a cone-like target is an efficient approach to generate high power radiations like attosecond pulses and terahertz waves. The object is to study the $\gamma$-ray generation under this…

Plasma Physics · Physics 2022-06-28 Cui-Wen Zhang , Yi-Xuan Zhu , Jian-Feng Lv , Bai-Song Xie

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…

In recent years nanoscale coherent imaging has emerged as an indispensable imaging modality allowing to surpass the resolution limit given by classical imaging optics. At the same time, attosecond science has experienced enormous progress…

High-order harmonic generation (HHG) enables the up-conversion of intense infrared or visible femtosecond laser pulses into extreme-ultraviolet attosecond pulses. However, the highly nonlinear nature of the process results in low conversion…

We present a novel spectroscopic technique for second harmonic generation (SHG) using femtosecond laser pulses at 30~kHz repetition rate, which nevertheless provides high spectral resolution limited only by the spectrometer. The potential…

Harmonic generation from solid surfaces is a promising tool for producing high energy attosecond pulses. We report shaping of the harmonic spectrum to achieve the bandwidth necessary for attosecond pulse generation. The shaping is…

Plasma Physics · Physics 2019-03-27 A. Seyen , R. Kohn , U. Bovensiepen , D. von der Linde , A. Tarasevitch

We investigate the photoionization spectrum of helium by attosecond XUV pulses both in the spectral region of doubly excited resonances as well as above the double ionization threshold. In order to probe for convergence, we compare three…

Parametric amplification of attosecond coherent pulses around 100 eV at the single-atom level is demonstrated for the first time by using the 3D time-dependent Schr{\"o}dinger equation in high-harmonic generation processes from excited…

Optics · Physics 2020-08-26 C. Serrat , J. Seres , E. Seres , T-H. Dinh , N. Hasegawa , M. Nishikino , S. Namba

Many experiments in attosecond science will benefit from attosecond pulses at high repetition rates with sufficient photon flux for pump-probe experiments. We use 7fs, 800nm pulses from a non-collinear optical parametric chirped pulse…

Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…

We perform a detailed analysis of how high-order harmonic generation (HHG) and above-threshold ionization (ATI) can be controlled by a time-delayed attosecond-pulse train superposed to a strong, near-infrared laser field. In particular we…

Atomic Physics · Physics 2009-11-11 C. Figueira de Morisson Faria , P. Salieres , P. Villain , M. Lewenstein

Over the past few decades, following the first demonstration of ultrafast electron microscopy, numerous research groups have focused on achieving attosecond temporal resolution in electron microscopy with the goal of imaging electron and…

Recent advances in the field of attosecond science hold the promise of tracking electronic processes at the shortest space and time scales. Imaging methods that combine attosecond temporal with nanometer spatial resolution are currently out…

High harmonic generation (HHG) is used to measure the spectral phase of the recombination dipole matrix element (RDM) in argon over a broad frequency range that includes the 3p Cooper minimum (CM). The measured RDM phase agrees well with…

Atomic Physics · Physics 2015-06-17 S. B. Schoun , R. Chirla , J. Wheeler , C. Roedig , P. Agostini , L. F. DiMauro , K. J. Schafer , M. B. Gaarde

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

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