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Lead-halide perovskites were demonstrated to exhibit some of the largest known optical nonlinearities, yet their potential for frequency conversion remains largely untapped. Here we demonstrate ultra-broadband four-wave mixing of near- and…

Lead halide perovskites (LHPs) have emerged as an excellent class of semiconductors for next-generation solar cells and optoelectronic devices. Tailoring physical properties by fine-tuning the lattice structures has been explored in these…

Halide perovskites have indisputably exceptional optical and electronic properties, which are attractive for next-generation optoelectronic device technologies. We report on a reversible photoluminescence (PL) peak in iodide-based…

Lead halide perovskites (LHPs) exhibit outstanding optoelectronic properties, making them highly promising for applications in various optoelectronics devices. However, rapid ion migration in LHPs not only undermines device stability but…

The family of hybrid organic-inorganic lead-halide perovskites are the subject of intense interest for optoelectronic applications, from light-emitting diodes to photovoltaics to X-ray detectors. Due to the inert nature of most organic…

Quantum wells made of two-dimensional organic-inorganic hybrid perovskites (2D-PKs) offer a high degree of flexibility in tailoring optoelectronic properties through carrier confinement and functional interlayers. Compared to their 3D…

Ultrafast vibrational dynamics of inorganic-organic hybrid lead halide perovskite CH3NH3PbI$ in the room-temperature tetragonal phase is investigated under moderate photoexcitation slightly below the band gap. Time-resolved optical Kerr…

Materials Science · Physics 2021-11-02 Kunie Ishioka , Terumasa Tadano , Masatoshi Yanagida , Yasuhiro Shirai , Kenjiro Miyano

Direct visualization of ultrafast coupling between charge carriers and lattice degrees of freedom in photo-excited semiconductors has remained a long-standing challenge and is critical for understanding the light-induced physical behavior…

Two-dimensional organic-inorganic hybrid perovskite (2D-OIHP) quantum wells are emerging as promising light sources for quantum communication technologies, owing to their ability to generate polarization-encoded optical signals. In this…

Quantum Physics · Physics 2025-12-01 Shuyue Feng , Zijian Gan , Camryn J. Gloor , Wei You , Andrew M. Moran

Hybrid organic-inorganic halide perovskites have shown remarkable optoelectronic properties (1-3), believed to originate from correlated motion of charge carriers and the polar lattice forming large polarons (4-7). Few experimental…

The chiral organic-inorganic halide perovskites (OIHPs) are vital candidates for superior nonlinear optical (NLO) effects associated with circularly polarized (CP) light. NLO in chiral materials often couples with magnetic dipole (MD)…

Optics · Physics 2024-01-25 Daichi Okada , Fumito Araoka

Lead halide perovskites have recently been reported to demonstrate an exceptionally high nonlinear (Kerr) refractive index n$_2$ of up to 10$^{-8}$ cm$^2$/W in CH$_3$NH$_3$PbBr$_3$. Other researchers however observe different, substantially…

Optics · Physics 2023-12-12 Dusan Lorenc , Ayan Zhumekenov , Osman M. Bakr , Zhanybek Alpichshev

Polarised light is critical for a wide range of applications, but is usually generated by filtering unpolarised light, which leads to significant energy losses and requires additional optics. Herein, the direct emission of…

Development of advanced optical data storage, information encryption, and security labeling technologies requires low-cost materials exhibiting local, pronounced, and diverse modification of their structure-dependent optical properties…

Organometallic lead halide perovskites are highly efficient materials for solar cells and other optoelectronic applications due to their high quantum efficiency and exceptional semiconducting properties. A peculiarity of these perovskites…

The outstanding photovoltaic performances of lead halide perovskite (LHP) thin film solar cells are due in particular to the large diffusion length of photocarriers. The mechanism behind this property and its dependence on the various…

Lead halide perovskites have emerged as platforms for exciton-polaritonic studies at room temperature thanks to their excellent photoluminescence efficiency and synthetic versatility. In this work we find proof of strong exciton-photon…

Materials Science · Physics 2024-05-07 Maximilian Black , Mehdi Asadi , Parsa Darman , Finja Schillmöller , Sara Darbari , Nahid Talebi

2D organic-inorganic hybrid perovskites (2DHPs) consist of alternating anionic metal-halide and cationic organic layers. They have widely tunable structural and optical properties. We review the role of the organic cation in defining the…

Materials Science · Physics 2022-04-28 Daniel B. Straus , Cherie R. Kagan

The ultrafast optical Kerr effect (OKE) is widely used to investigate the structural dynamics and interactions of liquids, solutions and solids by observing their intrinsic nonlinear temporal responses through nearly-collinear four-wave…

Optics · Physics 2021-03-15 Lucas Huber , Sebastian Maehrlein , Feifan Wang , Yufeng Liu , Xiaoyang Zhu

Lead halide perovskites (LHPs) are promising materials for opto-electronics and photovoltaics, thanks to favorable characteristics and low manufacturing costs enabled by solution processing. In light of this, it is crucial to assess the…

Materials Science · Physics 2021-10-01 Giovanni Procida , Richard Schier , Ana M. Valencia , Caterina Cocchi
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