Related papers: Echoes in Unidirectionally Rotating Molecules
We theoretically and numerically analyze x-ray scattering from asymmetric-top molecules three-dimensionally aligned using elliptically polarized laser light. A rigid-rotor model is assumed. The principal axes of the polarizability tensor…
We investigate the prospects of creating broad rotational wave packets by means of molecular interaction with long sequences of intense femtosecond pulses. Using state-resolved rotational Raman spectroscopy of oxygen, subject to a sequence…
We consider deflection of rotating symmetric molecules by inhomogeneous optical and static electric fields, compare results with the case of linear molecules, and find new singularities in the distribution of the scattering angle.…
Ultrashort laser pulses pose unique tools to trigger and probe the fastest charge dynamics in matter, allowing the investigation of fundamental physical phenomena with unprecedented resolution in space, time, and energy. One of the most…
We present a theoretical investigation of coherent control over the orientation of an individual molecule strongly coupled with a cavity using chirped-pulse driving. Specifically, we explore the dynamics of carbonyl sulfide (OCS) molecules…
Molecular rotation spectra, generated by the coupling of the molecular electric-dipole moments to an external time-dependent electric field, are discussed in a few particular conditions which can be of some experimental interest. First, the…
The novel isotope and magnetic effects on two level system echoes in glasses observed by Nagel et al.(Phys.Rev.Lett. 92, 245511 (2004)) provide unique experimental insight into the nature of tunneling systems in amorphous solids. We show…
We present a general analysis for the interaction of a probe laser radiation with a coherently prepared molecular Raman medium. We describe a general formalism which includes dispersive effects, such as group velocity and group velocity…
Photoemission and tunneling spectroscopies measure the energies at which single electrons can be added to or removed from an electronic system. Features observed in such spectra have revealed electrons coupling to vibrational modes of ions…
The coherent reflectivity of a dense, relativistic, ultra-thin electron layer is derived analytically for an obliquely incident probe beam. Results are obtained by two-fold Lorentz transformation. For the analytical treatment, a plane…
A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…
Correlation among particles in finite quantum systems leads to complex behaviour and novel states of matter. One remarkable example is predicted to occur in a semiconductor quantum dot (QD) where at vanishing density the Coulomb correlation…
Impulsive orientation of symmetric-top molecules excited by two-color femtosecond pulses is considered. In addition to the well-known transient orientation appearing immediately after the pulse and then reemerging periodically due to…
We report on a combined experimental and theoretical study of polarization self-rotation in an ultracold atomic sample. In the experiments, a probe laser is tuned in the spectral vicinity of the D1 line to observe polarization self-rotation…
In collisions at ultralow temperatures, molecules will possess Feshbach resonances, foreign to ultracold atoms, whose virtual excited states consist of rotations of the molecules. We estimate the mean spacing and mean widths of these…
We demonstrate experimentally a method of all-optical selective rotational control in gas mixtures. Using an optical centrifuge - an intense laser pulse whose linear polarization rotates at an accelerated rate, we simultaneously excite two…
The generation of laser-driven dense relativistic electron layers from ultra-thin foils and their use for coherent Thomson backscattering is discussed, applying analytic theory and one-dimensional particle-in-cell simulation. The blow-out…
Chirality and chiral molecules are key elements in modern chemical and biochemical industries. Individual addressing, and the eventual separation of chiral enantiomers has been and still is an important elusive task in molecular physics and…
We report on the first experimental demonstration of enantioselective rotational control of chiral molecules with a laser field. In our experiments, two enantiomers of propylene oxide are brought to accelerated unidirectional rotation by…
We study the acceleration of ultra-high-energy cosmic rays (UHECRs) at FR-II radio galaxies by performing Monte Carlo simulations for the transport, scattering, and energy change of the CR particles injected into the time-evolving jet flows…