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Quantum chemistry is a promising application of future quantum computers, but the requirements on qubit count and other resources suggest that modular computing architectures will be required. We introduce an implementation of a quantum…

Quantum Physics · Physics 2026-01-26 Tian Xue , Jacob P. Covey , Matthew Otten

Although quantum computers are capable of solving problems like factoring exponentially faster than the best-known classical algorithms, determining the resources responsible for their computational power remains unclear. An important class…

Quantum Physics · Physics 2016-05-11 Nana Liu , Jayne Thompson , Christian Weedbrook , Seth Lloyd , Vlatko Vedral , Mile Gu , Kavan Modi

Quantum computing holds the potential to revolutionize various fields by efficiently tackling complex problems. At its core are quantum circuits, sequences of quantum gates manipulating quantum states. The selection of the right quantum…

Software Engineering · Computer Science 2024-06-13 Xiaoyu Guo , Takahiro Muta , Jianjun Zhao

In this tutorial-style review we discuss basic concepts of coupled cluster theory and recent developments that increase its computational efficiency for calculations of molecules, solids and materials in general. We will touch upon the…

Materials Science · Physics 2020-04-15 Igor Ying Zhang , Andreas Grüneis

This study introduces a systematic approach for analyzing strongly correlated systems by adapting the conventional quantum cluster method to a quantum circuit model. We have developed a more concise formula for calculating the cluster's…

Quantum Physics · Physics 2025-12-24 Hengyue Li , Yusheng Yang , Pin Lv , Jinglong Qu , Zhe-Hui Wang , Jian Sun , Shenggang Ying

The curse of dimensionality (COD) limits the current state-of-the-art {\it ab initio} propagation methods for non-relativistic quantum mechanics to relatively few particles. For stationary structure calculations, the coupled-cluster (CC)…

Quantum Physics · Physics 2015-06-03 Simen Kvaal

Basic concepts of quantum theory of information, principles of quantum calculations and the possibility of creation on this basis unique on calculation power and functioning principle device, named quantum computer, are briefly reviewed.…

Quantum Physics · Physics 2007-12-10 Steven Duplij , Illia Shapoval

In the molecular quantum chemistry community, coupled-cluster (CC) methods are well-recognized for their systematic convergence and reliability. The extension of the theory to extended systems has been comparably recent, so that…

Chemical Physics · Physics 2024-10-31 Andreas Grüneis , Evgeny Moerman , Matthias Scheffler , Tonghao Shen , Igor Ying Zhang

In a quantum computer any superposition of inputs evolves unitarily into the corresponding superposition of outputs. It has been recently demonstrated that such computers can dramatically speed up the task of finding factors of large…

Quantum Physics · Physics 2016-09-08 I. Chuang , Raymond Laflamme , P. Shor , W. Zurek

Quantum algorithms are promising candidates for the enhancement of computational efficiency for a variety of computational tasks, allowing for the numerical study of physical systems intractable to classical computers. In the Noisy…

Quantum Physics · Physics 2021-05-13 Marco Majland , Nikolaj Thomas Zinner

We propose an approach to approximately implement the variational coupled cluster (VCC) theory on quantum computers, which struggles with exponential scaling of computational costs on classical computers. To this end, we employ expanding…

Quantum Physics · Physics 2024-06-12 Luca Erhart , Yuichiro Yoshida , Viktor Khinevich , Wataru Mizukami

An accurate description of strong correlation is quintessential for the exploration of emerging chemical phenomena. While near-term variational quantum algorithms provide a theoretically scalable framework for quantum chemical problems, the…

Quantum Physics · Physics 2025-10-20 Arpan Choudhury , Sonaldeep Halder , Rahul Maitra , Debashree Ghosh

Solving electronic structure problems is considered one of the most promising applications of quantum computing. However, due to limitations imposed by the coherence time of qubits in the Noisy Intermediate Scale Quantum (NISQ) era or the…

Quantum Physics · Physics 2025-03-20 Shuo Sun , Chandan Kumar , Kevin Shen , Elvira Shishenina , Christian B. Mendl

Variational quantum algorithms involve training parameterized quantum circuits using a classical co-processor. An important variational algorithm, designed for combinatorial optimization, is the quantum approximate optimization algorithm.…

We introduce the multistate iterative qubit coupled cluster (MS-iQCC) method, a quantum-inspired algorithm that runs efficiently on classical hardware and is designed to predict both ground and excited electronic states of molecules.…

Chemical Physics · Physics 2026-01-05 Robert A. Lang , Shashank G. Mehendale , Ilya G. Ryabinkin , Artur F. Izmaylov

Quantum algorithms are able to solve particular problems exponentially faster than conventional algorithms, when implemented on a quantum computer. However, all demonstrations to date have required already knowing the answer to construct…

Quantum Physics · Physics 2013-03-22 Xiao-Qi Zhou , Pruet Kalasuwan , Timothy C. Ralph , Jeremy L. O'Brien

We present a quantum variational algorithm based on a novel circuit that generates all permutations that can be spanned by one- and two-qubits permutation gates. The construction of the circuits follows from group-theoretical results, most…

Quantum Physics · Physics 2026-02-11 Dylan Laplace Mermoud , Andrea Simonetto , Sourour Elloumi

The quantum model of a cluster, consisting of A identical particles, coupled by the internal pair interactions and affected by the external field of a target, is considered. A symbolic-numerical algorithm for generating A-1-dimensional…

We demonstrate the use of the Variational Quantum Eigensolver (VQE) to simulate solid state crystalline materials. We adapt the Unitary Coupled Cluster ansatz to periodic boundary conditions in real space and momentum space representations…

Measurement-based quantum computation (MBQC) represents a powerful and flexible framework for quantum information processing, based on the notion of entangled quantum states as computational resources. The most prominent application is the…

Quantum Physics · Physics 2014-05-26 B. P. Lanyon , P. Jurcevic , M. Zwerger , C. Hempel , E. A. Martinez , W. Dür , H. J. Briegel , R. Blatt , C. F. Roos
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