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We theoretically consider the phenomenon of field-free long-lasting orientation of symmetric-top molecules ionized by two-color laser pulses. The anisotropic ionization produces a significant long-lasting orientation of the surviving…

Chemical Physics · Physics 2023-03-08 Long Xu , Ilia Tutunnikov , Yehiam Prior , Ilya Sh. Averbukh

Chirality and chiral molecules are key elements in modern chemical and biochemical industries. Individual addressing, and the eventual separation of chiral enantiomers has been and still is an important elusive task in molecular physics and…

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

We discuss how tensorial observables, available in photoelectron angular distributions resulting from interaction between isotropic chiral samples and cross polarized $\omega$-$2\omega$ bichromatic fields, allow for chiral discrimination…

Atomic Physics · Physics 2022-06-28 Andres F. Ordonez , Olga Smirnova

We analize the dipole spectrum of a two-level atom excited by a non-resonant intense monochromatic field, under the electric dipole approximation and beyond the rotating wave approximation. We show that the apparently complex spectral…

Optics · Physics 2010-03-25 A. Picón , L. Roso , J. Mompart , O. Varela , V. Ahufinger , R. Corbalán , L. Plaja

Enantiodetection of chiral molecules is important to pharmaceutical drug production, chemical reaction control, and biological function designs. Traditional optical methods of enantiodetection rely on the weak magnetic-dipole or…

Chemical Physics · Physics 2022-09-14 Mao-Rui Cai , Chong Ye , Hui Dong , Yong Li

Quantum information is often carried in the frequency and polarization degrees of freedom (DoFs) in single photons and entangled photons. We demonstrate a new approach to couple and decouple the frequency and polarization DoFs of broadband…

Quantum Physics · Physics 2023-11-27 Arash Riazi , Eric Y. Zhu , Dan Xu , Li Qian

Engineering of intensity and direction of radiation from a single quantum emitter by means of structuring of their environment at the nanoscale is at the cornerstone of modern nanophotonics. Recently discovered systems exhibiting…

Optics · Physics 2015-08-13 Sergey Lee , Denis Baranov , Alexander Krasnok , Pavel Belov

Strong-field ionization by counter-rotating two-color laser fields produces quantum interference between photoelectrons emitted on the leading and trailing edges of the laser field oscillations. We show that in chiral molecules, this…

Quantum interference between one- and two-photon absorption pathways allows coherent control of interband transitions in unbiased bulk semiconductors; carrier population, carrier spin polarization, photocurrent injection, and spin current…

Other Condensed Matter · Physics 2007-05-23 R. D. R. Bhat , J. E. Sipe

Entangled photon sources are crucial for quantum optics, quantum sensing and quantum communication. Semiconductor quantum dots generate on-demand entangled photon pairs via the biexciton-exciton cascade. However, the pair of photons are…

Quantum Physics · Physics 2019-07-09 Mohd Zeeshan , Nachiket Sherlekar , Arash Ahmadi , Robin L Williams , Michael E Reimer

We study the effects of a static electric field on the photoassociation of a heteronuclear atom-pair into a polar molecule. The interaction of permanent dipole moment with a static electric field largely affects the ground state continuum…

Atomic Physics · Physics 2015-05-27 Debashree Chakraborty , Jisha Hazra , Bimalendu Deb

Two mechanisms of two-color (\omega + 2\omega) laser-induced field-free molecular orientation, based on the hyperpolarizability and ionization depletion, are explored and compared. The CO molecule is used as a computational example. While…

Atomic Physics · Physics 2012-09-14 Michael Spanner , Serguei Patchkovskii , Eugene Frumker , Paul Corkum

Entangled photons are crucial for quantum technologies, but generating arbitrary entangled photon states deterministically, efficiently, and with high fidelity remains a challenge. Here, we demonstrate how hybridization and dipole-dipole…

Quantum Physics · Physics 2022-04-06 Derek S Wang , Inci Anali , Susanne F Yelin

Enantioselective orientation of chiral molecules excited by a shaped picosecond laser pulse and a delayed femtosecond pulse is considered. Using quantum mechanical simulations, we demonstrate a strong field-free enantioselective orientation…

Optics · Physics 2022-03-31 Long Xu

We show that the photoelectron angular distributions produced by elliptical and cross-polarized two-color laser fields interacting with randomly oriented chiral molecules decompose into four irreducible representations of the $D_{2h}$ point…

We study non-perturbative effects of a static electric field on two-color photoassociation of different atoms. A static electric field induces anisotropy in scattering between two different atoms and hybridizes field-free rotational states…

Atomic Physics · Physics 2014-05-08 Debashree Chakraborty , Bimalendu Deb

The effect of a strong magnetic field on the electric polarization of a three-flavor color superconducting medium is investigated. We found that the electric susceptibility of this strongly magnetized medium is highly anisotropic. In the…

Nuclear Theory · Physics 2015-05-30 Bo Feng , Efrain J. Ferrer , Vivian de la Incera

We propose a gain-assisted enantioselective scheme in dye-doped chiral particles, demonstrating optical pulling and pushing forces that can be tuned using externally controllable parameters. By controlling the concentration of dye molecules…

Today we are witnessing the electric-dipole revolution in chiral measurements. Here we reflect on its lessons and outcomes, such as the perspective on chiral measurements using the complementary principles of "chiral reagent" and "chiral…

Optics · Physics 2022-11-30 David Ayuso , Andres F. Ordonez , Olga Smirnova