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In this work we report studies of nitrogen adsorption and desorption onto solid surfaces using computer simulations of the three dimensional Ising model, for systems with complex porous structures at the mesoscopic and microscopic levels. A…

Soft Condensed Matter · Physics 2015-03-17 M. A. Balderas Altamirano , S. Cordero , G. Roman , A. Gama Goicochea

In cold astrophysical environments, some molecules are observed in the gas phase whereas they should have been depleted, frozen on dust grains. In order to solve this problem, astrochemists have proposed that a fraction of molecules…

Chemical Physics · Physics 2016-03-02 Minissale Marco , Dulieu François

The static friction between crystalline surfaces separated by a molecularly thin layer of adsorbed molecules is calculated using molecular dynamics simulations. These molecules naturally lead to a finite static friction that is consistent…

Materials Science · Physics 2009-11-07 Gang He , Mark O. Robbins

The synthesis of molecular magnets has undergone rapid progress in recent years. Each of the identical molecular units can contain as few as two and up to several dozens of paramagnetic ions (spins). Although these materials appear as…

Strongly Correlated Electrons · Physics 2009-11-11 J. Schnack

We calculate the electronic structure and magnetic properties of hydrogenated graphite surfaces using van der Waals density functional theory (DFT) and model Hamiltonians. We find, as previously reported, that the interaction between…

Mesoscale and Nanoscale Physics · Physics 2015-03-06 M. Moaied , J. V. Alvarez , J. J. Palacios

The adsorption of a single polymer to a flat surface in shear is investigated using Brownian hydrodynamics simulations and scaling arguments. Competing effects are disentangled: in the absence of hydrodynamic interactions, shear drag…

Soft Condensed Matter · Physics 2015-05-20 Andreas Serr , Christian Sendner , Florian Mueller , Thomas R. Einert , Roland R. Netz

Very often it is an implied paradigm of molecular magnetism that magnetic molecules in a crystal interact so weakly that measurements of dc magnetic observables reflect ensemble properties of single molecules. But the number of cases where…

Strongly Correlated Electrons · Physics 2016-03-02 J. Schnack

The confluence between high-energy physics and condensed matter has produced groundbreaking results via unexpected connections between the two traditionally disparate areas. In this work, we elucidate additional connectivity between…

Mesoscale and Nanoscale Physics · Physics 2023-08-02 Joseph Sklenar , Soho Shim , Hilal Saglam , Junseok Oh , M. G. Vergniory , Axel Hoffmann , Barry Bradlyn , Nadya Mason , Matthew J. Gilbert

Using first-principles calculations, we show that the magnetic properties of a two-dimensional antiferromagnetic transition-metal surface are modified on the atomic scale by the adsorption of small organic molecules. We consider benzene…

Materials Science · Physics 2015-06-16 Nuala M. Caffrey , Paolo Ferriani , Simone Marocchi , Stefan Heinze

Recent experiments have elucidated that novel nonequilibrium states inherent in the so-called hydrodynamic regime are realized in ultrapure metals with sufficiently strong momentum-conserving scattering. In this letter, we formulate a…

Mesoscale and Nanoscale Physics · Physics 2021-12-21 Ryotaro Sano , Riki Toshio , Norio Kawakami

The adsorption of $CO_2$ on the $Fe_3$$O_4$(001)-($\sqrt{2}$ $\times$ $\sqrt{2}$)R45{\deg} surface was studied experimentally using temperature programmed desorption (TPD), electron spectroscopies (UPS and XPS), and scanning tunneling…

We develop several configuration interaction approaches for characterizing the electronic structure of an adsorbate on a metal surface (at least in model form). When one can separate adsorbate from substrate, these methods can achieve a…

Chemical Physics · Physics 2020-02-26 Zuxin Jin , Wenjie Dou , Joseph E. Subotnik

A non-equilibrium thermodynamics model able to analyze the combined effect of diffusion and adsorption in porous materials is proposed. The model considers the coupled dynamics of the diffusive phase, described by a diffusion type equation,…

Materials Science · Physics 2015-06-04 I. Santamaria-Holek , Z. J. Grzywna , J. M. Rubi

The magnetic coupling between single Co atoms adsorbed on a copper surface is determined by probing the Kondo resonance using low-temperature scanning tunneling spectroscopy. The Kondo resonance, which is due to magnetic correlation effects…

Strongly Correlated Electrons · Physics 2007-05-23 P. Wahl , P. Simon , L. Diekhoener , V. S. Stepanyuk , P. Bruno , M. A. Schneider , K. Kern

The anisotropic magnetoresistance (AMR) in thin permalloy strips was calculated at each steps during magnetization by the finite element method. The magnetization at equilibrium under different external fields was obtained by micromagnetic…

Materials Science · Physics 2019-05-01 Wanli Zhang , Jing Chen , Wenxu Zhang

The magnetic moment of an electron gas on the surface of constant negative curvature is investigated. It is shown that the surface curvature leads to the appearance of the region of the monotonic dependence $M(B)$ at low magnetic fields. At…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 D. V. Bulaev , V. A. Margulis

Most of the studies on the adsorption of F$^-$ are experimental, and have been done with synthetic solutions. Such studies rarely mimic the field situation. Therefore, selection of an adsorbent that can remove F$^-$ from any kind of feed…

Chemical Physics · Physics 2017-02-27 Naga Samrat MVV , Gandhi K S , Kesava Rao K

Detailed semi-empirical interaction potential calculations are performed to determine the potential energy surface experienced by the molecules CO, HCN, H2O and H2CO, when adsorbed on the basal plane (0001) of graphite at low temperature.…

Chemical Physics · Physics 2015-05-13 Azzedine Lakhlifi , John P. Killingbeck

Our ab initio calculations of CO adsorption energies on low miller index (111), (100), stepped (211), and kinked (532) gold surfaces show a strong dependence on local coordination with a reduction in Au atom coordination leading to higher…

Materials Science · Physics 2009-11-13 F. Mehmood , A. Kara , T. S. Rahman , C. R. Henry

We study the chemisorption of CO molecule into sites of different coordination on (111) surfaces of late 4d and 5d transition metals. In an attempt to solve the well-known CO adsorption puzzle we have applied the relatively new vdW-DF…

Materials Science · Physics 2008-10-14 P. Lazic , M. Alaei , N. Atodiresei , V. Caciuc , R. Brako , S. Blugel