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Atom probe tomography (APT) analysis conditions play a major role in the composition measurement accuracy. Preferential evaporation, which significantly biases apparent composition, more than other well-known phenomena in APT, is strongly…

Electron evaporation plays an important role in the electron temperature evolution and thus expansion rate in low-density ultracold plasmas. In addition, evaporation is useful as a potential tool for obtaining colder electron temperatures…

Plasma Physics · Physics 2017-06-07 Craig Witte , Jacob L. Roberts

Atom probe tomography (APT) is a 3D analysis technique that offers unique chemical accuracy and sensitivity with sub-nanometer spatial resolution. Recently, there is an increasing interest in the application of APT to complex oxides…

Atom probe tomography data is composed of a list of coordinates of the reconstructed atoms in the probed volume. The elemental identity of each atom is derived from time-of-flight mass spectrometry, with no local energetic or chemical…

A new simulation approach of field evaporation is presented. The model combines classical electrostatics with molecular dynamics (MD) simulations. Unlike previous atomic-level simulation approaches, our method does not rely on an…

Materials Science · Physics 2022-10-17 Jiayuwen Qi , Christian Oberdorfer , Emmanuelle A. Marquis , Wolfgang Windl

In atom probe tomography (APT), atoms from the surface of a needle shape specimen are evaporated under a high electric field and analyzed via time of flight mass spectrometry and position sensitive detection. 3D reconstruction of the atom…

Materials Science · Physics 2023-11-28 Jiayuwen Qi , Fei Xue , Emmanuelle Marquis , Wolfgang Windl

Imaging of liquids and cryogenic biological materials by electron microscopy has been recently enabled by innovative approaches for specimen preparation and the fast development of optimised instruments for cryo-enabled electron microscopy…

We report the application of evaporative cooling to clouds of trapped antiprotons, resulting in plasmas with measured temperature as low as 9~K. We have modeled the evaporation process for charged particles using appropriate rate equations.…

The simulations of field-evaporation processes for silicon atoms on various Si(001) surfaces are implemented using the first-principles calculations based on the real-space finite-difference method. We find that the atoms which locate on…

Condensed Matter · Physics 2009-11-10 Tomoya Ono , Kikuji Hirose

There has been an increasing interest in atom probe tomography (APT) to characterise hydrated and biological materials. A major benefit of APT compared to microscopy techniques more commonly used in biology is its combination of outstanding…

Applied Physics · Physics 2023-11-13 Florant Exertier , Levi Tegg , Adam Taylor , Julie M. Cairney , Jing Fu , Ross K. W. Marceau

The purpose of this work is to identify the field evaporation mechanism associated with charge density distribution under extreme fields, linking atom probe tomography (APT) experiments with density functional theory (DFT) modeling. DFT is…

Materials Science · Physics 2016-12-21 Claudia Loyola , Joaquin Peralta , Scott R. Broderick , Krishna Rajan

Atom probe tomography (APT) fills a crucial need in the characterization workflow of materials by its ability to inform the 3D chemical microstructure at the nanoscale. As with any characterization techniques, APT has strengths and…

The experimental - calculated method is proposed to determine the full energy peak efficiency (FEPE) of detectors {\epsilon}(E) in case a measurement of the large-volume samples. Water is used as standard absorber in which the linear…

Instrumentation and Detectors · Physics 2012-07-20 E. G. Tertyshnik , A. T. Korsakov

We develop a theoretical model for calibrating the absorption imaging of cold atoms under high magnetic fields. Comparing to zero or low magnetic fields, the efficiency of the absorption imaging becomes lower while it requires an additional…

Atomic Physics · Physics 2023-07-20 Yuqi Liu , Zhongchi Zhang , Shiwan Miao , Zihan Zhao , Huaichuan Wang , Wenlan Chen , Jiazhong Hu

Atom probe tomography is frequently employed to characterize the elemental distribution in solids with atomic resolution. Here we review and discuss the potential of this technique to locally probe chemical bonds. Two processes characterize…

The modeling of deposition rates in Thermal Laser Epitaxy (TLE) is essential for the accurate prediction of the evaporation process and for improved dynamic process control. We demonstrate excellent agreement between experimental data and a…

Computational Engineering, Finance, and Science · Computer Science 2025-01-06 Thomas J. Smart , Bilen Emek Abali , Hans Boschker , Wolfgang Braun

In atom probe tomography (APT), accurate reconstruction of the spatial positions of field evaporated ions from measured detector patterns depends upon a correct understanding of the dynamic tip shape evolution and evaporation laws of…

We use transition path sampling to study evaporation in the SPC/E model of liquid water. Based on thousands of evaporation trajectories, we characterize the members of the transition state ensemble (TSE), which exhibit a liquid-vapor…

Soft Condensed Matter · Physics 2014-09-05 Patrick Varilly , David Chandler

We report a thorough investigation into the absorptive and dispersive properties of hot caesium vapour, culminating in the development of a simple analytical model for off-resonant Faraday rotation. The model, applicable to all hot alkali…

Atomic Physics · Physics 2015-05-28 Stefan L Kemp , Ifan G Hughes , Simon L Cornish

We present a combined computational and experimental study to optimize the efficiency of evaporative cooling for atoms in optical dipole traps. By employing a kinetic model of evaporation, we provide a strategy for determining the optimal…

Quantum Gases · Physics 2013-05-21 Abraham J. Olson , Robert J. Niffenegger , Yong P. Chen
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