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We propose an alternative scenario for the generation of entanglement between rotational quantum states of two polar molecules. This entanglement arises from dipole-dipole interaction, and is controlled by a sequence of laser pulses…

Quantum Physics · Physics 2016-08-16 Eric Charron , Pérola Milman , Arne Keller , Osman Atabek

Realising quantum control and entanglement of particles is crucial for advancing both quantum technologies and fundamental science. Significant developments in this domain have been achieved in a variety of systems. In this context,…

Atomic Physics · Physics 2025-01-27 Daniel K. Ruttley , Tom R. Hepworth , Alexander Guttridge , Simon L. Cornish

Polar molecules are an emerging platform for quantum technologies based on their long-range electric dipole-dipole interactions, which open new possibilities for quantum information processing and the quantum simulation of strongly…

In proposals for quantum computers using arrays of trapped ultracold polar molecules as qubits, a strong external field with appreciable gradient is imposed in order to prevent quenching of the dipole moments by rotation and to distinguish…

Quantum Physics · Physics 2015-05-27 Qi Wei , Sabre Kais , Bretislav Friedrich , Dudley Herschbach

Due to their intrinsic electric dipole moments and rich internal structure, ultracold polar molecules are promising candidate qubits for quantum computing and for a wide range of quantum simulations. Their long-lived molecular rotational…

We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…

Atomic Physics · Physics 2015-05-30 Mikhail Lemeshko , Bretislav Friedrich

While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a…

Atomic Physics · Physics 2013-02-27 Felipe Herrera , Sabre Kais , K. Birgitta Whaley

Entangled states of two coupled polar molecules controlled by laser pulses are studied theoretically. Schmidt decomposition is used to measure the degree of entanglement. By varying the pulse shape of the applied laser, transition from…

Atomic and Molecular Clusters · Physics 2007-05-23 Y. Y. Liao , Y. N. Chen , D. S. Chuu

Molecules have vibrational, rotational, spin-orbit and hyperfine degrees of freedom or quantum states, each of which responds in a unique fashion to external electromagnetic radiation. The control over superpositions of these quantum states…

Quantum Physics · Physics 2024-04-29 Svetlana Kotochigova , Qingze Guan , Eite Tiesinga , Vito Scarola , Brian DeMarco , Bryce Gadway

Fully internal and motional state controlled and individually manipulable polar molecules are desirable for many quantum science applications leveraging the rich state space and intrinsic interactions of molecules. While prior efforts at…

Ultracold polar molecules uniquely combine a rich structure of long-lived internal states with access to controllable long-range, anisotropic dipole-dipole interactions. In particular, the rotational states of polar molecules confined in…

Ultracold molecules trapped in optical tweezers show great promise for the implementation of quantum technologies and precision measurements. We study a prototypical scenario where two interacting polar molecules placed in separate traps…

Proposals for quantum computing using rotational states of polar molecules as qubits have previously considered only diatomic molecules. For these the Stark effect is second-order, so a sizable external electric field is required to produce…

Quantum Physics · Physics 2015-05-30 Qi Wei , Sabre Kais , Bretislav Friedrich , Dudley Herschbach

Polar molecules, with their rich internal structure, offer immense potential for fundamental physics, quantum technology, and controlled chemistry. However, their utilization is currently limited because of slow and imperfect state…

Quantum Physics · Physics 2026-02-16 Chi Zhang , Sara Murciano , Nathanan Tantivasadakarn , Ran Finkelstein

Selection of "magic" trapping conditions with ultracold atoms or molecules, where pairs of internal states experience identical trapping potentials, brings substantial benefits to precision measurements and quantum computing schemes.…

Quantum Physics · Physics 2011-01-04 Svetlana Kotochigova , David DeMille

Entanglement is one of the most fascinating features arising from quantum-mechanics and of great importance for quantum information science. Of particular interest are so-called hybrid-entangled states which have the intriguing property…

This article investigates entanglement of the motional states of massive coupled oscillators. The specific realization of an idealized diatomic molecule in one-dimension is considered, but the techniques developed apply to any massive…

Quantum Physics · Physics 2015-03-13 N. L. Harshman , W. F. Flynn

We investigate magic-wavelength trapping of ultracold bialkali molecules in the vicinity of weak optical transitions from the vibrational ground state of the X$^1\Sigma^+$ potential to low-lying rovibrational states of the b$^3\Pi_0$…

Quantum Physics · Physics 2021-04-14 Q. Guan , S. L. Cornish , S. Kotochigova

We show how state-dependent optical potentials can be used to trap a pair of molecules in different internal states at a separation much smaller than the wavelength of the trapping light. This close spacing greatly enhances the…

Atomic Physics · Physics 2021-04-05 L. Caldwell , M. R. Tarbutt

Entanglement is crucial to many quantum applications including quantum information processing, simulation of quantum many-body systems, and quantum-enhanced sensing. Molecules, because of their rich internal structure and interactions, have…

Quantum Gases · Physics 2024-06-18 Connor M. Holland , Yukai Lu , Lawrence W. Cheuk
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